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Temperature, p HH , and reduction triple‐stimuli‐responsive inner‐layer crosslinked micelles as nanocarriers for controlled release

机译：温度，p h h，还原三刺激响应的内层交联胶束作为控制释放的纳米载体

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ABSTRACT > Temperature, pH, and reduction triple‐stimuli‐responsive inner‐layer crosslinked micelles as nanocarriers for drug delivery and release are designed. The well‐defined tetrablock copolymer poly(polyethylene glycol methacrylate)–poly[2‐(dimethylamino) ethyl methacrylate]–poly( N ‐isopropylacrylamide)–poly(methylacrylic acid) (PPEGMA‐PDMAEMA‐PNIPAM‐PMAA) is synthesized via atom transfer radical polymerization, click chemistry, and esterolysis reaction. The tetrablock copolymer self‐assembles into noncrosslinked micelles in acidic aqueous solution. The core‐crosslinked micelles, shell‐crosslinked micelles, and shell–core dilayer‐crosslinked micelles are prepared via quaternization reaction or carbodiimide chemistry reaction. The crosslinked micelles are used as drug carriers to load doxorubicin (DOX), and the drug encapsulation efficiency with 20% feed ratio reached 59.2%, 73.1%, and 86.1%, respectively. The cumulative release rate of DOX is accelerated by single or combined stimulations. The MTT (3‐(4,5‐Dimethylthiazol‐2‐yl)‐2,5‐diphenyltetrazolium bromide) assay verifies that the inner‐layer crosslinked micelles show excellent cytocompatibility, and DOX‐loaded micelles exhibit significantly higher inhibition for HepG2 cell proliferation. ? 2018 Wiley Periodicals, Inc. J. Appl. Polym. Sci. 2018 , 135 , 46714. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract XMLNS =“http://www.wiley.com/namespaces/wiley”type =“main”> <title type =“main”>抽象</ title> >温度，pH和减少三刺激 - 设计为用于药物递送和释放的纳米载体作为纳米载体的偏移内层交联胶束。明确定义的四聚锁共聚物聚（聚乙二醇甲基丙烯酸酯） - 聚[2-（二甲基氨基）甲基丙烯酸乙酯] - 聚（ N = -I> - 丙烯酰胺） - 聚（甲基丙烯酸）（PPEGMA-PDMAEMA-PNIPAM-通过原子转移自由基聚合合成PMAA），单击化学，酯解反应。四聚锁共聚物在酸性水溶液中自组装成非粘土的胶束。通过季铵化反应或碳二亚胺化学反应制备核交联的胶束，壳交联胶束和壳核倍二蛋白交联胶束。交联的胶束用作负荷的药物载体（DOX），分别具有20％的进料比的药物包封效率分别达到59.2％，73.1％和86.1％。 DOX的累积释放率通过单一或组合刺激加速。 MTT（3-（4,5-二甲基噻唑-2-基）-2,5-二苯基四唑鎓溴化物）测定验证了内层交联胶束显示出优异的细胞相容性，并且DOX加载的胶束表现出对HepG2细胞增殖的显着抑制。还是2018 Wiley期刊，Inc.J.Phill。聚合物。 SCI。 2018 </ b>， 135 </ i>，46714. </ p> </ abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-33581/'>《Journal of Applied Polymer Science》</a> <b style="margin: 0 2px;">|</b><span>2018年第40期</span><b style="margin: 0 2px;">|</b><span>共10页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Kehu&option=202" target="_blank" rel="nofollow">Zhang Kehu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Jiangtao&option=202" target="_blank" rel="nofollow">Liu Jiangtao;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ma Xiao&option=202" target="_blank" rel="nofollow">Ma Xiao;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lei Lei&option=202" target="_blank" rel="nofollow">Lei Lei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Yan&option=202" target="_blank" rel="nofollow">Li Yan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Hong&option=202" target="_blank" rel="nofollow">Yang Hong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lei Zhongli&option=202" target="_blank" rel="nofollow">Lei Zhongli;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Key Laboratory of Applied Surface and Colloid Chemistry School of Chemistry &</p> <p>Chemical EngineeringShaanxi Normal UniversityXi'an 710062 China;</p> <p>Key Laboratory of Applied Surface and Colloid Chemistry School of Chemistry &</p> <p>Chemical EngineeringShaanxi Normal UniversityXi'an 710062 China;</p> <p>Key Laboratory of Applied Surface and Colloid Chemistry School of Chemistry &</p> <p>Chemical EngineeringShaanxi Normal UniversityXi'an 710062 China;</p> <p>Key Laboratory of Applied Surface and Colloid Chemistry School of Chemistry &</p> <p>Chemical EngineeringShaanxi Normal UniversityXi'an 710062 China;</p> <p>Key Laboratory of Applied Surface and Colloid Chemistry School of Chemistry &</p> <p>Chemical EngineeringShaanxi Normal UniversityXi'an 710062 China;</p> <p>Basic Experimental Teaching CenterShaanxi Normal UniversityXi'an 710062 China;</p> <p>Key Laboratory of Applied Surface and Colloid Chemistry School of Chemistry &</p> <p>Chemical EngineeringShaanxi Normal UniversityXi'an 710062 China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1821.html" title="高分子化合物工业（高聚物工业）">高分子化合物工业（高聚物工业）;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=biomaterials&option=203" rel="nofollow">biomaterials;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=crosslinking&option=203" rel="nofollow">crosslinking;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=drug delivery systems&option=203" rel="nofollow">drug delivery systems;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=self‐assembly&option=203" rel="nofollow">self‐assembly;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=stimuli‐sensitive polymers&option=203" rel="nofollow">stimuli‐sensitive polymers;</a> </p> <div class="translation"> 机译：生物材料;交联;药物递送系统;自组装;刺激敏感聚合物; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704020588853.html">Temperature, p <fc xmlns="http://www.wiley.com/namespaces/wiley">H</fc>H , and reduction triple‐stimuli‐responsive inner‐layer crosslinked micelles as nanocarriers for controlled release</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Kehu&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Zhang Kehu,</a> <a 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