Engineering third-order optical nonlinearities in hybrid chalcogenide-on-silicon platform

Serna Samuel; Lin Hogtao; Alonso-Ramos Carlos; Lafforgue Christian; Le Roux Xavier; Richardson Kathleen A.; Cassan Eric; Dubreuil Nicolas; Hu Juejun; Vivien Laurent

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Engineering third-order optical nonlinearities in hybrid chalcogenide-on-silicon platform

机译：杂交硫胺化物 - 硅平台中的工程三阶光学非线性

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We demonstrated a class of highly nonlinear hybrid waveguide structures based on infiltration of As2S3 chalcogenide glass into silicon slot waveguides. The nonlinear properties of the hybrid waveguides were precisely quantified via a bidirectional top-hat D-scan method, enabling a direct comparison between properties measured using different device geometries. We experimentally demonstrate hybrid As2S3-Si slot waveguides with a two-photon absorption (TPA) figure of merit exceeding 2 at near infrared wavelengths. These waveguides largely satisfy the critical criterion for efficient nonlinear integrated photonics (FOMTPAwg > 1), allowing phase shifts greater than pi with minimal overall losses. These results pave the way for efficient and robust ultrafast all-optical devices and circuits in large-scale silicon photonics technology. (C) 2019 Optical Society of America

机译：我们证明了基于AS2S3硫族化物玻璃的渗透到硅槽波导中的一类高度非线性杂交波导结构。通过双向顶帽D扫描方法精确地定量了混合波导的非线性性质，从而能够在使用不同器件几何形状测量的特性之间的直接比较。我们通过在近红外波长下，通过实验展示杂交AS2S3-SI槽波导具有超过2的双光子吸收（TPA）的优点。这些波导在很大程度上满足了高效非线性集成光子（FOMTPAWG> 1）的关键标准，允许相移大于PI，总体损耗最小。这些结果为大规模硅光子技术中的高效和鲁棒超速全光电装置和电路铺平了道路。（c）2019年光学学会

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《Optics Letters》 |2019年第20期|共4页
作者
Serna Samuel; Lin Hogtao; Alonso-Ramos Carlos; Lafforgue Christian; Le Roux Xavier; Richardson Kathleen A.; Cassan Eric; Dubreuil Nicolas; Hu Juejun; Vivien Laurent;
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Univ Paris Saclay Univ Paris Sud CNRS C2N F-91120 Palaiseau France;

MIT Dept Mat Sci &

Engn Cambridge MA 02139 USA;

Univ Paris Saclay Univ Paris Sud CNRS C2N F-91120 Palaiseau France;

Univ Paris Saclay Univ Paris Sud CNRS C2N F-91120 Palaiseau France;

Univ Paris Saclay Univ Paris Sud CNRS C2N F-91120 Palaiseau France;

Univ Cent Florida CREOL Coll Opt &

Photon Orlando FL 32816 USA;

Univ Paris Saclay Univ Paris Sud CNRS C2N F-91120 Palaiseau France;

Univ Paris Saclay CNRS Inst Opt Grad Sch Lab Charles Fabry 2 Ave Augustin Fresnel F-91127 Palaiseau France;

MIT Dept Mat Sci &

Engn Cambridge MA 02139 USA;

Univ Paris Saclay Univ Paris Sud CNRS C2N F-91120 Palaiseau France;

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正文语种 eng
中图分类计量学;光学;
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1. Engineering third-order optical nonlinearities in hybrid chalcogenide-on-silicon platform [J] . Serna Samuel, Lin Hogtao, Alonso-Ramos Carlos, Optics Letters . 2019,第20期

机译：杂交硫胺化物 - 硅平台中的工程三阶光学非线性
2. From Simplicity to Complexity in Grafting Dawson-Type Polyoxometalates on Porphyrin, Leading to the Formation of New Organic-Inorganic Hybrids for the Investigation of Third-Order Optical Nonlinearities [J] . Iqbal Arshad, Asif Hafiz Muhammad, Zhou Yunshan, Inorganic Chemistry: A Research Journal that Includes Bioinorganic, Catalytic, Organometallic, Solid-State, and Synthetic Chemistry and Reaction Dynamics . 2019,第13期

机译：从简单起见，在卟啉嫁接Dawson型多氧化物酸盐中的复杂性，导致形成新的有机无机杂种用于调查三阶光学非线性
3. Covalent Synthesis of Two Hybrids Composed of Dawson-Type Polyoxometalate and Porphyrin with Remarkable Third-Order Optical Nonlinearities Reflecting the Effect of Polyoxometalates [J] . Asif Hafiz Muhammad, Zhou Yunshan, Zhang Lijuan, Inorganic Chemistry: A Research Journal that Includes Bioinorganic, Catalytic, Organometallic, Solid-State, and Synthetic Chemistry and Reaction Dynamics . 2017,第16期

机译：两种杂交种与Dawson型聚氧酸盐和卟啉组成的共价合成，具有反映多氧化血清酸盐效应的显着三阶光学非线性
4. Third-Order Nonlinear Optical Studies of Ti and Hybrid Ti-Au Nanoparticles Generated by Laser Ablation in Liquids [C] . Moram Sree Satya Bharati, Byram Chandu, Sri Bhavya Muvva, International Conference on Optics and Electro-Optics . 2021

机译：液体激光烧蚀产生的Ti和杂种Ti-Au纳米粒子的三阶非线性光学研究
5. Third-Order Optical Nonlinearity of Tungsten and Molybdenum Disulfide Atomic Layers [D] . ?Neupane, Tikaram 2020

机译：钨和二硫化钼原子层的三阶光学非线性
6. Reversible Control of Third-Order Optical Nonlinearity of DNA Decorated Carbon Nanotube Hybrids [O] . Liangmin Zhang, Jacquelyn Thomas, Jianfeng Xu, -1

机译：DNa装饰碳纳米管杂交的三阶非线性光学性能的正反转控制
7. Reversible Control of Third-Order Optical Nonlinearity of DNA Decorated Carbon Nanotube Hybrids [O] . Liangmin Zhang, Jacquelyn Thomas, Jianfeng Xu, 2010

机译：DNA装饰碳纳米管杂交种的三阶光学非线性的可逆控制
8. Third-Order Optical Nonlinearities of Singlewall Carbon Nanotubes for Nonlinear Transmission Limiting Application [R] . Seo, J. , Ma, S. , Yang, Q. , 2006

机译：非线性传输限制应用中单壁碳纳米管的三阶光学非线性

Engineering third-order optical nonlinearities in hybrid chalcogenide-on-silicon platform

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