Perfect statistical symmetrization of a heterofunctional ligand induced by pseudo-copper trimer in an expanded matrix of HKUST-1

Lin Q.; Bu X.; Feng P.

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Perfect statistical symmetrization of a heterofunctional ligand induced by pseudo-copper trimer in an expanded matrix of HKUST-1

机译：伪铜三聚体在HKUST-1扩展基质中诱导的杂功能配体的完美统计对称性

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The rare coexistence of the copper monomer and paddle-wheel dimer in the same crystal framework creates an apparent linear pseudocopper trimer configuration that induces an unprecedented equalization of pyridyl and carboxyl functionality in a heterofunctional pyridyl dicarboxylate ligand, leading to an intriguing assembly into a highly symmetrical porous framework, despite the low symmetry of the ligand. The material shows a total CO_2 uptake of 55 cm~3/g at 1 atm and 273 K.

机译：铜单体和叶轮二聚体在同一晶体框架中的罕见共存产生了明显的线性拟铜三聚体构型，该构型在异官能吡啶基二羧酸酯配体中诱导了吡啶基和羧基官能团的空前的均等化，从而导致有趣的组装成为高度对称多孔骨架，尽管配体的对称性低。该材料显示在1个大气压和273 K下的总CO_2吸收量为55 cm〜3 / g。

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《Crystal growth & design》 |2013年第12期|共4页
作者
Lin Q.; Bu X.; Feng P.;
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正文语种 eng
中图分类晶体学;
关键词
Perfect statistical; symmetrization; HKUST-1;

机译：完美统计;对称化;HKUST-1;

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机译：伪铜三聚体在HKUST-1扩展基质中诱导的杂功能配体的完美统计对称性
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Perfect statistical symmetrization of a heterofunctional ligand induced by pseudo-copper trimer in an expanded matrix of HKUST-1

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