Engineered Nitrogen-Decorated Carbon Networks for the Metal-Free Catalytic Isomerization of Glucose to Fructose

Chen Season S.; Carraher Jack M.; Tuci Giulia; Rossin Andrea; Raman Caleb A.; Luconi Lapo; Tsang Daniel C. W.; Giambastiani Giuliano; Tessonnier Jean-Philippe

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Engineered Nitrogen-Decorated Carbon Networks for the Metal-Free Catalytic Isomerization of Glucose to Fructose

机译：用于葡萄糖的无金属催化异构化的工程化氮气装饰碳网络

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Bronsted bases have recently been reported to catalyze the glucose isomerization to fructose. This contribution describes the rational bottom-up approach to the design and synthesis of heterogeneous systems based on a C-60 platform surface engineered with catalytically active amino functionalities tethered to carbon nanomaterials within variable (polar/apolar) chemical microenvironments. We demonstrate how carbocatalysts performance for the glucose-to-fructose isomerization may improve depending on amines' neighboring functional groups and their chemical interplay at the C-nanocarrier surface.

机译：最近据报道勃朗斯特基地据报道催化葡萄糖异构化对果糖。该贡献描述了基于C-60平台表面的基于C-60平台表面的基于C-60平台表面的无均匀系统的结构和合成的合理自下而上的方法，所述C-60平台表面与可变（极性/浮动）化学微环境中的碳纳米材料系在碳纳米材料中。我们证明了葡萄糖催化剂的性能如何对葡萄糖对果糖异构化的性能可以根据胺的相邻官能团及其在C纳米载体表面的化学相互作用而改善。

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来源
《ACS Sustainable Chemistry & Engineering》 |2019年第20期|共5页
作者
Chen Season S.; Carraher Jack M.; Tuci Giulia; Rossin Andrea; Raman Caleb A.; Luconi Lapo; Tsang Daniel C. W.; Giambastiani Giuliano; Tessonnier Jean-Philippe;
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作者单位

Iowa State Univ Dept Chem &

Biol Engn Ames IA 50011 USA;

Iowa State Univ Dept Chem &

Biol Engn Ames IA 50011 USA;

CNR Inst Chem OrganoMetall Cpds ICCOM CNR Via Madonna Piano 10 I-50019 Florence Italy;

CNR Inst Chem OrganoMetall Cpds ICCOM CNR Via Madonna Piano 10 I-50019 Florence Italy;

Iowa State Univ Dept Chem &

Biol Engn Ames IA 50011 USA;

CNR Inst Chem OrganoMetall Cpds ICCOM CNR Via Madonna Piano 10 I-50019 Florence Italy;

Hong Kong Polytech Univ Dept Civil &

Environm Engn Kowloon Hong Kong Peoples R China;

CNR Inst Chem OrganoMetall Cpds ICCOM CNR Via Madonna Piano 10 I-50019 Florence Italy;

Iowa State Univ Dept Chem &

Biol Engn Ames IA 50011 USA;

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原文格式 PDF
正文语种 eng
中图分类化学工业;
关键词
Glucose-to-fructose isomerization; Metal-free heterogeneous catalysis; N-Decorated nanocarbons; Chemical functionalization; Functional group synergy;

机译：葡萄糖 - 果糖异构化;无金属异质催化;N装饰纳米碳;化学功能化;功能群协同作用;

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专利

1. Engineered Nitrogen-Decorated Carbon Networks for the Metal-Free Catalytic Isomerization of Glucose to Fructose [J] . Chen Season S., Carraher Jack M., Tuci Giulia, ACS Sustainable Chemistry & Engineering . 2019,第20期

机译：用于葡萄糖的无金属催化异构化的工程化氮气装饰碳网络
2. Catalytic isomerization of D-glucose to D-fructose over BEA base zeotypes using different energy supply methods [J] . Antunes Margarida M., Falcao Diogo, Fernandes Auguste, Catalysis Today . 2021,第1期

机译：用不同能量供应方法将D-葡萄糖对D-果糖的催化异构化
3. Cooperative Catalytic Performance of Lewis and Bronsted Acids from AlCl3 Salt in Aqueous Solution toward Glucose-to-Fructose Isomerization [J] . Qi Ting, He Meng-Fu, Zhu Liang-Fang, The journal of physical chemistry, C. Nanomaterials and interfaces . 2019,第8期

机译：从AlCl3盐中的Lewis和BrONsted酸的合作催化性能在水溶液中对葡萄糖 - 果糖异构化的
4. The beneficial effect of fructose on the catalytic oxidation of glucose to gluconic acid [C] . Fabiana S. Lima, Joao Guilherme, R. Poco AIChE Annual Meeting . 2016

机译：果糖对葡萄糖催化氧化对葡萄糖酸的有益作用
5. Catalytic conversion of glucose, fructose, and sucrose to high-valued chemicals. [D] . Jacobs, Jennifer Elizabeth. 2000

机译：葡萄糖，果糖和蔗糖催化转化为高价值化学品。
6. A Double-Blind Randomized Controlled Acute Feeding Equivalence Trial of Small Catalytic Doses of Fructose and Allulose on Postprandial Blood Glucose Metabolism in Healthy Participants: The Fructose and Allulose Catalytic Effects (FACE) Trial [O] . Catherine R. Braunstein, Jarvis C. Noronha, Andrea J. Glenn, 2018

机译：小剂量果糖和阿卢糖催化剂量对健康参与者餐后血糖代谢的双盲随机对照急性进食当量试验：果糖和阿卢糖催化作用（FACE）试验
7. Catalytic isomerization of glucose to fructose using heterogeneous solid Base catalysts in a continuous-flow tubular reactor: Catalyst screening study [O] . Sadra Souzanchi, Laleh Nazari, Kasanneni Tirumala Venkateswara Rao, 2019

机译：在连续流管式反应器中使用非均相固体基催化剂催化异构化葡萄糖对果糖：催化剂筛选研究
8. Photochemical Formation of Mononuclear Bis and Tris Ethylene Complexes from Irradiation of Iron Pentacarbonyl or Triruthenium Dodecarcarbonyl: Species Involved in Catalytic Alkene Isomerization [R] . Wuu, Y. M., Bentsen, J. G., Brinkley, C. G., 1986

机译：由五羰基铁或三钌十二烷基羰基化合物光化学形成单核双和三乙烯配合物：参与催化烯烃异构化的物种

Engineered Nitrogen-Decorated Carbon Networks for the Metal-Free Catalytic Isomerization of Glucose to Fructose

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