Alignment, orientation, and Coulomb explosion of difluoroiodobenzene studied with the pixel imaging mass spectrometry (PImMS) camera

Amini Kasra; Boll Rebecca; Lauer Alexandra; Burt Michael; Lee Jason W. L.; Christensen Lauge; Brausse Felix; Mullins Terence; Savelyev Evgeny; Ablikim Utuq; Berrah Nora; Bomme Cedric; Duesterer Stefan; Erk Benjamin; Hoeppner Hauke; Johnsson Per; Kierspel Thomas; Krecinic Faruk; Kuepper Jochen; Mueller Maria; Mueller Erland; Redlin Harald; Rouzee Arnaud; Schirmel Nora; Thogersen Jan; Techert Simone; Toleikis Sven; Treusch Rolf; Trippel Sebastian; Ulmer Anatoli; Wiese Joss; Vallance Claire; Rudenko Artem; Stapelfeldt Henrik; Brouard Mark; Rolles Daniel

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Alignment, orientation, and Coulomb explosion of difluoroiodobenzene studied with the pixel imaging mass spectrometry (PImMS) camera

机译：用像素成像质谱（PIMM）相机研究二氟苯苯苯的对准，取向和库仑爆炸

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Laser-induced adiabatic alignment and mixed-field orientation of 2,6-difluoroiodobenzene (C6H3F2I) molecules are probed by Coulomb explosion imaging following either near-infrared strong-field ionization or extreme-ultraviolet multi-photon inner-shell ionization using free-electron laser pulses. The resulting photoelectrons and fragment ions are captured by a double-sided velocity map imaging spectrometer and projected onto two position-sensitive detectors. The ion side of the spectrometer is equipped with a pixel imaging mass spectrometry camera, a time-stamping pixelated detector that can record the hit positions and arrival times of up to four ions per pixel per acquisition cycle. Thus, the time-of-flight trace and ion momentum distributions for all fragments can be recorded simultaneously. We show that we can obtain a high degree of one-and three-dimensional alignment and mixed-field orientation and compare the Coulomb explosion process induced at both wavelengths. Published by AIP Publishing.

机译：通过使用游离电子在近红外强 - 野外电离或极端紫外多光子内壳电离之后的库仑爆炸成像探测了激光诱导的2,6-二氟苯苯苯（C6H3F2I）分子的混合场取向激光脉冲。得到的光电子和片段离子被双面速度映射成像光谱仪捕获并投影到两个位置敏感的探测器上。光谱仪的离子侧配备有像素成像质谱相机，这是一个时冲印的像素化检测器，其可以记录每个获取循环每像素的每像素多达四个离子的命中位置和到达时间。因此，可以同时记录所有片段的飞行时间跟踪和离子动量分布。我们表明我们可以获得高度的单尺和三维对准和混合场取向，并比较在两个波长处感应的库仑爆炸过程。通过AIP发布发布。

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《The Journal of Chemical Physics》 |2017年第1期|共8页
作者
Amini Kasra; Boll Rebecca; Lauer Alexandra; Burt Michael; Lee Jason W. L.; Christensen Lauge; Brausse Felix; Mullins Terence; Savelyev Evgeny; Ablikim Utuq; Berrah Nora; Bomme Cedric; Duesterer Stefan; Erk Benjamin; Hoeppner Hauke; Johnsson Per; Kierspel Thomas; Krecinic Faruk; Kuepper Jochen; Mueller Maria; Mueller Erland; Redlin Harald; Rouzee Arnaud; Schirmel Nora; Thogersen Jan; Techert Simone; Toleikis Sven; Treusch Rolf; Trippel Sebastian; Ulmer Anatoli; Wiese Joss; Vallance Claire; Rudenko Artem; Stapelfeldt Henrik; Brouard Mark; Rolles Daniel;
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作者单位

Univ Oxford Dept Chem Chem Res Lab Oxford OX1 3TA England;

Deutsch Elekt Synchrotron DESY D-22607 Hamburg Germany;

Univ Oxford Dept Chem Chem Res Lab Oxford OX1 3TA England;

Univ Oxford Dept Chem Chem Res Lab Oxford OX1 3TA England;

Univ Oxford Dept Chem Chem Res Lab Oxford OX1 3TA England;

Aarhus Univ Dept Chem DK-8000 Aarhus C Denmark;

Max Born Inst Nichtlineare Opt &

Kurzzeitspektros D-12489 Berlin Germany;

Deutsch Elekt Synchrotron DESY Ctr Free Electron Laser Sci CFEL D-22607 Hamburg Germany;

Deutsch Elekt Synchrotron DESY D-22607 Hamburg Germany;

Kansas State Univ Dept Phys JR Macdonald Lab Cardwell Hall Manhattan KS 66506 USA;

Univ Connecticut Dept Phys Storrs CT 06269 USA;

Deutsch Elekt Synchrotron DESY D-22607 Hamburg Germany;

Deutsch Elekt Synchrotron DESY D-22607 Hamburg Germany;

Deutsch Elekt Synchrotron DESY D-22607 Hamburg Germany;

Deutsch Elekt Synchrotron DESY D-22607 Hamburg Germany;

Lund Univ Dept Phys S-22100 Lund Sweden;

Deutsch Elekt Synchrotron DESY Ctr Free Electron Laser Sci CFEL D-22607 Hamburg Germany;

Max Born Inst Nichtlineare Opt &

Kurzzeitspektros D-12489 Berlin Germany;

Deutsch Elekt Synchrotron DESY Ctr Free Electron Laser Sci CFEL D-22607 Hamburg Germany;

Tech Univ Berlin Inst Opt &

Atomare Phys D-10623 Berlin Germany;

Deutsch Elekt Synchrotron DESY D-22607 Hamburg Germany;

Deutsch Elekt Synchrotron DESY D-22607 Hamburg Germany;

Max Born Inst Nichtlineare Opt &

Kurzzeitspektros D-12489 Berlin Germany;

Deutsch Elekt Synchrotron DESY D-22607 Hamburg Germany;

Aarhus Univ Dept Chem DK-8000 Aarhus C Denmark;

Deutsch Elekt Synchrotron DESY D-22607 Hamburg Germany;

Deutsch Elekt Synchrotron DESY D-22607 Hamburg Germany;

Deutsch Elekt Synchrotron DESY D-22607 Hamburg Germany;

Deutsch Elekt Synchrotron DESY Ctr Free Electron Laser Sci CFEL D-22607 Hamburg Germany;

Tech Univ Berlin Inst Opt &

Atomare Phys D-10623 Berlin Germany;

Deutsch Elekt Synchrotron DESY Ctr Free Electron Laser Sci CFEL D-22607 Hamburg Germany;

Univ Oxford Dept Chem Chem Res Lab Oxford OX1 3TA England;

Kansas State Univ Dept Phys JR Macdonald Lab Cardwell Hall Manhattan KS 66506 USA;

Aarhus Univ Dept Chem DK-8000 Aarhus C Denmark;

Univ Oxford Dept Chem Chem Res Lab Oxford OX1 3TA England;

Deutsch Elekt Synchrotron DESY D-22607 Hamburg Germany;

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正文语种 eng
中图分类物理化学（理论化学）、化学物理学;
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1. Alignment, orientation, and Coulomb explosion of difluoroiodobenzene studied with the pixel imaging mass spectrometry (PImMS) camera [J] . Amini Kasra, Boll Rebecca, Lauer Alexandra, The Journal of Chemical Physics . 2017,第1期

机译：用像素成像质谱（PIMM）相机研究二氟苯苯苯的对准，取向和库仑爆炸
2. Modifications to a commercially available linear mass spectrometer for mass-resolved microscopy with the pixel imaging mass spectrometry (PImMS) camera [J] . E. Halford, B. Winter, M. D. Mills, Rapid Communications in Mass Spectrometry: RCM . 2014,第15期

机译：使用像素成像质谱（PImMS）相机对用于质量分辨显微镜的市售线性质谱仪的修改
3. Multimass velocity-map imaging with the pixel imaging mass spectrometry (PImMS) sensor: An ultra-fast event-triggered camera for particle imaging [J] . Clark A.T., Crooks J.P., Sedgwick I., The journal of physical chemistry, A. Molecules, spectroscopy, kinetics, environment, & general theory . 2012,第45期

机译：使用像素成像质谱（PImMS）传感器的多质量速度图成像：用于粒子成像的超快速事件触发相机
4. The Pixel Imaging Mass Spectrometry (PImMS) Sensor A Versatile High-Speed Position-Sensitive Detector for Imaging Mass Spectrometry [C] . Jason W. L. Lee, A. T. Clark, J. P. Crooks, American Society for Mass Spectrometry Conference on Mass Spectrometry and Allied Topics . 2013

机译：像素成像质谱（PIMMS）传感器是用于成像质谱法的多功能高速位置敏感探测器
5. The interactions of cisplatin and model proteins studied by electrospray ionization mass spectrometry and tandem mass spectrometry. [D] . Zhao, Ting. 2009

机译：通过电喷雾电离质谱和串联质谱研究了顺铂与模型蛋白的相互作用。
6. Classification of Thyroid Tumors Based on Mass Spectrometry Imaging of Tissue Microarrays; a Single-Pixel Approach [O] . Agata Kurczyk, Marta Gawin, Mykola Chekan, 2020

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7. Alignment, orientation, and Coulomb explosion of difluoroiodobenzene studied with the pixel imaging mass spectrometry (PImMS) camera [O] . Amini, K, Boll, R, Lauer, A, 2017

机译：像素成像质谱（PImMS）相机研究了二氟碘苯的排列，取向和库仑爆炸
8. GEODETIC LOCATION OF CAMERA SUPPORTS AND ALIGNMENT OF THE ORIENTATION MARKERS FOR THE FLIGHT-LINE RECORDERS [R] . William F. McIntosh 1963

机译：摄像机支持的大地位置和飞行记录器的方向标记的对齐

Alignment, orientation, and Coulomb explosion of difluoroiodobenzene studied with the pixel imaging mass spectrometry (PImMS) camera

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