Ruthenium Nanoparticle-Decorated Porous Organic Network for Direct Hydrodeoxygenation of Long-Chain Fatty Acids to Alkanes

Mondal Sujan; Singuru Ramana; Shit Subhash Chandra; Hayashi Taku; Irle Stephan; Hijikata Yuh; Mondal John; Bhaumik Asim

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Ruthenium Nanoparticle-Decorated Porous Organic Network for Direct Hydrodeoxygenation of Long-Chain Fatty Acids to Alkanes

机译：钌纳米粒子装饰多孔有机网络，用于直链脂肪酸的直链加氢氧基对烷烃

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With the rapidly diminishing fossil fuel resources, development of a new strategy for synthesis of biofuels from renewable resources can provide a sustainable alternative to our energy demand. We present the design, synthesis, and characterization of a new porous organic network (TpPON) through acid-catalyzed condensation of 1,3,5-triformylphloroglucinol (Tp) and triphenylamine (TPA). Ru-0 nanoparticles are successfully fabricated at the porous surface of TpPON to obtain a novel catalytic system Ru@TpPON, which exhibits excellent catalytic performance together with outstanding stability for the hydrodeoxygenation of various vegetable oils to long-chain alkanes in water, and thus TpPON has wide potential for large-scale biodiesel production from renewable resources.

机译：随着化石燃料资源迅速减少，开发来自可再生资源的生物燃料的合成策略可以为我们的能源需求提供可持续的替代品。我们通过酸催化的1,3,5-曲氯葡糖蛋白（TP）和三苯胺（TPA）呈现新多孔有机网络（TPPON）的设计，合成和表征TPPON）。 Ru-0纳米颗粒在TPPON的多孔表面上成功制造，得到一种新型催化系统Ru @TPPON，其具有优异的催化性能，以及各种植物油的水牛氧基在水中的长链烷烃中的优异稳定性，因此TPPON 具有可再生资源的大型生物柴油生产潜力。

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来源
《ACS Sustainable Chemistry & Engineering》 |2018年第2期|共10页
作者
Mondal Sujan; Singuru Ramana; Shit Subhash Chandra; Hayashi Taku; Irle Stephan; Hijikata Yuh; Mondal John; Bhaumik Asim;
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作者单位

Indian Assoc Cultivat Sci Dept Mat Sci 2A &

2B Raja SC Mullick Rd Kolkata 700032 India;

CSIR Indian Inst Chem Technol Inorgan &

Phys Chem Div Uppal Rd Hyderabad 500007 Andhra Pradesh India;

CSIR Indian Inst Chem Technol Inorgan &

Phys Chem Div Uppal Rd Hyderabad 500007 Andhra Pradesh India;

Nagoya Univ Inst Transformat Biomol WPI ITbM Chikusa Ku Furo Cho Nagoya Aichi 4648602 Japan;

Nagoya Univ Inst Transformat Biomol WPI ITbM Chikusa Ku Furo Cho Nagoya Aichi 4648602 Japan;

Nagoya Univ Inst Transformat Biomol WPI ITbM Chikusa Ku Furo Cho Nagoya Aichi 4648602 Japan;

CSIR Indian Inst Chem Technol Inorgan &

Phys Chem Div Uppal Rd Hyderabad 500007 Andhra Pradesh India;

Indian Assoc Cultivat Sci Dept Mat Sci 2A &

2B Raja SC Mullick Rd Kolkata 700032 India;

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原文格式 PDF
正文语种 eng
中图分类化学工业;
关键词
Microporous; Free hydroxyl groups; Heterogeneous catalyst; Hydrogenation; Long-chain alkane fuel;

机译：微孔;游离羟基;非均相催化剂;氢化;长链烷烃燃料;

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1. Ruthenium Nanoparticle-Decorated Porous Organic Network for Direct Hydrodeoxygenation of Long-Chain Fatty Acids to Alkanes [J] . Mondal Sujan, Singuru Ramana, Shit Subhash Chandra, ACS Sustainable Chemistry & Engineering . 2018,第2期

机译：钌纳米粒子装饰多孔有机网络，用于直链脂肪酸的直链加氢氧基对烷烃
2. The potential use of n-alkanes, long-chain alcohols and long-chain fatty acids as diet composition markers: indoor validation with sheep and herbage species from the rangeland of Inner Mongolia of China [J] . C. Jiang, F. Z. Hong, H. L. Luo, Animal . 2011,第3期

机译：正构烷烃，长链醇和长链脂肪酸作为饮食成分标记物的潜在用途：使用来自中国内蒙古草原的绵羊和牧草种进行室内验证
3. Direct hydrodeoxygenation of cellulose and xylan to lower alkanes on ruthenium catalysts in subcritical water [J] . Yuriko Osaka, Yoichi Ikeda, Daisuke Hashizume, Biomass & bioenergy . 2013,第sepa期

机译：亚临界水中钌催化剂上的纤维素和木聚糖直接加氢脱氧为低级烷烃
4. Carbonaceous material, alkanes, long-chain carboxylic acids and PAHs in PM10: concentration levels and sources in Rome [C] . P. Avino, D. Brocco, A. Cecinato Tenth International Conference on Modelling, Monitoring and Management of Air Pollution Jul, 2002 City of Segovia . 2002

机译：PM10中的含碳物质，烷烃，长链羧酸和PAH：罗马的浓度水平和来源
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机译：罹患乳腺癌高风险女性的长链多不饱和脂肪酸摄入及其与红细胞和血浆长链多不饱和脂肪酸的关系。
6. Direct hydrodeoxygenation of raw woody biomass into liquid alkanes [O] . Qineng Xia, Zongjia Chen, Yi Shao, -1

机译：将原始木质生物质直接加氢脱氧成液态烷烃
7. Enhanced induction of cytochromes P450alk that oxidize methyl-ends of n-alkanes and fatty acids in the long-chain dicarboxylic acid-hyperproducing mutant of Candida maltosa [O] . Takahisa Kogure, Hiroyuki Horiuchi, Hitoshi Matsuda, 2007

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8. Synthesis and Biological Evaluation of (E)-19-Iodo-3,3-Dimethyl-18-Nonadecenoic Acid, a New Dimethyl-Branched Long-Chain Fatty Acid to Evaluate Regional Myocardial Fatty Acid Uptake [R] . Goodman, M. M., Ambrose, K. R., Neff, K. H., 1986

机译：（E）-19-碘-3,3-二甲基-18-十一碳烯酸（一种新的二甲基支链长链脂肪酸）的合成和生物学评价，用于评估局部心肌脂肪酸的摄取

Ruthenium Nanoparticle-Decorated Porous Organic Network for Direct Hydrodeoxygenation of Long-Chain Fatty Acids to Alkanes

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