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首页> 外文期刊>ChemPlusChem >Artificial Molecular Photosynthetic Systems: Towards Efficient Photoelectrochemical Water Oxidation
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Artificial Molecular Photosynthetic Systems: Towards Efficient Photoelectrochemical Water Oxidation

机译:人造分子光合系统:迈向高效的光电化学水氧化

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摘要

Artificial photosynthesis is of great importance in the production of clean fuels such as hydrogen from sunlight and water. In such systems, water oxidation is kinetically demanding; therefore, efficient catalysts and systems for water oxidation are required. Among the artificial systems, photosynthesis has been recently developed owing to the emergence of efficient molecular catalysts for water oxidation. This Review highlights several important concepts including electron transfer and catalysis, and the representative systems of molecular systems for visible-light-driven water oxidation. In addition, the remaining challenges in this field, including the interfacial recombination and the restricted utilization of visible light of over 500nm, are discussed.
机译:人造光合作合作是在阳光和水中的清洁燃料的生产中具有重要意义。 在这种系统中,水氧化在动力学上要求; 因此,需要有效的催化剂和用于水氧化的系统。 在人工系统中,由于有效的分子催化剂用于水氧化,最近已经开发了光合作用。 本综述凸显了几种重要概念,包括电子转移和催化,以及用于可见光水氧化的分子系统的代表性系统。 此外,讨论了该领域的剩余挑战,包括界面重组和可见光的可见光超过500nm的限制使用。

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