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首页> 外文期刊>ACS Macro Letters >100th Anniversary of Macromolecular Science Viewpoint: Recent Advances and Opportunities for Mixed Ion and Charge Conducting Polymers
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100th Anniversary of Macromolecular Science Viewpoint: Recent Advances and Opportunities for Mixed Ion and Charge Conducting Polymers

机译：大分子科学观点100周年：最近的混合离子和电荷导电聚合物的进步和机会

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Macromolecules that exhibit both electron transport and ionic mass transport (i.e., mixed conducting polymers) are ascendant with respect to both emerging application spaces and the elucidation of their fundamental physical principles. The unique coupling between the two modes of conduction puts these materials at the center of many next-generation organic electronic applications. The molecular details of this coupling are also at the epicenter of outstanding questions about how these materials function; how monomer and macromolecular chemistry dictates observable properties; and ultimately, how these macromolecular materials can be rationally designed, processed, and implemented into high-performance devices. Here, we focus on what is currently known about coupled ionic-electronic transport in these polymers and where there are open opportunities in the field. These opportunities include the syntheses of designer macromolecules, the need for significant simulation efforts that provide molecular-level insights into the mixed conduction mechanism, and the need for advanced characterization techniques for real-time monitoring of polymer morphology, as this is critical to coupled ion-charge transport processes. Considering the early stage of this important subfield of polymer science, we also present our view of how the development of mixed conductors can benefit from the lessons learned from previous polymerbased electronic devices.
机译：表现出电子传输和离子质量转运（即混合导电聚合物）的大分子是关于新兴应用空间的升级，并阐明其基本物理原则。两种传导方式之间的独特耦合将这些材料放在许多下一代有机电子应用的中心。该耦合的分子细节也在出色问题的震中，了解这些材料功能如何;单体和大分子化学如何决定可观察的性质;最终，这些大分子材料如何合理地设计，处理和实施到高性能设备中。在这里，我们专注于这些聚合物中关于耦合离子电子传输的内容以及在该领域的开放机会。这些机会包括设计师大分子的合成，需要进行重大模拟努力，这些努力提供分子水平洞察的混合传导机制，以及对聚合物形态的实时监测的先进表征技术的需求，因为这对耦合离子至关重要 - 充电运输过程。考虑到这个重要的聚合物科学子场的早期阶段，我们还提出了了解混合导体的发展如何从来自以前的聚合物电子设备中学到的经验教训中受益。

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    《ACS Macro Letters》 |2020年第5期|共10页
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  • 正文语种 eng
  • 中图分类 有机化学;
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