Synthesis and color tuning of boron diiminate conjugated polymers with aggregation-induced scintillation properties

Tanaka Kazuo; Yanagida Takayuki; Hirose Amane; Yamane Honami; Yoshii Ryousuke; Chujo Yoshiki

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Synthesis and color tuning of boron diiminate conjugated polymers with aggregation-induced scintillation properties

机译：聚集诱导的闪烁性能的硼偶氮共轭聚合物的合成与色调

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We report film-type scintillators based on conjugated polymers with aggregation-induced emission (AIE) properties and the modulation of their scintillation abilities by chemical modification. Alternating copolymers containing a series of boron diiminates with various substituents and comonomers were synthesized via the palladium-catalyzed cross-coupling reaction. The synthesized polymers showed AIE properties. In addition, the corresponding emission colors to photoluminescence were also obtained with X-ray excitation. These data suggest that the AIE-active polymers should be a promising platform for developing a function-tunable plastic scintillator.

机译：我们通过具有聚集诱导的发射（AIE）性能的共轭聚合物报告膜型闪烁体，并通过化学改性调节其闪烁能力。通过钯催化的交叉偶联反应合成含有一系列具有各种取代基和共聚单体的硼二氰酸酯的交替的共聚物。合成的聚合物显示AIE性质。此外，还通过X射线激发获得相应的发光颜色对光致发光。这些数据表明，AIE活性聚合物应该是开发功能可调塑料闪烁体的有希望的平台。

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《RSC Advances》 |2015年第117期|共7页
作者
Tanaka Kazuo; Yanagida Takayuki; Hirose Amane; Yamane Honami; Yoshii Ryousuke; Chujo Yoshiki;
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Kyoto Univ Grad Sch Engn Dept Polymer Chem Nishikyo Ku Kyoto 6158510 Japan;

Nara Inst Sci &

Technol Grad Sch Mat Sci Nara 6300192 Japan;

Kyoto Univ Grad Sch Engn Dept Polymer Chem Nishikyo Ku Kyoto 6158510 Japan;

Kyoto Univ Grad Sch Engn Dept Polymer Chem Nishikyo Ku Kyoto 6158510 Japan;

Kyoto Univ Grad Sch Engn Dept Polymer Chem Nishikyo Ku Kyoto 6158510 Japan;

Kyoto Univ Grad Sch Engn Dept Polymer Chem Nishikyo Ku Kyoto 6158510 Japan;

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正文语种 eng
中图分类化学;
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1. Synthesis and color tuning of boron diiminate conjugated polymers with aggregation-induced scintillation properties [J] . Tanaka Kazuo, Yanagida Takayuki, Hirose Amane, RSC Advances . 2015,第117期

机译：聚集诱导的闪烁性能的硼偶氮共轭聚合物的合成与色调
2. Synthesis of Aggregation-Induced Emission-Active Conjugated Polymers Composed of Group 13 Diiminate Complexes with Tunable Energy Levels via Alteration of Central Element [J] . Shunichiro Ito, Amane Hirose, Madoka Yamaguchi, Polymers . 2017,第2期

机译：通过中心元素的改变合成由可调节能级的13族二胺配合物组成的聚集诱导的发射活性共轭聚合物。
3. Synthesis of binaphthyl-oligothiophene copolymers with emissions of different colors: Systematically tuning the photoluminescence of conjugated polymers [J] . Musick KY., Pu L., Hu QS. Macromolecules . 1998,第9期

机译：具有不同颜色发射光的联萘-低聚噻吩共聚物的合成：系统地调节共轭聚合物的光致发光
4. Elucidation of Relationships between Solid-State Photophysical Properties and Crystal Structures of Boron Diiminates Showing Thermochromism and Non-linear Optical Properties of Boron Diiminates [C] . HIMENO Ryoji, ITO Shunichiro, TANAKA Kazuo 日本化学会春季年会講演予稿集 . 2018

机译：释放硼二氰酸硼晶体结构与硼二嘧啶的热切割和非线性光学性能的关系
5. Boron-containing pi-conjugated polymers built with transition metal cage complexes and C3-symmetric pi-conjugation: Modular synthesis of oligomers and polymers. [D] . Zhang, Jing. 2013

机译：用过渡金属笼型络合物和C3对称pi共轭构建的含硼pi共轭聚合物：低聚物和聚合物的模块合成。
6. Synthesis of Aggregation-Induced Emission-Active Conjugated Polymers Composed of Group 13 Diiminate Complexes with Tunable Energy Levels via Alteration of Central Element [O] . Shunichiro Ito, Amane Hirose, Madoka Yamaguchi, 2017

机译：通过中心元素的改变合成由可调节能级的13族二胺配合物组成的聚集诱导的发射活性共轭聚合物。
7. Synthesis of Aggregation-Induced Emission-Active Conjugated Polymers Composed of Group 13 Diiminate Complexes with Tunable Energy Levels via Alteration of Central Element [O] . Shunichiro Ito, Amane Hirose, Madoka Yamaguchi, 2017

机译：通过中心元素的改变合成具有可调节能级的13族二亚胺配合物的聚集诱导发光 - 活性共轭聚合物

Synthesis and color tuning of boron diiminate conjugated polymers with aggregation-induced scintillation properties

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