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Realizing the Embedded Growth of Large Li ₂2 O ₂2 Aggregations by Matching Different Metal Oxides for High‐Capacity and High‐Rate Lithium Oxygen Batteries

机译：实现大李的嵌入式生长 _{2 2 O. _{2 2 通过匹配不同的金属氧化物，用于高容量和高速锂氧气电池的聚集}}

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Abstract > Large Li <sub>2</sub> O <sub>2</sub> aggregations can produce high‐capacity of lithium oxygen (Li‐O <sub>2</sub> ) batteries, but the larger ones usually lead to less‐efficient contact between Li <sub>2</sub> O <sub>2</sub> and electrode materials. Herein, a hierarchical cathode architecture based on different discharge characteristics of α‐MnO <sub>2</sub> and Co <sub>3</sub> O <sub>4</sub> is constructed, which can enable the embedded growth of large Li <sub>2</sub> O <sub>2</sub> aggregations to solve this problem. Through experimental observations and first‐principle calculations, it is found that α‐MnO <sub>2</sub> nanorod tends to form uniform Li <sub>2</sub> O <sub>2</sub> particles due to its preferential Li + adsorption and similar LiO <sub>2</sub> adsorption energies of different crystal faces, whereas Co <sub>3</sub> O <sub>4</sub> nanosheet tends to simultaneously generate Li <sub>2</sub> O <sub>2</sub> film and Li <sub>2</sub> O <sub>2</sub> nanosheets due to its preferential O <sub>2</sub> adsorption and different LiO <sub>2</sub> adsorption energies of varied crystal faces. Thus, the composite cathode architecture in which Co <sub>3</sub> O <sub>4</sub> nanosheets are grown on α‐MnO <sub>2</sub> nanorods can exhibit extraordinary synergetic effects, i.e., α‐MnO <sub>2</sub> nanorods provide the initial nucleation sites for Li <sub>2</sub> O <sub>2</sub> deposition while Co <sub>3</sub> O <sub>4</sub> nanosheets provide dissolved LiO <sub>2</sub> to promote the subsequent growth of Li <sub>2</sub> O <sub>2</sub> . Consequently, the composite cathode achieves the embedded growth of large Li <sub>2</sub> O <sub>2</sub> aggregations and thus exhibits significantly improved specific capacity, rate capability, and cyclic stability compared with the single metal oxide electrode. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract XMLNS =“http://www.wiley.com/namespaces/wiley”type =“main”xml：lang =“en”> <标题类型=“main”>抽象</ title> > 大李 <sub> 2 </ sub> O. <sub> 2 </ sub> 聚集可以产生高容量的锂氧气（Li-O. <sub> 2 </ sub> ）电池，但较大的电池通常会导致李之间的效率较差接触 <sub> 2 </ sub> O. <sub> 2 </ sub> 和电极材料。这里，基于α-mno的不同放电特性的分层阴极架构 <sub> 2 </ sub> 和co. <sub> 3 </ sub> O. <sub> 4 </ sub> 构建，可以实现大李的嵌入式生长 <sub> 2 </ sub> O. <sub> 2 </ sub> 聚合来解决这个问题。通过实验观察和第一原理计算，发现α-mno <sub> 2 </ sub> Nanorod倾向于形成均匀的李 <sub> 2 </ sub> O. <sub> 2 </ sub> 颗粒由于其优惠李 + </ sup> 吸附和类似的Lio <sub> 2 </ sub> 不同水晶面的吸附能量，而CO <sub> 3 </ sub> O. <sub> 4 </ sub> Nanosheet往往同时产生李 <sub> 2 </ sub> O. <sub> 2 </ sub> 电影和李 <sub> 2 </ sub> O. <sub> 2 </ sub> 纳米表由于其优惠o <sub> 2 </ sub> 吸附和不同的Lio <sub> 2 </ sub> 不同水晶面的吸附能量。因此，复合阴极架构在其中有限公司 <sub> 3 </ sub> O. <sub> 4 </ sub> Nanosheets在α-mno种植 <sub> 2 </ sub> 纳米棒可以表现出非凡的协同作用，即α-mno <sub> 2 </ sub> Nanorods为Li提供初始成核位点 <sub> 2 </ sub> O. <sub> 2 </ sub> CO. <sub> 3 </ sub> O. <sub> 4 </ sub> Nanosheets提供溶解的Lio <sub> 2 </ sub> 促进李的随后生长 <sub> 2 </ sub> O. <sub> 2 </ sub> 。因此，复合阴极达到大李的嵌入式生长 <sub> 2 </ sub> O. <sub> 2 </ sub> 与单一金属氧化物电极相比，聚合并因此表现出显着提高的特定容量，速率能力和循环稳定性。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2017年第11期</span><b style="margin: 0 2px;">|</b><span>共1页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Peng&option=202" target="_blank" rel="nofollow">Zhang Peng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Shoufeng&option=202" target="_blank" rel="nofollow">Zhang Shoufeng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=He Mu&option=202" target="_blank" rel="nofollow">He Mu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lang Junwei&option=202" target="_blank" rel="nofollow">Lang Junwei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ren Aimin&option=202" target="_blank" rel="nofollow">Ren Aimin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xu Shan&option=202" target="_blank" rel="nofollow">Xu Shan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yan Xingbin&option=202" target="_blank" rel="nofollow">Yan Xingbin;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Laboratory of Clean Energy Chemistry and MaterialsChinese Academy of SciencesLanzhou 730000 P. R. China;</p> <p>State Key Laboratory of Theoretical and Computational ChemistryJilin UniversityJilin 130023 P. R. China;</p> <p>University of Chinese Academy of SciencesBeijing 100039 P. R. China;</p> <p>Laboratory of Clean Energy Chemistry and MaterialsChinese Academy of SciencesLanzhou 730000 P. R. China;</p> <p>State Key Laboratory of Theoretical and Computational ChemistryJilin UniversityJilin 130023 P. R. China;</p> <p>State Key Laboratory for Oxo Synthesis and Selective OxidationChinese Academy of SciencesLanzhou 730000 P. R. China;</p> <p>Laboratory of Clean Energy Chemistry and MaterialsChinese Academy of SciencesLanzhou 730000 P. R. China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=discharge characteristics&option=203" rel="nofollow">discharge characteristics;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li 2 O 2&option=203" rel="nofollow">Li 2 O 2;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=LiO 2 adsorption energy&option=203" rel="nofollow">LiO 2 adsorption energy;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li‐O 2 batteries&option=203" rel="nofollow">Li‐O 2 batteries;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=metal oxides&option=203" rel="nofollow">metal oxides;</a> </p> <div class="translation"> 机译：放电特性;Li 2 O 2;LiO 2吸附能量;Li-O 2电池;金属氧化物; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022434827.html">Realizing the Embedded Growth of Large Li <sub xmlns="http://www.wiley.com/namespaces/wiley">2</sub>2 O <sub 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Realizing the Embedded Growth of Large Li 22 O 22 Aggregations by Matching Different Metal Oxides for High‐Capacity and High‐Rate Lithium Oxygen Batteries

摘要

Realizing the Embedded Growth of Large Li ₂2 O ₂2 Aggregations by Matching Different Metal Oxides for High‐Capacity and High‐Rate Lithium Oxygen Batteries