Ruthenium( II)- polypyridyl doped zirconium( IV) metal- organic frameworks for solid- state electrochemiluminescence

Cai Meng; Loague Quentin R.; Zhu Jie; Lin Shaoyang; Usov Pavel M.; Morris Amanda J.

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Ruthenium( II)- polypyridyl doped zirconium( IV) metal- organic frameworks for solid- state electrochemiluminescence

机译：钌（II） - 掺杂锆（IV）金属有机框架的固态电化学发光

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Solid-state electrochemiluminescence (ECL) has drawn increasing attention due to its advantages over solution-phase ECL, such as reducing the consumption of expensive reagents and enhancing the ECL signal. Herein we report a ruthenium(ii)-polypyridyl doped zirconium(iv) metal-organic framework (MOF) film, UiO-67-Ru@FTO, for solid-state electrochemiluminescence. With tripropylamine (TPA) as a coreactant, UiO-67-Ru@FTO exhibited high ECL intensity and good stability. A linear relationship was found between the ECL intensity and TPA concentration in a wide range of 0.04-20 mM. Additionally, UiO-67-Ru@FTO was successfully used for dopamine detection, implying its great potential in real-life applications.

机译：固态电化学发光（ECL）由于其优于溶液相ECL而导致的升高，例如降低昂贵试剂的消耗并增强ECL信号。在此，我们报道了一种钌（II）-polypyridyl掺杂的锆（IV）金属 - 有机骨架（MOF）膜，UIO-67-RU @ FTO，用于固态电化学发光。用三丙基胺（TPA）作为固件，UIO-67-RU @ FTO表现出高ECL强度和良好的稳定性。在0.04-20mm的宽范围内的ECL强度和TPA浓度之间发现了线性关系。此外，UIO-67-Ru @ FTO已成功用于多巴胺检测，暗示其现实生活应用中的巨大潜力。

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《Dalton transactions: An international journal of inorganic chemistry》 |2018年第46期|共6页
作者
Cai Meng; Loague Quentin R.; Zhu Jie; Lin Shaoyang; Usov Pavel M.; Morris Amanda J.;
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作者单位

Virginia Polytech Inst &

State Univ Dept Chem 800 W Campus Dr Blacksburg VA 24061 USA;

Virginia Polytech Inst &

State Univ Dept Chem 800 W Campus Dr Blacksburg VA 24061 USA;

Virginia Polytech Inst &

State Univ Dept Chem 800 W Campus Dr Blacksburg VA 24061 USA;

Virginia Polytech Inst &

State Univ Dept Chem 800 W Campus Dr Blacksburg VA 24061 USA;

Virginia Polytech Inst &

State Univ Dept Chem 800 W Campus Dr Blacksburg VA 24061 USA;

Virginia Polytech Inst &

State Univ Dept Chem 800 W Campus Dr Blacksburg VA 24061 USA;

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正文语种 eng
中图分类化学;无机化学;
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1. Ruthenium( II)- polypyridyl doped zirconium( IV) metal- organic frameworks for solid- state electrochemiluminescence [J] . Cai Meng, Loague Quentin R., Zhu Jie, Dalton transactions: An international journal of inorganic chemistry . 2018,第46期

机译：钌（II） - 掺杂锆（IV）金属有机框架的固态电化学发光
2. Ruthenium(II)-polypyridyl zirconium(IV) metal–organic frameworks as a new class of sensitized solar cells [J] . W. A. Maza, A. J. Haring, S. R. Ahrenholtz, Chemical science . 2016,第1期

机译：钌（II）-聚吡啶基锆（IV）金属-有机框架作为新型敏化太阳能电池
3. Ruthenium(ii)-polypyridyl zirconium(iv) metal–organic frameworks as a new class of sensitized solar cells [J] . W. A. Maza, A. J. Haring, S. R. Ahrenholtz, Chemical science . 2015,第1期

机译：钌（II）-polypyridyl锆（IV）金属有机框架作为新的敏化太阳能电池
4. The Effect of electronic structure on molecular first hyperpolarizabilities of highly conjugated (polypyridyl)metal-(porphinato)zinc(II) chromophores [C] . Ivan R. Miloradovic, Yuxia Zhao, Kurt Wostyn, Conference on linear and nonlinear optics of organic materials . 2003

机译：电子结构对高缀合（聚吡啶）金属 - （卟啉）金属锌（II）发色团的分子第一种超极化的影响
5. Ruthenium(II) and Osmium(II) Polypyridyl Complexes as Luminescence Sensors and PDT Agents. [D] . Sun, Yujie. 2010

机译：钌（II）和O（II）聚吡啶基配合物作为发光传感器和PDT试剂。
6. Ruthenium(ii)-polypyridyl zirconium(iv) metal–organic frameworks as a new class of sensitized solar cells [O] . W. A. Maza, A. J. Haring, S. R. Ahrenholtz, 2016

机译：钌（ii）-聚吡啶基锆（iv）金属-有机框架作为新型敏化太阳能电池
7. Ruthenium(ii)-polypyridyl zirconium(iv) metal–organic frameworks as a new class of sensitized solar cells [O] . W. A. Maza, A. J. Haring, S. R. Ahrenholtz, 2016

机译：钌（II）-polypyridyl锆（IV）金属有机框架作为新的敏化太阳能电池
8. Inductively Coupled Plasma Mass Spectrometry: Sample Analysis of Zirconium and Ruthenium in Metal Organic Frameworks. [R] . Dubbs, A. B., Hoffland, L. 2018

机译：电感耦合等离子体质谱：金属有机框架中锆和钌的样品分析。

Ruthenium( II)- polypyridyl doped zirconium( IV) metal- organic frameworks for solid- state electrochemiluminescence

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