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Wet‐to‐Dry Hybrid Spinning of Graphene Fiber Inspired by Spider Silk Production Mechanisms

机译：石墨烯纤维的湿化混合纺纱受蜘蛛丝制作机制的启发

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Abstract >This study describes a graphene oxide (GO) fiber spinning method that produces a nearly 100% yield for converting a GO suspension into fibers. The fiber formation method is inspired by the spider silk spinning strategy. The dissolved silk protein, spidroin (wet state), is extruded and shear‐thinned through a posterior spinneret, exposing the silk to a dry state for curing. The wet‐to‐dry conversion in a spider spinneret enables nearly all the fiber precursor, spidroin, to be fabricated into a silk fiber with no loss of protein. Inspired by the process, a “wet‐to‐dry” hybrid spinning of GO is developed in which nearly all GOs are converted into fiber. At the liquid–liquid interface of two droplets containing GO and polyethyleneimine, the two oppositely charged components bind to each other in the wet state. Subsequently, one component touches and pulls the interfacial mixing point of the two droplets, forming a vertical, thin liquid column in which GO complexes experience shear force and directionally align into a thin fiber. Compared to existing wet‐spinning methods, this wet‐to‐dry method is highly energy efficient in terms of the simple procedure, lack of waste chemicals, and nearly 100% conversion of GO precursors. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> 本研究描述了一种石墨烯（GO）纤维纺丝方法，其产生近100％的产率，将悬浮液转化为纤维。纤维形成方法受到蜘蛛丝纺丝策略的启发。溶解的丝蛋白，蜘蛛素（湿态）通过后旋转喷丝挤出和剪切，使丝绸暴露于干燥状态以进行固化。蜘蛛Spinneret中的湿化转化使得几乎所有的纤维前体，蜘蛛素都能够制造成丝纤维，没有蛋白质。通过该方法的启发，开发了“湿到干燥”的杂种纺丝，其中几乎所有的GOS都被转化为纤维。在含有Go和聚乙烯亚胺的两个液滴的液体 - 液体界面处，两个相反的带电部件在湿状状态下彼此结合。随后，一个部件接触并拉动两个液滴的界面混合点，形成垂直的薄液柱，其中去复合物经验剪切力并向薄纤维方向对准。与现有的湿纺丝方法相比，这种湿化的方法在简单的程序，缺乏废物化学品的方面是高度节能，并且近100％转化前体。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2018年第21期</span><b style="margin: 0 2px;">|</b><span>共7页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lee Kyueui&option=202" target="_blank" rel="nofollow">Lee Kyueui;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Do Minjae&option=202" target="_blank" rel="nofollow">Do Minjae;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Seo Young Chang&option=202" target="_blank" rel="nofollow">Seo Young Chang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lee Haeshin&option=202" target="_blank" rel="nofollow">Lee Haeshin;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of ChemistryKorea Advanced Institute of Science and Technology (KAIST)291 University Road Daejeon 34141 Republic of Korea;</p> <p>Department of ChemistryKorea Advanced Institute of Science and Technology (KAIST)291 University Road Daejeon 34141 Republic of Korea;</p> <p>Department of ChemistryKorea Advanced Institute of Science and Technology (KAIST)291 University Road Daejeon 34141 Republic of Korea;</p> <p>Department of ChemistryKorea Advanced Institute of Science and Technology (KAIST)291 University Road Daejeon 34141 Republic of Korea;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=amphiphile&option=203" rel="nofollow">amphiphile;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=graphene fiber&option=203" rel="nofollow">graphene fiber;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=self‐assembly&option=203" rel="nofollow">self‐assembly;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=spider silk&option=203" rel="nofollow">spider silk;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=spinning&option=203" rel="nofollow">spinning;</a> </p> <div class="translation"> 机译：两亲;石墨烯纤维;自组装;蜘蛛丝;旋转; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022434753.html">Wet‐to‐Dry Hybrid Spinning of Graphene Fiber Inspired by Spider Silk Production Mechanisms</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lee Kyueui&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Lee Kyueui,</a> <a 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