Synthesis of porous Al doped ZnO nanosheets with high adsorption and photodecolorizative activity and the key role of Al doping for methyl orange removal

Sun Xiaohua; Luo Weilong; Chen Linlin; Zheng Linjie; Bao Chao; Sun Panpan; Huang Niu; Sun Yihua; Fang Liang; Wang Lei

首页> 外文期刊>RSC Advances >Synthesis of porous Al doped ZnO nanosheets with high adsorption and photodecolorizative activity and the key role of Al doping for methyl orange removal

【24h】

Synthesis of porous Al doped ZnO nanosheets with high adsorption and photodecolorizative activity and the key role of Al doping for methyl orange removal

机译：具有高吸附和光致抗溶解活性的多孔Al掺杂ZnO纳米片的合成及Al掺杂对甲基橙去除的关键作用

获取原文

获取原文并翻译 | 示例

掌桥外文数据库（机构版） >>

开具论文收录证明 >>

文献代查 >>

页面导航

摘要
著录项
相似文献
相关主题

摘要

Porous Al doped ZnO (AZO) nanosheets have been prepared as an efficient multifunctional water treatment material. Their fundamental properties were characterized by various spectroscopic testing methods. The AZO nanosheets displayed very rapid adsorption rate and high adsorption capacity for methyl orange (MO) dye. The kinetics and equilibrium of adsorption process were found to follow the pseudo-second-order kinetic and Langmuir isotherm models, respectively. Furthermore, the AZO nanosheets exhibited superior photodecolorizative activity compared with the commercial P25 TiO2 nanoparticles. It was found that Al doping increased the zeta potential of AZO nanosheets and then significantly enhanced the adsorption capacity for MO dye and, at the same time, retarded the recombination of photoexcited electron-hole pairs, and prolonged the lifetime of the photo-generated carriers, and then improved the semiconductor photocatalytic activity. In addition, the visible-light-driven dye photosensitized degradation was also an important reason for enhanced photodecolorizative activity. Therefore, AZO nanosheets are a potential multifunctional water treatment material combining highly efficient adsorption and photocatalytic degradation.

机译：多孔Al掺杂ZnO（AZO）纳米片已被制备为有效的多功能水处理材料。它们的基本特性是通过各种光谱检测方法的特征。 AZO纳米片显示出非常快速的吸附速率和甲基橙（Mo）染料的高吸附容量。发现吸附过程的动力学和平衡分别遵循伪二阶动力学和Langmuir等温模型。此外，与商业P25 TiO2纳米颗粒相比，Azo纳米蛋白酶表现出优异的光致沉淀活性。结果发现，掺杂氧化氮纳米片的Zeta电位，然后显着提高了Mo染料的吸附能力，同时延迟了光屏蔽电子 - 孔对的重组，并延长了光产生的载体的寿命然后改善了半导体光催化活性。此外，可见光驱动的染料光敏性降解也是增强光耐热活性的重要原因。因此，AZO纳米片是一种相结合高效吸附和光催化降解的潜在多功能水处理材料。

著录项

来源
《RSC Advances》 |2016年第3期|共11页
作者
Sun Xiaohua; Luo Weilong; Chen Linlin; Zheng Linjie; Bao Chao; Sun Panpan; Huang Niu; Sun Yihua; Fang Liang; Wang Lei;
展开▼
作者单位

China Three Gorges Univ Coll Mech &

Power Engn Coll Mat &

Chem Engn Collaborat Innovat Ctr Energ Hubei Prov Collaborat Innovat Ctr New Energy Micr Yichang 443002 Peoples R China;

China Three Gorges Univ Coll Mech &

Power Engn Coll Mat &

Chem Engn Collaborat Innovat Ctr Energ Hubei Prov Collaborat Innovat Ctr New Energy Micr Yichang 443002 Peoples R China;

China Three Gorges Univ Coll Mech &

Power Engn Coll Mat &

Chem Engn Collaborat Innovat Ctr Energ Hubei Prov Collaborat Innovat Ctr New Energy Micr Yichang 443002 Peoples R China;

China Three Gorges Univ Coll Mech &

Power Engn Coll Mat &

Chem Engn Collaborat Innovat Ctr Energ Hubei Prov Collaborat Innovat Ctr New Energy Micr Yichang 443002 Peoples R China;

China Three Gorges Univ Coll Mech &

Power Engn Coll Mat &

Chem Engn Collaborat Innovat Ctr Energ Hubei Prov Collaborat Innovat Ctr New Energy Micr Yichang 443002 Peoples R China;

China Three Gorges Univ Coll Mech &

Power Engn Coll Mat &

Chem Engn Collaborat Innovat Ctr Energ Hubei Prov Collaborat Innovat Ctr New Energy Micr Yichang 443002 Peoples R China;

China Three Gorges Univ Coll Mech &

Power Engn Coll Mat &

Chem Engn Collaborat Innovat Ctr Energ Hubei Prov Collaborat Innovat Ctr New Energy Micr Yichang 443002 Peoples R China;

China Three Gorges Univ Coll Mech &

Power Engn Coll Mat &

Chem Engn Collaborat Innovat Ctr Energ Hubei Prov Collaborat Innovat Ctr New Energy Micr Yichang 443002 Peoples R China;

Guilin Univ Technol GuangXi Key Lab New Energy &

Bldg Energy Saving Guilin 541004 Peoples R China;

Guilin Univ Technol GuangXi Key Lab New Energy &

Bldg Energy Saving Guilin 541004 Peoples R China;

展开▼
收录信息
原文格式 PDF
正文语种 eng
中图分类化学;
关键词

相似文献

外文文献
中文文献
专利

1. Synthesis of porous Al doped ZnO nanosheets with high adsorption and photodecolorizative activity and the key role of Al doping for methyl orange removal [J] . Sun Xiaohua, Luo Weilong, Chen Linlin, RSC Advances . 2016,第3期

机译：具有高吸附和光致抗溶解活性的多孔Al掺杂ZnO纳米片的合成及Al掺杂对甲基橙去除的关键作用
2. Low-Cost Y-Doped TiO2 Nanosheets Film with Highly Reactive {001} Facets from CRT Waste and Enhanced Photocatalytic Removal of Cr(VI) and Methyl Orange [J] . Qijun Zhang, Yu Fu, Yufeng Wu ACS Sustainable Chemistry & Engineering . 2016,第3期

机译：低成本的Y掺杂TiO2纳米片薄膜，具有来自CRT废料的高反应性{001}刻面，并具有增强的光催化去除Cr（VI）和甲基橙的性能
3. Facile synthesis of ZnO and transition metal doped ZnO nanoparticles for the photocatalytic degradation of Methyl Orange [J] . Japinder Kaur, Sonal Singhal CERAMICS INTERNATIONAL . 2014,第5期

机译：方便地合成ZnO和掺杂过渡金属的ZnO纳米粒子对甲基橙的光催化降解
4. Photocatalytic Degradation of Methylene Blue and Methyl Orange with Fe-doped ZnO Nanoparticles Modified with Natural Zeolite and Montmorillonite: Comparative Study [C] . Nur Afifah, Siti Adriani, Nadia F. Djaja International Conference on Advanced Materials Science and Technology . 2015

机译：用天然沸石和蒙脱石改性Fe掺杂ZnO纳米粒子的光催化降解亚甲基橙色和蒙脱石：比较研究
5. Experimental investigations of a proposed chromophore correlation model of self healing of Disperse Orange 11 doped in Poly(methyl methacrylate) [D] . Ramini, Shiva Kumar 2012

机译：聚甲基丙烯酸甲酯中掺杂的分散橙11的自修复生色团相关模型的实验研究
6. Facile Synthesis of Mn-Doped ZnO Porous Nanosheets as Anode Materials for Lithium Ion Batteries with a Better Cycle Durability [O] . Linlin Wang, Kaibin Tang, Min Zhang, 2015

机译：Mn掺杂的ZnO多孔纳米片的方便合成作为锂离子电池负极材料具有更好的循环耐久性
7. Facile Synthesis of Mn-Doped ZnO Porous Nanosheets as Anode Materials for Lithium Ion Batteries with a Better Cycle Durability [O] . Linlin Wang, Kaibin Tang, Min Zhang, 2015

机译：Mn掺杂的ZnO多孔纳米片的方便合成作为锂离子电池负极材料，具有更好的循环耐久性

Synthesis of porous Al doped ZnO nanosheets with high adsorption and photodecolorizative activity and the key role of Al doping for methyl orange removal

摘要

著录项

相似文献

相关主题

期刊订阅