Aerobic oxidation of alcohols and alkenes over a novel lacunary phosphomolybdate anchored to zeolite H beta

Singh Sukriti; Narkhede Nilesh; Patel Anjali

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Aerobic oxidation of alcohols and alkenes over a novel lacunary phosphomolybdate anchored to zeolite H beta

机译：在锚定沸石Hβ的新型格拉族磷钼酸盐上有氧氧化醇和alkenes

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Lacunary phosphomolybdate anchored to zeolite H beta was synthesized and characterised by various physicochemical techniques. The catalytic activity was evaluated for aerobic oxidation of benzyl alcohol and styrene. The catalyst was found to be efficient, especially in terms of selectivity for the desired benzaldehyde product (for benzyl alcohol - 90%, styrene - 72%), very high turnover number (alcohols > 3500, alkenes > 18 000) as well as recyclability. The viability of the catalyst was also extended to various alkenes and alcohols.

机译：通过各种物理化学技术合成并表征锚定的硅藻土Hβ的磷钼酸盐。评价催化活性的苄醇和苯乙烯的有氧氧化。发现催化剂有效，特别是在所需苯甲醛产物的选择性方面（对于苄醇 - 90％，苯乙烯 - 72％），非常高的周转数（醇> 3500，alkEnes> 18000）以及可回收性。催化剂的可行性也延伸到各种烯烃和醇。

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来源
《RSC Advances》 |2015年第46期|共9页
作者
Singh Sukriti; Narkhede Nilesh; Patel Anjali;
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作者单位

Maharaja Sayajirao Univ Baroda Fac Sci Dept Chem Polyoxometalates &

Catalysis Lab Vadodara 390002 Gujarat India;

Maharaja Sayajirao Univ Baroda Fac Sci Dept Chem Polyoxometalates &

Catalysis Lab Vadodara 390002 Gujarat India;

Maharaja Sayajirao Univ Baroda Fac Sci Dept Chem Polyoxometalates &

Catalysis Lab Vadodara 390002 Gujarat India;

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正文语种 eng
中图分类化学;
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1. Aerobic oxidation of alcohols and alkenes over a novel lacunary phosphomolybdate anchored to zeolite H beta [J] . Singh Sukriti, Narkhede Nilesh, Patel Anjali RSC Advances . 2015,第46期

机译：在锚定沸石Hβ的新型格拉族磷钼酸盐上有氧氧化醇和alkenes
2. Mono lacunary phosphomolybdate supported on MCM-41: synthesis, characterization and solvent free aerobic oxidation of alkenes and alcohols [J] . Nilesh Narkhede, Anjali Patel, Sukriti Singh Dalton transactions: An international journal of inorganic chemistry . 2014,第6期

机译：MCM-41上负载的单钼酸钼钼酸酯：烯烃和醇的合成，表征和无溶剂好氧氧化
3. Photocatalytic anion oxidation achieves direct aerobic difunctionalization of alkenes leading to beta-thiocyanato alcohols [J] . Zhang Wei, Guo Jun-Tao, Yu Yue, Tetrahedron . 2018,第24期

机译：光催化阴离子氧化实现了导致β-硫代氰酸酯的烯烃的直接好氧双官能化
4. The Addition of Water and Alcohol to Alkenes by Alkyl-Immobilized Zeolite Catalysts in the Liquid Phase [C] . Haruo Ogawa, Takashi Hosoe, Hao Xiuhua, International conference on colloid and surface science . 2001

机译：通过液相中的烷基固定的沸石催化剂将水和醇加入烯烃中
5. Mechanistic studies of palladium-catalyzed 'Wacker type' intramolecular aerobic oxidative amination of alkenes and Development of safe and scalable continuous-flow methods for palladium-catalyzed aerobic oxidation [D] . Ye, Xuan 2010

机译：钯催化烯烃的“ Wacker型”分子内需氧氧化胺化的机理研究和开发安全，可扩展的连续流法进行钯催化的需氧氧化
6. Aerobic Alcohol Oxidation Coupled to Palladium-Catalyzed Alkene Hydroarylation with Boronic Esters [O] . Yasumasa Iwai, Keith M. Gligorich, Matthew S. Sigman -1

机译：需氧醇氧化与硼酸酯偶联钯催化的烯烃加氢芳基化
7. Palladium Nanoparticles Entrapped in Aluminum Hydroxide: Dual Catalyst for Alkene Hydrogenation and Aerobic Alcohol Oxidation. [O] . Min Serk Kwon, Namdu Kim, Cheon Min Park, 2005

机译：钯纳米包埋在氢氧化铝：双催化剂的加氢烯烃和有氧醇的氧化。

Aerobic oxidation of alcohols and alkenes over a novel lacunary phosphomolybdate anchored to zeolite H beta

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