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首页> 外文期刊>Annual Review of Physical Chemistry >Atmospheric Spectroscopy and Photochemistry at Environmental Water Interfaces
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Atmospheric Spectroscopy and Photochemistry at Environmental Water Interfaces

机译：环境水界面的大气光谱和光化学

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The air-water interface is ubiquitous in nature, as manifested in the form of the surfaces of oceans, lakes, and atmospheric aerosols. The aerosol interface, in particular, can play a crucial role in atmospheric chemistry. The adsorption of atmospheric species onto and into aerosols modifies their concentrations and chemistries. Moreover, the aerosol phase allows otherwise unlikely solution-phase chemistry to occur in the atmosphere. The effect of the air-water interface on these processes is not entirely known. This review summarizes recent theoretical investigations of the interactions of atmosphere species with the air-water interface, including reactant adsorption, photochemistry, and the spectroscopy of reactants at the water surface, with an emphasis on understanding differences between interfacial chemistries and the chemistries in both bulk solution and the gas phase. The results discussed here enable an understanding of fundamental concepts that lead to potential air-water interface effects, providing a framework to understand the effects of water surfaces on our atmosphere.
机译：气水界面本质上是无处不在的，如海洋，湖泊和大气气溶胶表面的形式。特别是气溶胶界面可以在大气化学中发挥至关重要的作用。将大气层的吸附到气溶胶中改变它们的浓度和化学品。此外，气溶胶相允许在大气中发生否则不太可能的溶液相化学。空气界面对这些过程的影响并不完全已知。本综述总结了近大气法与空气水界面相互作用的理论研究，包括水面反应物的反应性吸附，光化学和光谱，重点是理解界面化学物质与散装中的化学物质之间的差异溶液和气相。这里讨论的结果能够理解导致潜在的空气界面效应的基本概念，提供了一个框架，以了解水面对我们大气的影响。

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