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首页> 外文期刊>Crystal growth & design >Controllable synthesis of three-dimensional well-defined BiVO4 mesocrystals via a facile additive-free aqueous strategy
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Controllable synthesis of three-dimensional well-defined BiVO4 mesocrystals via a facile additive-free aqueous strategy

机译：通过简便的无添加剂水溶液策略可控地合成三维明确定义的BiVO4介观晶体

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摘要

The controllable synthesis of two novel types of BiVO4 mesocrystals, with flower-like and dendrite morphology, has been successfully realized via a facile aqueous strategy. Without any additive, the primary building units perfectly aligned in three-dimension and built up well-defined mesocrystals with sharp facets and edges. The formation mechanism was further investigated, and new growth models for the mesocrystals were observed. It was found that that the pH value and reaction temperature had great influences on the formation of these unique mesocrystals. The present study not only opens new avenues for rationally designing various kinds of inorganic materials with ideal hierarchy and controllable length scale but also offers a good opportunity to understand the formation process of these unique crystalline superstructures.
机译：两种新颖的BiVO4介孔晶体的可控合成，具有花状和枝晶形态，已通过一种简便的水策略成功实现。在没有任何添加剂的情况下，主要的构建单元在三维方向上完美对齐，并构建了具有清晰的小面和边缘的轮廓分明的介晶。进一步研究了形成机理，并观察到了新的介孔晶体生长模型。发现pH值和反应温度对这些独特的介晶的形成有很大的影响。本研究不仅为合理设计具有理想层次和可控制长度尺度的各种无机材料开辟了新途径，而且为了解这些独特的晶体超结构的形成过程提供了一个很好的机会。

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