Near- and Mid-IR Gas-Phase Absorption Spectra of H-2@C-60(+)-He

Strelnikov Dmitry V; Jasik Juraj; Gerlich Dieter; Murata Michihisa; Murata Yasujiro; Komatsu Koichi; Roithova Jana

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Near- and Mid-IR Gas-Phase Absorption Spectra of H-2@C-60(+)-He

机译：H-2 @ C-60（+）的近和中红外气相吸收光谱 - 他

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Near- and mid-IR absorption spectra of endohedral H-2@C-60(+) have been measured using He-tagging. The samples have been prepared using a "molecular surgery" synthetic approach and were ionized and spectroscopically characterized in the gas phase. In contrast to neutral C-60 and H-2@C-60, the corresponding He-tagged cationic species show distinct spectral differences. Shifts and line splittings in the near- and mid-IR regions indicate the influence of the caged hydrogen molecule on both the electronic ground and excited states. Possible relevance to astronomy is discussed.

机译：使用HE标记测量EndoheDral H-2 @ C-60（+）的近和中红外吸收光谱。已经使用“分子手术”合成方法制备样品，并在气相中电离和光谱表征。与中性C-60和H-2 @ C-60相反，相应的He标记的阳离子物种显示出不同的光谱差异。近乎和中红外区域的换档和排插表示表明笼中的氢分子对电子地面和激发态的影响。讨论了与天文学的相关性。

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《The journal of physical chemistry, A. Molecules, spectroscopy, kinetics, environment, & general theory》 |2018年第41期|共5页
作者
Strelnikov Dmitry V; Jasik Juraj; Gerlich Dieter; Murata Michihisa; Murata Yasujiro; Komatsu Koichi; Roithova Jana;
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KIT Div Phys Chem Microscop Syst Karlsruhe Germany;

Charles Univ Prague Dept Organ Chem Fac Sci Prague 12843 2 Czech Republic;

Univ Technol Dept Phys D-09107 Chemnitz Germany;

Kyoto Univ Inst Chem Res Kyoto 6110011 Japan;

Kyoto Univ Inst Chem Res Kyoto 6110011 Japan;

Kyoto Univ Inst Chem Res Kyoto 6110011 Japan;

Charles Univ Prague Dept Organ Chem Fac Sci Prague 12843 2 Czech Republic;

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正文语种 eng
中图分类物理化学（理论化学）、化学物理学;
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1. Near- and Mid-IR Gas-Phase Absorption Spectra of H-2@C-60(+)-He [J] . Strelnikov Dmitry V, Jasik Juraj, Gerlich Dieter, The journal of physical chemistry, A. Molecules, spectroscopy, kinetics, environment, & general theory . 2018,第41期

机译：H-2 @ C-60（+）的近和中红外气相吸收光谱 - 他
2. High-resolution and high-sensitivity laser spectroscopy of atoms and molecules in the near- and mid-IR spectral regions [J] . Sasso A., Pesce G., Rusciano G. Physica Scripta: An International Journal for Experimental and Theoretical Physics . 2003,第0期

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3. The mid-IR absorption spectrum of gas-phase clusters of the nucleobases guanine and cytosine [J] . Joost M.Bakker, Isabelle Compagnon, Gerard Meijer, Physical chemistry chemical physics: PCCP . 2004,第10期

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Near- and Mid-IR Gas-Phase Absorption Spectra of H-2@C-60(+)-He

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