Electrocatalysis of Cu?MOF/Graphene Composite and its Sensing Application for Electrochemical Simultaneous Determination of Dopamine and Paracetamol

Ma Baolong; Guo Hao; Wang Mingyue; Li Li; Jia Xueyan; Chen Huiqin; Xue Rui; Yang Wu

摘要

Abstract >A nanocomposite of HKUST‐1 (MOF) and electroreduction graphene oxide (ERGO) is prepared and applied as an electrochemical sensor for the simultaneous determination of paracetamol and dopamine by means of one‐step electrodeposition. The MOF/ERGO composite displays excellent electrochemical catalytic activities towards the paracetamol and dopamine, which is attributed to the synergistic effect of big surface area, porosity and high electrocataytic activity of the MOF and good conductivity of ERGO. The modified electrode could be applied to determine simultaneously paracetamol and dopamine in biochemical samples with wide linear ranges (0.2?μM to 160?μM for paracetamol and 0.2?μM to 300?μM for dopamine) and low detection limits (0.016?μM for paracetamol and 0.013?μM for dopamine). Meanwhile, the proposed sensor still displays high sensitivity, good selectivity and excellent stability. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>摘要</标题> > HKust-1（MOF）的纳米复合材料和电导氧化物氧化物（ERGO）施加为电化学传感器，用于通过一步电沉积同时测定扑热息痛和多巴胺。 MOF / ERGO Compopite显示朝向扑热息痛和多巴胺的优异的电化学催化活性，这归因于大表面积，孔隙率和MOF的高电凝活度和良好的ERGO导电性的协同效应。可以施加改性电极以在具有宽线性范围（0.2×μm至160μm的生化样品中同时测定扑热胺和多巴胺，用于扑热酰胺和0.2Ω·μm至300μm的多巴胺）和低检测限（0.016≤μm用于扑热氨基酚为多巴胺0.013？μm）。同时，所提出的传感器仍然显示出高灵敏度，良好的选择性和优异的稳定性。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-22546/'>《Electroanalysis》</a> <b style="margin: 0 2px;">|</b><span>2019年第6期</span><b style="margin: 0 2px;">|</b><span>共7页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ma Baolong&option=202" target="_blank" rel="nofollow">Ma Baolong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Guo Hao&option=202" target="_blank" rel="nofollow">Guo Hao;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Mingyue&option=202" target="_blank" rel="nofollow">Wang Mingyue;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Li&option=202" target="_blank" rel="nofollow">Li Li;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jia Xueyan&option=202" target="_blank" rel="nofollow">Jia Xueyan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chen Huiqin&option=202" target="_blank" rel="nofollow">Chen Huiqin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xue Rui&option=202" target="_blank" rel="nofollow">Xue Rui;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Wu&option=202" target="_blank" rel="nofollow">Yang Wu;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Key Lab of Bioelectrochemistry and Environmental Analysis of Gansu ProvinceLanzhou 730070 PR China;</p> <p>Key Lab of Bioelectrochemistry and Environmental Analysis of Gansu ProvinceLanzhou 730070 PR China;</p> <p>Key Lab of Bioelectrochemistry and Environmental Analysis of Gansu ProvinceLanzhou 730070 PR China;</p> <p>Key Lab of Bioelectrochemistry and Environmental Analysis of Gansu ProvinceLanzhou 730070 PR China;</p> <p>Key Lab of Bioelectrochemistry and Environmental Analysis of Gansu ProvinceLanzhou 730070 PR China;</p> <p>Key Lab of Bioelectrochemistry and Environmental Analysis of Gansu ProvinceLanzhou 730070 PR China;</p> <p>Key Lab of Bioelectrochemistry and Environmental Analysis of Gansu ProvinceLanzhou 730070 PR China;</p> <p>Key Lab of Bioelectrochemistry and Environmental Analysis of Gansu ProvinceLanzhou 730070 PR China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/4817.html" title="电化学、电解、磁化学">电化学、电解、磁化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Simultaneous determination&option=203" rel="nofollow">Simultaneous determination;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Cu–MOF&option=203" rel="nofollow">Cu–MOF;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Electrodeposition&option=203" rel="nofollow">Electrodeposition;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Paracetamol&option=203" rel="nofollow">Paracetamol;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Dopamine&option=203" rel="nofollow">Dopamine;</a> </p> <div class="translation"> 机译：同时测定;Cu-Mof;电沉积;扑热息痛;多巴胺; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704023174196.html">Electrocatalysis of Cu?MOF/Graphene Composite and its Sensing Application for Electrochemical Simultaneous Determination of Dopamine and Paracetamol</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ma Baolong&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Ma Baolong,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Guo Hao&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Guo Hao,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang 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href="/academic-conference-cn_meeting-7084_thesis/020221847655.html">二氧化硅覆盖的氧化石墨烯-表面分子印迹复合材料的研制及其对多巴胺电化学性质研究</a> <b>[C]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yanbo Zeng&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 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href="/patent-detail/06120103829103.html">一种Cu-MOFs负载的氮掺杂石墨烯复合材料及其制备方法和应用</a> <b>[P]</b> . <span> 中国专利： CN111272840A </span> <span> . 2020-06-12</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120100945890.html">一种π-d共轭Cu-MOF/碳化钛复合材料的制备及其在电化学储能中的应用</a> <b>[P]</b> . <span> 中国专利： CN109994320A </span> <span> . 2019-07-09</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130419391992.html">ELECTROCHEMICAL BIOSENSOR BY ELECTROCATALYSIS OF ELECTROCHEMICALLY REDUCED GRAPHENE OXIDES, METHOD FOR MANUFACTURING THE SAME, AND SENSING METHOD</a> <b>[P]</b> . <span> 外国专利：  KR20130121464A </span> <span> . 2013-11-06</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：通过电化学还原的石墨烯氧化物进行电化学电解的电化学生物传感器，其制造方法和传感方法 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130425401244.html">ELECTROCHEMICAL BIOSENSOR FOR SIMULTANEOUS DETERMINATION OF SUPEROXIDE ANION RADICAL AND NITRITE USING CU, ZNSOD IMMOBILIZED ON HYBRID GOLD NANOPARTICLES/CARBON NANOTUBES IN CONDUCTING POLYMER NANOCOMPOSITE</a> <b>[P]</b> . <span> 外国专利：  IN2010CH00668A </span> <span> . 2011-09-23</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：电化学生物传感器同时测定混合金纳米粒子/碳纳米管中固定化的铜，ZNSOD铜，同时测定聚合物纳米复合材料中的过氧化阴离子自由基和亚硝酸根 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130422992553.html">A kind of Multilayer Composite Tube or plastic / metal composition can be termofusionado simultaneously in two sectors, an accessory for termofusionarse simultaneously with the two sectors of the composite Tube, a Nozzle for Heat fusion simultaneously Said Tube C</a> <b>[P]</b> . <span> 外国专利：  AR079308A1 </span> <span> 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