On the origin of functionalization in one-pot radiation synthesis of nanogels from aqueous polymer solutions

Dispenza C.; Sabatino M. A.; Grimaldi N.; Mangione M. R.; Walo M.; Murugan E.; Jonsson M.

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On the origin of functionalization in one-pot radiation synthesis of nanogels from aqueous polymer solutions

机译：从聚合物溶液中纳米凝胶一锅辐射合成官能化起源

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Radiation-engineered poly(N-vinyl pyrrolidone) nanogels are very interesting biocompatible nanocarriers for i.v. administration of therapeutics and contrast agents for bioimaging. The manufacturing process is fast and effective, it grants excellent control of particle size and simultaneous sterilization of the formed nanogels. Interestingly, primary amino groups and carboxyl groups, useful for (bio) conjugation, are also formed in a dose-dependent fashion. In this paper, by means of both numerical simulations and experiments, the origin of nanogel size control and functionalization is investigated. This understanding offers a new dimension for the design and production of radiation-sculptured multifunctional nanocarriers from aqueous solutions of polymers.

机译：辐射工程化聚（N-乙烯基吡咯烷酮）纳米凝胶是非常有趣的生物相容性纳米载体，用于I.V。施用治疗和造影剂的生物体。制造过程快速有效，它授予粒度的优异控制和形成的纳米凝胶的同时灭菌。有趣的是，初级氨基和羧基，可用于（生物）缀合，也以剂量依赖性的方式形成。本文通过数值模拟和实验，研究了纳米凝胶尺寸控制和官能化的起源。这种理解为来自聚合物水溶液的辐射雕塑多功能纳米载体的设计和生产提供了新的尺寸。

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《RSC Advances》 |2016年第4期|共10页
作者
Dispenza C.; Sabatino M. A.; Grimaldi N.; Mangione M. R.; Walo M.; Murugan E.; Jonsson M.;
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作者单位

Univ Palermo Dipartimento Ingn Chim Gest Informat Meccan I-90128 Palermo Italy;

Univ Palermo Dipartimento Ingn Chim Gest Informat Meccan I-90128 Palermo Italy;

Univ Palermo Dipartimento Ingn Chim Gest Informat Meccan I-90128 Palermo Italy;

CNR Ist Biofis IBF UOS Palermo I-90146 Palermo Italy;

Inst Nucl Chem &

Technol Ctr Radiat Res &

Technol PL-03195 Warsaw Poland;

KTH Royal Inst Technol Sch Chem Sci &

Engn Appl Phys Chem SE-10044 Stockholm Sweden;

KTH Royal Inst Technol Sch Chem Sci &

Engn Appl Phys Chem SE-10044 Stockholm Sweden;

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正文语种 eng
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1. On the origin of functionalization in one-pot radiation synthesis of nanogels from aqueous polymer solutions [J] . Dispenza C., Sabatino M. A., Grimaldi N., RSC Advances . 2016,第4期

机译：从聚合物溶液中纳米凝胶一锅辐射合成官能化起源
2. Starch functionalized magnetite nanoparticles: A green, biocatalyst for one-pot multicomponent synthesis of imidazopyrimidine derivatives in aqueous medium under ultrasound irradiation [J] . Journal of Molecular Structure . 2020,第期

机译：淀粉官能化磁铁矿纳米粒子：在超声辐射下，用于一锅多组合合成咪唑嘧啶衍生物的绿色，生物催化剂
3. One-Pot Hydrothermal Synthesis of Polyethylenimine Functionalized Magnetic Clay for Efficient Removal of Noxious Cr(VI) from Aqueous Solutions [J] . Fayazi Maryam, Ghanbarian Maryam Silicon . 2020,第1期

机译：聚乙基亚胺官能化磁性粘土的单壶水热合成，以便于水溶液中有效去除有毒Cr（VI）
4. Stimuli-responsive nanogels by e-beam irradiation of dilute aqueous micellar solutions: Nanogels with pH controlled LCST [C] . L. A. Picos-Corrales, A. Licea-Claverie, K. F. Arndt NSTI nanotechnology conference and expo;Nanotech conference expo;NSTI-Nanotech 2012;TechConnect world annual conference expo . 2012

机译：通过电子束辐照稀胶束水溶液刺激刺激的纳米凝胶：pH控制LCST的纳米凝胶
5. Synthesis and aqueous solution studies of stimuli-responsive block copolymers synthesized by reversible addition-fragmentation chain transfer polymerization. [D] . Convertine, Anthony Joseph. 2006

机译：通过可逆加成-断裂链转移聚合反应合成的刺激反应性嵌段共聚物的合成和水溶液研究。
6. One-Pot synthesis characterization and adsorption studies of amine-functionalized magnetite nanoparticles for removal of Cr (VI) and Ni (II) ions from aqueous solution: kinetic isotherm and thermodynamic studies [O] . Abbas Norouzian Baghani, Amir Hossein Mahvi, Mitra Gholami, 2016

机译：用于从水溶液中去除Cr（VI）和Ni（II）离子的胺官能化磁铁矿纳米粒子的一锅法合成表征和吸附研究：动力学等温线和热力学研究
7. One-Pot synthesis, characterization and adsorption studies of amine-functionalized magnetite nanoparticles for removal of Cr (VI) and Ni (II) ions from aqueous solution: kinetic, isotherm and thermodynamic studies [O] . Abbas Norouzian Baghani, Amir Hossein Mahvi, Mitra Gholami, 2016

机译：用于从水溶液中去除Cr（VI）和Ni（II）离子的胺官能化磁铁矿纳米粒子的一锅法合成，表征和吸附研究：动力学，等温线和热力学研究

On the origin of functionalization in one-pot radiation synthesis of nanogels from aqueous polymer solutions

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