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Highly bright perovskite light-emitting diodes based on quasi-2D perovskite film through synergetic solvent engineering

机译:通过协同溶剂工程,基于准2D钙钛矿薄膜的高度明亮的Perovskite发光二极管

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摘要

Recently, quasi-two dimensional (2D) perovskites have attracted great interest as they can be facilely fabricated and yield high photoluminescence quantum yield. However, the luminance and the efficiency of perovskite light-emitting diodes (PeLEDs) based on quasi-2D perovskites are limited by the carrier transport and the crystallization properties of the quasi-2D perovskite films. Herein, a synergetic solvent engineering approach is proposed to improve the crystallinity and the carrier transport by optimizing the film morphology of the quasi-2D perovskite films. Consequently, the maximum luminance of green PeLEDs based on quasi-2D PEA(2) (MAPbBr(3))(2)PbBr4 perovskite is dramatically enhanced from 4000 cd m (2) to 18 000 cd m (2) and the current efficiency increases from 3.40 cd A (1) to 8.74 cd A (1). This work provides a promising way to control the morphology and the crystallinity properties of quasi-2D perovskite films for high-performance optoelectronic devices.
机译:最近,准二维(2D)Perovskites引起了极大的兴趣,因为它们可以易于制造并产生高光致发光量子产量。 然而,基于准2D钙钛矿的钙钛矿发光二极管(PELEDS)的亮度和效率受载体传输的限制和准2D钙钛矿薄膜的结晶性能。 这里,提出了一种通过优化Quasi-2d Perovskite薄膜的薄膜形态来改善结晶度和载体传输来改善结晶度和载流子。 因此,基于准2D豌豆(2)(MAPBBR(3))(2)PBBR4 Perovskite的绿色封面的最大亮度从4000cd m(2)到18 000cd m(2)和电流效率显着增强 从3.40cd a(1)到8.74cd a(1)增加。 该工作提供了一种有希望的方法来控制用于高性能光电器件的准2D钙钛矿薄膜的形态和结晶性能。

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  • 来源
    《RSC Advances》 |2019年第15期|共6页
  • 作者单位

    Beijing Jiaotong Univ Key Lab Luminescence &

    Opt Informat Minist Educ Beijing 100044 Peoples R China;

    Beijing Jiaotong Univ Key Lab Luminescence &

    Opt Informat Minist Educ Beijing 100044 Peoples R China;

    Beijing Jiaotong Univ Key Lab Luminescence &

    Opt Informat Minist Educ Beijing 100044 Peoples R China;

    Beijing Jiaotong Univ Key Lab Luminescence &

    Opt Informat Minist Educ Beijing 100044 Peoples R China;

    Beijing Jiaotong Univ Key Lab Luminescence &

    Opt Informat Minist Educ Beijing 100044 Peoples R China;

    Beijing Jiaotong Univ Key Lab Luminescence &

    Opt Informat Minist Educ Beijing 100044 Peoples R China;

    Beijing Jiaotong Univ Key Lab Luminescence &

    Opt Informat Minist Educ Beijing 100044 Peoples R China;

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  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类 化学;
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