首页> 外文期刊>RSC Advances >Ferroelectric domain structure evolution in Ba(Zr0.1Ti0.9)O-3/(Ba0.75Ca0.25)TiO3 heterostructures
【24h】

Ferroelectric domain structure evolution in Ba(Zr0.1Ti0.9)O-3/(Ba0.75Ca0.25)TiO3 heterostructures

机译:Ba(Zr0.1Ti0.9)O-3 /(Ba0.75ca0.25)TiO3异质结构的铁电域结构演进

获取原文
获取原文并翻译 | 示例
           

摘要

Highly oriented multilayerd Ba(Zr0.1Ti0.9)O-3/(Ba0.75Ca0.25)TiO3 thin films were fabricated on Nb doped (001) SrTiO3 (Nb: STO) substrates by pulsed laser deposition. Microstructural characterization by X-ray diffraction indicates that the as-deposited multilayered thin films are highly c-axis oriented. Transmission electron microscopy shows that the films present epitaxial correspondence with the substrate at the first layer and multi-oriented twin domain structures near the surface, especially with increasing periodic number (N). Piezoresponse force microscopy (PFM) studies reveal an intense polarization component in the out-of-plane direction, which increases greatly with increasing periodic number (N), whereas the in-plane shows inferior phase contrast. The optimized combination was found to be the annealed 16 layer structure (N = 8, layer thickness = 712 nm) which displays the best polarization domain structures and the saturated piezo response loop. The annealing process benefits the 180 degrees domains with the same angle in the growth direction, which brings more piezo response in the in-plane signal. Our results suggest that the increasing of piezo response is greatly associated with the interface effect and the twining structure.
机译:通过脉冲激光沉积在Nb掺杂(001)SRTIO3(Nb:STO)基板上制造高度取向的多层BA(Zr0.1Ti0.9)O-3 /(Ba0.75Ca0.25)TiO3薄膜。 X射线衍射的微观结构表征表明,沉积的多层薄膜是高度C轴的取向。透射电子显微镜表明,膜存在与第一层的基板的外延对应,以及在表面附近的多取向的双畴结构,特别是随着周期性数量(n)的增加。压电响应力显微镜(PFM)研究在平面外方向上显示强烈的偏振分量,这随着周期性数量(n)而大大增加,而在平面内显示出低位相反。发现优化的组合是退火的16层结构(n = 8,层厚度= 712nm),其显示最佳偏振域结构和饱和的压电响应环。退火过程有利于在增长方向上具有相同角度的180度域,这在面内信号中引起更多的压电响应。我们的结果表明,压电响应的增加与界面效应和缠绕结构大大相关。

著录项

  • 来源
    《RSC Advances》 |2015年第81期|共7页
  • 作者单位

    Zhejiang Univ Dept Mat Sci &

    Engn Lab Dielect Mat Hangzhou 310027 Zhejiang Peoples R China;

    Univ Texas San Antonio Dept Phys &

    Astron San Antonio TX 78249 USA;

    Univ Texas San Antonio Dept Phys &

    Astron San Antonio TX 78249 USA;

    Univ Texas San Antonio Dept Elect &

    Comp Engn San Antonio TX 78249 USA;

    Univ Texas San Antonio Dept Elect &

    Comp Engn San Antonio TX 78249 USA;

    Univ Texas Arlington Dept Mat Sci &

    Engn Arlington TX 76019 USA;

    Univ Texas Arlington Dept Mat Sci &

    Engn Arlington TX 76019 USA;

    Univ Texas San Antonio Dept Phys &

    Astron San Antonio TX 78249 USA;

    Zhejiang Univ Dept Mat Sci &

    Engn Lab Dielect Mat Hangzhou 310027 Zhejiang Peoples R China;

  • 收录信息
  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类 化学;
  • 关键词

相似文献

  • 外文文献
  • 中文文献
  • 专利
获取原文

客服邮箱:kefu@zhangqiaokeyan.com

京公网安备:11010802029741号 ICP备案号:京ICP备15016152号-6 六维联合信息科技 (北京) 有限公司©版权所有
  • 客服微信

  • 服务号