One-pot construction of carbohydrate scaffolds mediated by metal catalysts

Mukherjee Mana Mohan; Maity Sajal Kumar; Ghosh Rina

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One-pot construction of carbohydrate scaffolds mediated by metal catalysts

机译：金属催化剂介导的碳水化合物支架的一锅施工

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Owing to the environmental concern worldwide and also due to cost, time and labour issues, use of one-pot reactions [domino/cascade/tandem/multi-component (MC) or sequential] has gained much attention among the scientific and industrial communities for the generation of compound libraries having different scaffolds. Inclusion of sugars in such compounds is expected to increase the pharmacological efficacy because of the possibility of better interactions with the receptors of such unnatural glycoconjugates. In many of the one-pot transformations, the presence of a metal salt/complex can improve the reaction/change the course of reaction with remarkable increase in chemo-/regio-/stereo-selectivity. On the other hand because of the importance of natural polymeric glycoconjugates in life processes, the development and efficient synthesis of related oligosaccharides, particularly utilising one-pot MC-glycosylation techniques are necessary. The present review is an endeavour to discuss one-pot transformations involving carbohydrates catalysed by a metal salt/complex.

机译：由于全世界环境所关注，而且由于成本，时间和劳动问题，使用单锅反应[Domino / Cascade / Tandem / Mod-Component（MC）或顺序]在科学和工业社区中获得了很多关注具有不同支架的复合文库的产生。由于可能与这种非自然糖缀合物的受体更好地相互作用，预期在这些化合物中包含糖的包含增加药理学效果。在许多单壶转化中，金属盐/复合物的存在可以改善反应/改变反应的过程，以显着增加的化学/测定/立体选择性。另一方面，由于生命过程中天然聚合物糖凝集物的重要性，需要相关寡糖的显影和有效合成，特别是利用单锅MC-糖基化技术是必要的。本综述是努力讨论涉及由金属盐/络合物催化的碳水化合物的单锅转化。

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《RSC Advances》 |2020年第54期|共26页
作者
Mukherjee Mana Mohan; Maity Sajal Kumar; Ghosh Rina;
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作者单位

NIDDK Lab Cell &

Mol Biol NIH Bethesda MD 20892 USA;

Jadavpur Univ Dept Chem Kolkata 700032 India;

Jadavpur Univ Dept Chem Kolkata 700032 India;

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正文语种 eng
中图分类化学;
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1. One-pot construction of carbohydrate scaffolds mediated by metal catalysts [J] . Mukherjee Mana Mohan, Maity Sajal Kumar, Ghosh Rina RSC Advances . 2020,第54期

机译：金属催化剂介导的碳水化合物支架的一锅施工
2. Ultrasound-Mediated One-Pot Synthesis of 7-Methyl-Substituted Pyrido[4,3-d]pyrimidine Scaffolds by a Catalyst-Free Protocol [J] . Sarmah Manas M., Prajapati Dipak Synlett . 2015,第1期

机译：超声介导的无催化剂方案一锅法合成7-甲基取代的吡啶并[4,3-d]嘧啶骨架
3. Polyoxometalate-based ionic complexes immobilized in mesoporous silicas prepared via a one-pot procedure: Efficient and reusable catalysts for H2O2-mediated alcohol oxidations in aqueous media [J] . Haihong Zhao, Linxiang Zeng, Yunlong Li Microporous and mesoporous materials: The offical journal of the International Zeolite Association . 2013,第Null期

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4. CoFe_2O_4 magnetic catalyst assisted a facile one-pot multicomponent construction of 2,4,5-trisubstituted-1H-imidazole derivatives [C] . A. H. Cahyana, B. Ardiansah, A. Mubardiani International Symposium on Current Progress in Mathematics and Sciences . 2018

机译：CoFe_2O_4磁性催化剂辅助2,4,5-三取代-1H-咪唑衍生物的容易一锅多组分构建
5. New developments toward the synthesis of heterocycles and applications in green chemistry. I. A simple and essentially one-pot synthesis of N-aminated heterocycles using phase transfer catalyst (Aliquat-336). II. Synthesis of pharmaceutically important pyrrole derivatives. III. Applications in green chemistry: Surfactant-mediated environmentally friendly cleavage of aromatic esters and trans-esterification under solvent-free neutral conditions . [D] . Patel, Nitinchandra. 2005

机译：杂环合成的新进展及其在绿色化学中的应用。 I.使用相转移催化剂（Aliquat-336）简单且基本上一锅合成N-胺化的杂环。二。药学上重要的吡咯衍生物的合成。三，在绿色化学中的应用：在无溶剂的中性条件下，表面活性剂介导的环境友好的芳族酯裂解和酯交换反应。
6. An Efficient One-Pot Protocol for the Synthesis of Substituted 34-Dihydropyrimidin-2(1H)-ones Using Metallophthalocyanines (MPcs) as Potent Heterogeneous Catalysts: Synthesis Characterization Aggregation and Antimicrobial Activity [O] . Naceur Hamdi, Rawdha Medyouni, Hallouma Bilel, 2017

机译：使用金属酞菁（MPcs）作为强效多相催化剂合成取代的34-二氢嘧啶-2（1H）-酮的高效一锅方案：合成表征聚集和抗菌活性
7. Use of InCl3 as a Cocatalyst and a Cl2Pd(DPEphos)-P(2-Furyl)3 Catalyst System for One-Pot Hydrometalation-Cross-Coupling and Carbometalation-Cross-Coupling Tandem Processes [O] . -1

机译：使用CLOP3作为一种助催化剂和CL2PD（DPEPHOS）-P（2-呋喃）3催化剂系统，用于一锅含氟量 - 交叉耦合和碳滤成交叉耦合串联工艺
8. Oxidation of Carbohydrates and Derivatives Using Carbon Supported Nobel Metal Catalysts [R] . Vinke, P. 1991

机译：碳载体诺贝尔金属催化剂氧化碳水化合物和衍生物

One-pot construction of carbohydrate scaffolds mediated by metal catalysts

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