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首页> 外文期刊>Dalton transactions: An international journal of inorganic chemistry >Noncentrosymmetric (NCS) solid solutions: elucidating the structure-nonlinear optical (NLO) property relationship and beyond
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Noncentrosymmetric (NCS) solid solutions: elucidating the structure-nonlinear optical (NLO) property relationship and beyond

机译：非团体二元（NCS）固溶解决方案：阐明结构 - 非线性光学（NLO）性能关系及更远

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摘要

A systematic approach toward the discovering of novel functional noncentrosymmetric (NCS) materials revealing technologically useful applications is an ongoing challenge. This Frontiers article investigates a series of NCS solid solutions with respect to their crystal structure and second-harmonic generation (SHG) response. The solid solutions include NCS polar aluminoborates, Al5-xGaxBO9 (0.0 <= x <= 0.5), rare earth element-doped bismuth tellurites, Bi2-xRExTeO5 (RE = Y, Ce, and Eu; 0.0 <= x <= 0.2), layered perovskites, Bi4-xLaxTi3O12 (0.0 <= x <= 0.75: Aurivillius phases) and CsBi1-xEuxNb2O7 (0.0 <= x <= 0.2: Dion-Jacobson phases), calcium bismuth oxides, Ca(4)Bi(6-x)Ln(x)O(13) (Ln = La and Eu; x = 0, 0.06 and 0.12), and sodium lanthanide iodates, NaLa(1-x)Ln(x)(IO3)(4) (Ln = Sm and Eu; 0 <= x <= 1). The origin of SHG for all the NCS solid solutions is discussed and the detailed structure-nonlinear optical (NLO) property relationships are elucidated. In addition, photoluminescence (PL) properties and subsequent energy transfer mechanisms for NCS solid solutions are provided.
机译：发现发现新型功能性非团体二核（NCS）材料的系统方法揭示了技术有用的应用是持续的挑战。该领域文章研究了一系列基于其晶体结构和二次谐波产生（SHG）响应的NCS固体解决方案。固溶体包括NCS极性铝硼酸盐，Al5-XgaxbO9（0.0 <= x <= 0.5），稀土元素掺杂的碲酸盐，Bi2-XRexteO5（Re = Y，Ce和Eu; 0.0 <= x <= 0.2） ，层状蠕动，Bi4-XlaxTi3O12（0.0 <= x <= 0.75：Aurivillius阶段）和CsBi1-Xeuxnb2O7（0.0 <= x <= 0.2：Dion-jacobson阶段），氧化钙氧化物，Ca（4）Bi（6- x）Ln（x）O（13）（Ln = La和Eu; x = 0,0.06和0.12），含镧碘酸钠，NALA（1-X）LN（X）（IO3）（4）（LN = SM和EU; 0 <= x <= 1）。讨论了所有NCS固溶解决的SHG的起源，并阐明了详细的结构 - 非线性光学（NLO）性质关系。另外，提供了光致发光（PL）性能和随后的NCS固体溶液的能量转移机制。

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