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Sulfur Immobilizer by Nanoscale TiO ₂2 Trapper Deposited on Hierarchical Porous Carbon and Graphene for Cathodes of Lithium–Sulfur Batteries

机译：纳米级TiO的硫磺固定剂 _{2 2 矿床上沉积在分层多孔碳和石墨烯上，用于锂 - 硫磺电池的阴极}

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Abstract > Lithium–sulfur (Li–S) batteries are the promising candidate for future energy storage systems due to their high specific capacities and energy densities. However, shuttle effect of the soluble polysulfides severely affects the cycle stability and thus restricts the application of the batteries. Here, a preparation of the titanium oxide (TiO <sub>2</sub> ) nanoparticles uniformly deposited on hierarchical porous carbon (HPC@TiO <sub>2</sub> ) as an efficient sulfur host is reported. The large specific surface area (1016.5 m 2 g ?1 ) and high pore volume of the HPC@TiO <sub>2</sub> host can buffer the volume expansion of the loaded sulfur. The HPC@TiO <sub>2</sub> @S cathode is further wrapped with the TiO <sub>2</sub> nanoparticles interspersed graphene sheets (G/TiO <sub>2</sub> ), which can improve the electrical conductivity of the electrode and suppress the dissolution of polysulfides. As a result, polysulfides are well confined in the G/TiO <sub>2</sub> ‐coated HPC@TiO <sub>2</sub> @S cathode through a synergistic combination of the G/TiO <sub>2</sub> coating and the HPC@TiO <sub>2</sub> host. The resultant G/TiO <sub>2</sub> ‐coated HPC@TiO <sub>2</sub> @S cathode with a sulfur loading about 2.4 mg cm ?2 delivers a high reversible capacity of ≈919 mAh g ?1 after 80 cycles at 0.2 C, and a satisfactory capacity of ≈717 mAh g ?1 is retained after 200 cycles at 0.5 C. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 锂 - 硫（LI-S）电池是未来储能系统的有希望的候选者，因为它们的高特定能力和能量密度。然而，可溶性多硫化物的梭效应严重影响循环稳定性，从而限制了电池的应用。这里，氧化钛的制备（TiO <sub> 2 </ sub> ）均匀沉积在分层多孔碳（HPC @ TiO）上均匀沉积的纳米颗粒 <sub> 2 </ sub> ）报告了一种有效的硫磺宿主。大的比表面积（1016.5米 2 </ sup> G ？1 </ sup> ）HPC @ TiO的高孔体积 <sub> 2 </ sub> 主机可以缓冲加载硫的卷扩展。 HPC @ Tio <sub> 2 </ sub> @S阴极进一步与TIO包裹 <sub> 2 </ sub> 纳米颗粒间隙的石墨烯片（G / TiO <sub> 2 </ sub> ），可以改善电极的电导率并抑制多硫化物的溶解。结果，多硫化物在G / TiO中很好地限制 <sub> 2 </ sub> -Coated HPC @ Tio <sub> 2 </ sub> @S阴极通过G / TIO的协同组合 <sub> 2 </ sub> 涂层和HPC @ TiO <sub> 2 </ sub> 主持人。得到的G / TIO <sub> 2 </ sub> -Coated HPC @ Tio <sub> 2 </ sub> @S阴极带有硫磺加载约2.4mg cm ？2 </ sup> 提供≈919mahg的高可逆能力？1 </ sup> 在0.2 c时80次循环，令人满意的容量≈717mahg ？1 </ sup> 在0.5℃下200次循环后保留。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2018年第7期</span><b style="margin: 0 2px;">|</b><span>共8页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Shang Xiaonan&option=202" target="_blank" rel="nofollow">Shang Xiaonan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Guo Pengqian&option=202" target="_blank" rel="nofollow">Guo Pengqian;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Qin Tianfeng&option=202" target="_blank" rel="nofollow">Qin Tianfeng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Mengting&option=202" target="_blank" rel="nofollow">Liu Mengting;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lv Mingzhi&option=202" target="_blank" rel="nofollow">Lv Mingzhi;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Dequan&option=202" target="_blank" rel="nofollow">Liu Dequan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=He Deyan&option=202" target="_blank" rel="nofollow">He Deyan;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>School of Physical Science and Technology and Key Laboratory for Magnetism and Magnetic Materials of the Ministry of EducationLanzhou UniversityLanzhou 730000 China;</p> <p>School of Physical Science and Technology and Key Laboratory for Magnetism and Magnetic Materials of the Ministry of EducationLanzhou UniversityLanzhou 730000 China;</p> <p>School of Physical Science and Technology and Key Laboratory for Magnetism and Magnetic Materials of the Ministry of EducationLanzhou UniversityLanzhou 730000 China;</p> <p>School of Physical Science and Technology and Key Laboratory for Magnetism and Magnetic Materials of the Ministry of EducationLanzhou UniversityLanzhou 730000 China;</p> <p>School of Physical Science and Technology and Key Laboratory for Magnetism and Magnetic Materials of the Ministry of EducationLanzhou UniversityLanzhou 730000 China;</p> <p>School of Physical Science and Technology and Key Laboratory for Magnetism and Magnetic Materials of the Ministry of EducationLanzhou UniversityLanzhou 730000 China;</p> <p>School of Physical Science and Technology and Key Laboratory for Magnetism and Magnetic Materials of the Ministry of EducationLanzhou UniversityLanzhou 730000 China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ketjen black&option=203" rel="nofollow">Ketjen black;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=lithium–sulfur batteries&option=203" rel="nofollow">lithium–sulfur batteries;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=shuttle effect&option=203" rel="nofollow">shuttle effect;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=sulfur cathode&option=203" rel="nofollow">sulfur cathode;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=TiO 2&option=203" rel="nofollow">TiO 2;</a> </p> <div class="translation"> 机译：Ketjen Black;锂 - 硫磺电池;梭效果;硫阴极;TiO 2; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" 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Sulfur Immobilizer by Nanoscale TiO 22 Trapper Deposited on Hierarchical Porous Carbon and Graphene for Cathodes of Lithium–Sulfur Batteries

摘要

Sulfur Immobilizer by Nanoscale TiO ₂2 Trapper Deposited on Hierarchical Porous Carbon and Graphene for Cathodes of Lithium–Sulfur Batteries