Methane adsorption and methanol desorption of copper modified boron silicate

Wang Xueting; Shishkin Alexander; Hemmingsson Felix; Skoglundh Magnus; Martinez-Casado Francisco Javier; Bock Lorenz; Idstrom Alexander; Nordstierna Lars; Harelind Hanna; Carlsson Per-Anders

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Methane adsorption and methanol desorption of copper modified boron silicate

机译：甲烷吸附和甲醇解吸铜改性硼硅酸盐

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Boron silicate (BS) with a chabazite framework structure was synthesised using a direct route and rigorously characterized before it was ion-exchanged with copper to form Cu-BS. Employing in situ infrared spectroscopy, we show that Cu-BS is capable of oxidising methane to methoxy species and methanol interacts with the boron sites without deprotonation.

机译：使用直接途径合成具有Chabazite框架结构的硼硅酸盐（BS），并且在用铜进行离子交换以形成Cu-Bs之前，合成了砾岩骨架结构。在原位红外光谱中使用，我们表明Cu-BS能够将甲烷氧化成甲氧基物种，甲醇与硼部位的不含去质子化相互作用。

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来源
《RSC Advances》 |2018年第63期|共6页
作者
Wang Xueting; Shishkin Alexander; Hemmingsson Felix; Skoglundh Magnus; Martinez-Casado Francisco Javier; Bock Lorenz; Idstrom Alexander; Nordstierna Lars; Harelind Hanna; Carlsson Per-Anders;
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作者单位

Chalmers Univ Technol Dept Chem &

Chem Engn S-41296 Gothenburg Sweden;

Chalmers Univ Technol Dept Chem &

Chem Engn S-41296 Gothenburg Sweden;

Chalmers Univ Technol Dept Chem &

Chem Engn S-41296 Gothenburg Sweden;

Chalmers Univ Technol Dept Chem &

Chem Engn S-41296 Gothenburg Sweden;

Lund Univ MAX Lab 4 S-22100 Lund Sweden;

Chalmers Univ Technol Dept Chem &

Chem Engn S-41296 Gothenburg Sweden;

Chalmers Univ Technol Dept Chem &

Chem Engn S-41296 Gothenburg Sweden;

Chalmers Univ Technol Dept Chem &

Chem Engn S-41296 Gothenburg Sweden;

Chalmers Univ Technol Dept Chem &

Chem Engn S-41296 Gothenburg Sweden;

Chalmers Univ Technol Dept Chem &

Chem Engn S-41296 Gothenburg Sweden;

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正文语种 eng
中图分类化学;
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1. Methane adsorption and methanol desorption of copper modified boron silicate [J] . Wang Xueting, Shishkin Alexander, Hemmingsson Felix, RSC Advances . 2018,第63期

机译：甲烷吸附和甲醇解吸铜改性硼硅酸盐
2. Adsorption and Desorption Performance of Dichloromethane over Activated Carbons Modified by Metal Ions [J] . Hongyan Pan, Min Tian, Hui Zhang Journal of Chemical and Engineering Data: the ACS Journal for Data . 2013,第9期

机译：金属离子改性活性炭对二氯甲烷的吸附和解吸性能
3. Copper-Modified Zeolites and Silica for Conversion of Methane to Methanol [J] . Xueting Wang, Natalia M. Martin, Johan Nilsson, Catalysts . 2018,第11期

机译：铜改性沸石和二氧化硅，可将甲烷转化为甲醇
4. Study of Cadmium Adsorption and Desorption by Simulant Acid Rain on Different Silicate Clay Minerals in Soil [C] . Zhu Xiaping 2010 4th International Conference on Bioinformatics and Biomedical Engineering . 2010

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Methane adsorption and methanol desorption of copper modified boron silicate

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