Production, consumption, and migration of methane in accretionary prism of southwestern Taiwan

Chen Nai‐Chen; Yang Tsanyao Frank; Hong Wei‐Li; Chen Hsuan‐Wen; Chen Hsiao‐Chi; Hu Ching‐Yi; Huang Yu‐Chun; Lin Saulwood; Lin Li‐Hung; Su Chih‐Chieh; Liao Wei‐Zhi; Sun Chih‐Hsien; Wang Pei‐Ling; Yang Tao; Jiang Shao‐Yong; Liu Char‐Shine; Wang Yunshuen; Chung San‐Hsiung

摘要

Abstract > To systematically quantify the production, consumption, and migration of methane, 210 sediment cores were collected from offshore southwestern Taiwan and analyzed for their gas and aqueous geochemistry. These data, combined with published results, were used to calculate the diffusive methane fluxes across different geochemical transitions and to develop scenarios of mass balance and constrain deep microbial and thermogenic methane production rates within the accretionary prism. The results showed that methane diffusive fluxes ranged from 2.71 × 10 ?3 to 2.78 × 10 ?1 and from –1.88 × 10 ?1 to 3.97 mmol m ?2 d ?1 at the sulfate‐methane‐transition‐zone (SMTZ) and sediment‐seawater interfaces, respectively. High methane fluxes tend to be associated with structural features, suggesting a strong structural control on the methane transport. A significant portion of ascending methane (50%) is consumed by anaerobic oxidation of methane at the SMTZ at most sites, indicating effective biological filtration. Gas compositions and isotopes revealed a transition from the predominance of microbial methane in the passive margin to thermogenic methane at the upper slope of the active margin and onshore mud volcanoes. Methane production and consumption at shallow depths were nearly offset with a small fraction of residual methane discharged into seawater. The flux imbalance arose primarily due to the larger production of methane through deep microbial and thermogenic processes at a magnitude of 1512–43,096 Tg Myr ?1 and could be likely accounted for by the sequestration of methane into hydrate forms, and clay absorption. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“main”> <标题类型=“main”>抽象</ title> > 为了系统地量化甲烷的生产，消费和迁移，从台湾海上陆上收集了210个沉积物核心，并分析了它们的天然气和地球化学水质。这些数据与已发表的结果相结合用于计算不同地球化学过渡的衍射甲烷通量，并在增生棱镜中制定质量平衡和限制深层微生物和热甲烷产量的情况。结果表明，甲烷扩散势率范围为2.71×10 ？3 </ sup> 到2.78×10 ？1 </ sup> 并且从-1.88×10 ？1 </ sup> 到3.97 mmol m ？2 </ sup> D. ？1 </ sup> 在硫酸盐 - 甲烷 - 过渡区（SMTZ）和沉积物海水界面。高甲烷助熔剂往往与结构特征有关，表明甲烷运输的强大结构控制。在大多数位点的SMTZ在SMTZ上的甲烷厌氧氧化消耗了升高的甲烷（＆ 50％）的显着部分，表明有效的生物过滤。气体组合物和同位素揭示了在主动边距和陆上泥火山的上坡中的微生物甲烷中的微生物甲烷中的主要甲烷的过渡。浅层深度的甲烷生产和消耗几乎抵消了一小部分残留的甲烷排放到海水中。助焊剂不平衡主要是由于甲烷生产较大的甲烷通过深微生物和产量的幅度为1512-43,096 TG MYR ？1 </ sup> 并且可能通过甲烷的封存成水合物形式和粘土吸收来占核算。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-23285/'>《Geochemistry, geophysics, geosystems》</a> <b style="margin: 0 2px;">|</b><span>2017年第8期</span><b style="margin: 0 2px;">|</b><span>共20页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chen Nai‐Chen&option=202" target="_blank" rel="nofollow">Chen Nai‐Chen;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Tsanyao Frank&option=202" target="_blank" rel="nofollow">Yang Tsanyao Frank;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Hong Wei‐Li&option=202" target="_blank" rel="nofollow">Hong Wei‐Li;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chen Hsuan‐Wen&option=202" target="_blank" rel="nofollow">Chen Hsuan‐Wen;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chen Hsiao‐Chi&option=202" target="_blank" rel="nofollow">Chen Hsiao‐Chi;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Hu Ching‐Yi&option=202" target="_blank" rel="nofollow">Hu Ching‐Yi;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Huang Yu‐Chun&option=202" target="_blank" rel="nofollow">Huang Yu‐Chun;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lin Saulwood&option=202" target="_blank" rel="nofollow">Lin Saulwood;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lin Li‐Hung&option=202" target="_blank" rel="nofollow">Lin Li‐Hung;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Su Chih‐Chieh&option=202" target="_blank" rel="nofollow">Su Chih‐Chieh;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liao Wei‐Zhi&option=202" target="_blank" rel="nofollow">Liao Wei‐Zhi;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Sun Chih‐Hsien&option=202" target="_blank" rel="nofollow">Sun Chih‐Hsien;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Pei‐Ling&option=202" target="_blank" rel="nofollow">Wang Pei‐Ling;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Tao&option=202" target="_blank" rel="nofollow">Yang Tao;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jiang Shao‐Yong&option=202" target="_blank" rel="nofollow">Jiang Shao‐Yong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Char‐Shine&option=202" target="_blank" rel="nofollow">Liu Char‐Shine;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Yunshuen&option=202" target="_blank" rel="nofollow">Wang Yunshuen;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chung San‐Hsiung&option=202" target="_blank" rel="nofollow">Chung San‐Hsiung;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of GeosciencesNational Taiwan UniversityTaipei Taiwan;</p> <p>Department of GeosciencesNational Taiwan UniversityTaipei Taiwan;</p> <p>Department of GeosciencesNational Taiwan UniversityTaipei Taiwan;</p> <p>Department of GeosciencesNational Taiwan UniversityTaipei Taiwan;</p> <p>Department of GeosciencesNational Taiwan UniversityTaipei Taiwan;</p> <p>Department of GeosciencesNational Taiwan UniversityTaipei Taiwan;</p> <p>Department of GeosciencesNational Taiwan UniversityTaipei Taiwan;</p> <p>Institute of Oceanography National Taiwan UniversityTaipei Taiwan;</p> <p>Department of GeosciencesNational Taiwan UniversityTaipei Taiwan;</p> <p>Institute of Oceanography National Taiwan UniversityTaipei Taiwan;</p> <p>Institute of Oceanography National Taiwan UniversityTaipei Taiwan;</p> <p>Exploration and Production Research Institute CPC CorporationMiaoli Taiwan;</p> <p>Institute of Oceanography National Taiwan UniversityTaipei Taiwan;</p> <p>State Key Laboratory for Mineral Deposits Research Department of Earth SciencesNanjing UniversityNanjing China;</p> <p>State Key Laboratory for Mineral Deposits Research Department of Earth SciencesNanjing UniversityNanjing China;</p> <p>Institute of Oceanography National Taiwan UniversityTaipei Taiwan;</p> <p>Central Geological Survey MOEATaipei Taiwan;</p> <p>Central Geological Survey MOEATaipei Taiwan;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/163.html" title="地球物理学">地球物理学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=thermal maturation&option=203" rel="nofollow">thermal maturation;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=methanogenesis&option=203" rel="nofollow">methanogenesis;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=anaerobic methanotrophy&option=203" rel="nofollow">anaerobic methanotrophy;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=methane efflux&option=203" rel="nofollow">methane efflux;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=subduction&option=203" rel="nofollow">subduction;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Taiwan&option=203" rel="nofollow">Taiwan;</a> </p> <div class="translation"> 机译：热成熟;甲烷化;厌氧甲基萎缩;甲烷流出;俯冲;台湾; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. 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C.&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Speed, R. C. </a> <span>1987</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：巴巴多斯自治棱镜中的深层天然气：来源，迁移，探测：最终报告。</span> </p> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/academic-journal-cn_hebei-chemical-industry_thesis/0201246761796.html">二氯甲烷的生产及消费</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=李伟&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 李伟</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=李晓燕&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,李晓燕</a> <span> <a href="/journal-cn-9134/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 河北化工 </a> </span> <span> . 1997</span><span>,第004期</span> </span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/academic-journal-cn_youth-society-on_thesis/0201267901110.html">从奢侈品看中国人的“面子”消费以库利“镜中自我”和布希亚消费理论分析</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=肖丹&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 肖丹</a> <span> <a href="/journal-cn-52208/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 青年与社会：上 </a> </span> <span> . 2015</span><span>,第007期</span> </span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/academic-journal-cn_journal-china-west-normal-university-philosophy-social-sciences_thesis/0201227470114.html">符号之镜中的消费异化——鲍德里亚《消费社会》解读</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=黄波&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 黄波</a> <span> <a href="/journal-cn-1466/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 西华师范大学学报（哲学社会科学版） </a> </span> <span> . 2007</span><span>,第006期</span> </span> </div> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/academic-journal-cn_chinese-population-resources-environment_thesis/0201292546830.html">我国工业重心迁移、生产与消费分离及其环境效应研究</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=黄乐文&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 黄乐文</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=钱曦&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,钱曦</a> <span> <a href="/journal-cn-51605/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 中国人口·资源与环境 </a> </span> <span> . 2011</span><span>,第S2期</span> </span> </div> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/academic-journal-cn_china-chlor-alkali_thesis/0201249159147.html">甲烷热氯化吸附分离组合工艺生产二氯甲烷、三氯甲烷</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=杨峰&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 杨峰</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=文咏祥&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,文咏祥</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=韩向阳&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,韩向阳</a> <span> <a href="/journal-cn-9255/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 中国氯碱 </a> </span> <span> . 2001</span><span>,第002期</span> </span> </div> </li> <li> <div> <b>6. </b><a class="enjiyixqcontent" href="/academic-conference-cn_meeting-40724_thesis/020222443157.html">刺竹林生长于台湾西南部恶地土壤对细菌族群之影响</a> <b>[C]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lin Yude&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . Lin Yude</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=林育德&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,林育德</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Huang Yuxuan&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,Huang Yuxuan</a> <span> <a href="/conference-cn-40724/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 中国土壤学会第十三次全国会员代表大会暨第十一届海峡两岸土壤肥料学术交流研讨会 </a> <span> <span> . 2016</span> </span> </div> </li> <li> <div> <b>7. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020311829659.html">兴义市西南部喀斯特地区土壤砷的空间分布及迁移富集特征</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=汪花&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 汪花</a> <span> . 2019</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/06120104592735.html">扬声器棱边,其发泡成型方法,生产扬声器棱边的装置和系统以及包括该棱边的扬声器</a> <b>[P]</b> . <span> 中国专利： CN1394456A </span> <span> . 2003-01-29</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/061201687381.html">二丁氧基甲烷、二乙氧基甲烷、二丙氧基甲烷或二戊氧基甲烷的生产方法</a> <b>[P]</b> . <span> 中国专利： CN103965029B </span> <span> . 2015.06.24</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130416489453.html">Producing methane from biomass, comprises producing acidified biomass, and consuming acidified biomass to obtain methane, in which acidified biomass is temporarily stored after its production and before its consumption</a> <b>[P]</b> . <span> 外国专利：  DE102013101882A1 </span> <span> . 2014-08-28</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：由生物质生产甲烷，包括生产酸化的生物质，以及消耗酸化的生物质以获得甲烷，其中酸化的生物质在其生产之后和消耗之前被暂时存储。 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130416518350.html">Methane supply system for diesel engine, sets consumption ratio of fuel to be specific percent of methane and preset percent of diesel per kilometer and introduces methane on aspiration battery</a> <b>[P]</b> . <span> 外国专利：  DE102012025594A1 </span> <span> . 2014-06-26</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：柴油发动机的甲烷供应系统，将燃料的消耗比设置为每公里甲烷的特定百分比和预设的柴油百分比，并将甲烷引入吸气电池 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130423668418.html">Production manner of the prism, being production manner of the prism and the prism which</a> <b>[P]</b> . <span> 外国专利：  JP4860268B2 </span> <span> . 2012-01-25</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：棱镜的生产方式，是棱镜的生产方式和 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704023360804','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div class="journalsub-pop-up" style="display: none"> <div class="journal-sub"> <h2>期刊订阅</h2> <img src="https://cdn.zhangqiaokeyan.com/img/loginclose.png" alt="关闭" onclick="$('.journalsub-pop-up').hide()"> <p class="pardon">抱歉，该期刊暂不可订阅，敬请期待！</p> <p 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