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Waste spunlaced facial puff derived monolithic flexible carbon framework (WCF): an ultralow-cost, recyclable and eco-friendly sorbent for oils and organic solvents

机译:浪费循环面部泡芙衍生的单片柔性碳框架(WCF):用于油和有机溶剂的超级成本,可回收和环保的吸附剂

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摘要

Due to the spunlaced effect, waste spunlaced facial puff has a high degree of fiber entanglement and an abundant three-dimensional (3D) network porous structure, which make it form a 3D carbon framework material more easily after carbonization. For the first time, the monolithic 3D carbon framework is synthesized from waste spunlaced facial puff (WCF) and used as the adsorbent for contaminants in water. The adsorption capacity of WCF for oils and organic reagents can be 34-137 times its own weight. Over five adsorption-harvesting cycles, the adsorption capacity of WCF to organic pollutants can recover up to 95% of its initial capacity. Moreover, WCF exhibits stable permeation flux and high separation efficiency in a water-heavy oil system, which is about 7714 L m(-2) h(-1) and higher than 99%, respectively. With a combination of waste spunlaced facial puff with monolithic 3D porous structure as a raw material, facile and green preparation process, low density, excellent hydrophobicity and lipophilicity, WCF as an adsorbent has great superiority in removal of organic pollutant solvents and environmental protection as well as other applications, such as energy storage materials, catalyst carriers, electric information, etc. Furthermore, this work would provide a new strategy for recovery use of waste spunlaced cotton materials.
机译:由于循环效果,浪费循环面部粉末具有高度的纤维缠结和丰富的三维(3D)网络多孔结构,使其在碳化之后更容易形成3D碳框架材料。首次首次,单片3D碳框架由废物循环的面部粉扑(WCF)合成,并用作水中污染物的吸附剂。 WCF用于油和有机试剂的吸附能力可以是其自身重量的34-137倍。在五个吸附收获循环中,WCF与有机污染物的吸附能力可恢复最高可达其初始容量的95%。此外,WCF在水重油系统中表现出稳定的渗透通量和高分分离效率,其分别为约7714μm(-2)H(-1),分别高于99%。随着废物循环面粉的组合,用整体式3D多孔结构作为原料,容易和绿色制备过程,低密度,优异的疏水性和亲脂性,WCF作为吸附剂在除去有机污染物溶剂和环保方面具有很大的优势作为其他应用,例如储能材料,催化剂载体,电力信息等。此外,这项工作将提供一种用于恢复使用废物循环棉质材料的新策略。

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    《RSC Advances》 |2019年第54期|共9页
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  • 正文语种 eng
  • 中图分类 化学;
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