Highly Efficient and Selective Transformations of Glycerol Using Reusable Heterogeneous Catalysts

Tomoo Mizugaki; Racha Arundhathi; Takato Mitsudome

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Highly Efficient and Selective Transformations of Glycerol Using Reusable Heterogeneous Catalysts

机译：使用可重复使用的多相催化剂高效和选择性地转化甘油

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摘要

The highly efficient and selective transformations of glycerol to valuable compounds using reusable heterogeneous catalysts are demonstrated. Lanthanum cationexchanged montmorillonite shows high activity for the selective synthesis of diacetylglycerols through acetylation with acetic acid. Furthermore, the diacetylglycerols obtained can be subsequently oxidized into 1,3-diacetoxyacetone under air using an AlOx-embedded copper nanoparticle catalyst.

机译：证明了使用可重复使用的多相催化剂将甘油高效地选择性转化为有价值的化合物。镧阳离子交换蒙脱土对通过乙酸乙酰化选择性合成二乙酰甘油具有很高的活性。此外，所获得的二乙酰基甘油可随后在空气中使用嵌入AlOx的铜纳米粒子催化剂氧化为1,3-二乙酰氧基丙酮。

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《ACS Sustainable Chemistry & Engineering》 |2014年第4期|共5页
作者
Tomoo Mizugaki; Racha Arundhathi; Takato Mitsudome;
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正文语种 eng
中图分类化学工业;
关键词
Glycerol; Acetylglycerols; Lanthanum-exchanged montmorillonite; Copper nanoparticles; One-pot reaction;

机译：甘油;乙酰甘油;镧交换蒙脱石;铜纳米颗粒;一锅法反应;

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1. Highly Efficient and Selective Transformations of Glycerol Using Reusable Heterogeneous Catalysts [J] . Tomoo Mizugaki, Racha Arundhathi, Takato Mitsudome ACS Sustainable Chemistry & Engineering . 2014,第4期

机译：使用可重复使用的多相催化剂高效和选择性地转化甘油
2. Natural phosphate as new, highly efficient and reusable heterogeneous catalyst for the selective preparation of beta-enaminoesters under solvent-free conditions [J] . Mohamed Anouar Harrad, Issam Houssini, Brahim Boualy, Chemistry and Materials Research . 2014,第3期

机译：天然磷酸盐作为一种新型，高效且可重复使用的多相催化剂，可在无溶剂条件下选择性制备β-烯胺酯
3. Preparation and characterization of multi-walled carbon nanotubes (MWCNTs),functionalized with phosphonic acid (MWCNTs-C-PO_3H_2) and its application as a novel,efficient, heterogeneous,highly selective and reusable catalyst for acetylation of alcohols,phenols,aromatic amines,and thiols [J] . Farzaneh Dehghani, Ali Reza Sardarian, Mohammad Mehdi Doroodmand Journal of the Iranian Chemical Society . 2014,第3期

机译：用膦酸官能化的多壁碳纳米管（MWCNTs-C-PO_3H_2）的制备，表征及其作为新型，高效，多相，高选择性和可重复使用的醇，酚，芳胺乙酰化催化剂的应用和硫醇
4. Green synthesis of platinum/gold bimetallic nanoparticles supported onto hydrotalcite surface as heterogeneous catalyst for selective oxidation of glycerol [C] . Duangta Tongsakul, Chuchaat Thammacharoen Sanong Ekgasit, Sensor Research Unit AIChE annual meeting . 2011

机译：绿色合成负载水滑石表面的铂/金双金属纳米颗粒作为甘油选择性氧化的非均相催化剂
5. Efficient and selective multifunctional nanoporous and heterogeneous catalysts: Novel synthetic methods, characterizations and applications. [D] . Sharma, Krishna Kant. 2010

机译：高效，选择性的多功能纳米多孔和非均相催化剂：新型合成方法，表征和应用。
6. Efficient and selective chemical transformations under flow conditions: The combination of supported catalysts and supercritical fluids [O] . M Isabel Burguete, Eduardo García-Verdugo, Santiago V Luis 2011

机译：流动条件下的高效选择性化学转化：负载型催化剂和超临界流体的结合
7. B2O3/Al2O3 as a new, highly efficient and reusable heterogeneous catalyst for the selective synthesis of β-enamino ketones and esters under solvent-free conditions [O] . Jiu-Xi Chen, Chang-Fu Zhang, Wen-Xia Gao, 2010

机译：B2O3 / Al 2O3作为一种新的高效可重复使用的非均相催化剂，用于在无溶剂条件下选择性合成β-烯氨基酮和酯

Highly Efficient and Selective Transformations of Glycerol Using Reusable Heterogeneous Catalysts

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