Collision-Energy Dependence of the Ion-Molecule Charge-Exchange Reaction Ar+ + CO -> Ar + CO+

He Miao-Miao; Hu Jie; Wu Chun-Xiao; Zhi Yaya; Tian Shan Xi

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Collision-Energy Dependence of the Ion-Molecule Charge-Exchange Reaction Ar+ + CO -> Ar + CO+

机译：离子分子电荷交换反应Ar + + Co - > Ar + Co +的碰撞 - 能量依赖性

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Ion-molecule charge-exchange reactions Ar+ + CO -> Ar + CO+ at the centerof-mass collision energies of 4.40, 6.40, and 8.39 eV are investigated using ion velocity map imaging technique. Although multiple electronically excited states of CO+ are accessed, the population of CO+ at the A(2)Pi state is predominant in the present collision-energy range. In contrast to our previous study for NO, but similar to the case of O-2, the forward-scattered CO+ yields show a broader angular distribution at the higher collision energy. Typically, the Franck-Condon-region charge transfer, energy resonant charge transfer, and intimate collision are three different mechanisms in which the intimate collision experiences an intermediate complex, and this mechanism usually plays an essential role in the thermal-energy reactions. However, the present observations indicate that this mechanism, concerning the intermediate (Ar-Co)(+), is still of utmost importance in a relatively high collision-energy range.

机译：使用离子速度映射成像技术研究了离子分子电荷反应Ar ++ Co - > Ar + Co + CO + CO + ..使用离子速度映射成像技术研究了4.40,6.40和8.39eV。尽管访问了多种电子激发态的CO +状态，但在A（2）PI状态下的CO +群是主要的碰撞能量范围。与我们以前的NO研究相比，但类似于O-2的情况，前散散的CO +产量在更高的碰撞能量下显示出更广泛的角度分布。通常，Franck-Condon区电荷转移，能量谐振电荷转移和紧密碰撞是三种不同的机制，其中紧密碰撞经历中间复合物，并且该机制通常在热能反应中起重要作用。然而，本观察结果表明，关于中间体（Ar-Co）（+）的这种机制在相对高的碰撞能量范围内仍然至关重要。

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《The journal of physical chemistry, A. Molecules, spectroscopy, kinetics, environment, & general theory》 |2020年第17期|共6页
作者
He Miao-Miao; Hu Jie; Wu Chun-Xiao; Zhi Yaya; Tian Shan Xi;
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Univ Sci &

Technol China Collaborat Innovat Ctr Chem Energy Mat iChEM Dept Chem Phys Hefei Natl Lab Phys Sci Microscale Hefei 230026 Peoples R China;

Univ Sci &

Technol China Collaborat Innovat Ctr Chem Energy Mat iChEM Dept Chem Phys Hefei Natl Lab Phys Sci Microscale Hefei 230026 Peoples R China;

Univ Sci &

Technol China Collaborat Innovat Ctr Chem Energy Mat iChEM Dept Chem Phys Hefei Natl Lab Phys Sci Microscale Hefei 230026 Peoples R China;

Univ Sci &

Technol China Collaborat Innovat Ctr Chem Energy Mat iChEM Dept Chem Phys Hefei Natl Lab Phys Sci Microscale Hefei 230026 Peoples R China;

Univ Sci &

Technol China Collaborat Innovat Ctr Chem Energy Mat iChEM Dept Chem Phys Hefei Natl Lab Phys Sci Microscale Hefei 230026 Peoples R China;

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正文语种 eng
中图分类物理化学（理论化学）、化学物理学;
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1. Collision-Energy Dependence of the Ion-Molecule Charge-Exchange Reaction Ar+ + CO -> Ar + CO+ [J] . He Miao-Miao, Hu Jie, Wu Chun-Xiao, The journal of physical chemistry, A. Molecules, spectroscopy, kinetics, environment, & general theory . 2020,第17期

机译：离子分子电荷交换反应Ar + + Co - > Ar + Co +的碰撞 - 能量依赖性
2. Ion momentum imaging study of the ion-molecule reaction Ar+ + O-2 -> Ar + O-2(+) [J] . Wu Chun-Xiao, Hu Jie, He Miao-Miao, Physical chemistry chemical physics: PCCP . 2020,第8期

机译：离子分子反应Ar + + O-2 - > Ar + O-2（+）的离子动量成像研究
3. A high-pressure mass spectrometric study of ion-molecule reactions of Ar+ with C3H6 [J] . Bederski K. Vacuum: Technology Applications & Ion Physics: The International Journal & Abstracting Service for Vacuum Science & Technology . 2003,第2a3期

机译：Ar +与C3H6的离子分子反应的高压质谱研究
4. The Pairing Correlation Study in the ~(40)Ar+~(208)Pb Reaction [C] . T. Mijatovi?, S. Szilner, L. Corradi, International Conference on Nuclear Structure and Dynamics . 2015

机译：〜（40）AR +〜（208）PB反应的配对相关研究
5. Measured temperature dependencies of ternary ion-molecule association reactions yielding nitrogen ion-molecule(3), nitrogen ion-molecule(4) and carbonyl ion-molecule [D] . Guthrie, John Allan, Jr. 1989

机译：三价离子-分子缔合反应产生氮离子-分子（3），氮离子-分子（4）和羰基离子-分子的温度依赖性
6. GABARAPL1 Promotes AR+ Prostate Cancer Growth by Increasing FL-AR/AR-V Transcription Activity and Nuclear Translocation [O] . Bing Su, Lijuan Zhang, Shenglin Liu, 2019

机译：通过增加FL-AR / AR-V转录活动和核易位来促进AR +前列腺癌生长
7. I. State-selected study of ion-molecule reactions using tandem molecular beam photoionization mass spectrometry; II. Absolute spin-orbit-state excitation cross sections for the reactions Ar+(2P3/2 ) + Ar(1S0) and Ar+(2P3/2) + N2(X~, v=0) [O] . Shao, Jian-dong 1986

机译：一，使用串联分子束光电离质谱技术对离子-分子反应进行的国家选择研究；二。反应Ar +（2P3 / 2）+ Ar（1S0）和Ar +（2P3 / 2）+ N2（X〜，v = 0）的绝对自旋轨道激发截面
8. Temperature Dependence of the Ion-Molecule Reactions N+ + CO, C+ + NO, and C+, CO+, CO2+ + O2 from 90-450 K. [R] . Miller, T. M., Wetterskog, R. E., Paulson, J. F. 1984

机译：离子 - 分子反应的温度依赖性N + + CO，C + + NO和C +，CO +，CO2 + + O2从90-450 K.

Collision-Energy Dependence of the Ion-Molecule Charge-Exchange Reaction Ar+ + CO -> Ar + CO+

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