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Evolution of Chain Length Distribution and Microstructure of Macromolecules in Irreversible Copolymerization Proceeding with Segmental Exchange Investigated with a New Monte Carlo Algorithm

机译：一种新的蒙特卡罗算法对不可逆共聚进展中不可逆共聚进展中的长度分布和微观结构的演变

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Abstract >A process of irreversible copolymerization with segmental exchange reactions is simulated using a Monte Carlo algorithm. The terminal (dyad) model is assumed for eight considered reactions: propagations and attacks of active centers on monomeric units in chains with subsequent chain scissions. It is established that microstructure of macromolecules at any given moment depends on the values of reaction rate constants and evolves from the beginning one, defined mainly by propagation rates, to the final one, determined by chain transfer rates. Dispersity and randomization degree of unit sequences in macromolecules can change nonmonotonically with progress of the process. Equilibration of the microstructure needs usually significantly longer time than needed for attaining the equilibrium chain lengths distribution. The proposed new Monte Carlo algorithm allows to more efficiently investigate the studied process. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> 使用蒙特卡罗算法模拟与节段性交换反应不可逆共聚的过程。假设终端（Dyad）模型用于八次被认为是反应的：在链条中的单体单元上的活性中心的传播和攻击具有随后的链缩写的链条中的单体单元。建立在任何给定时刻的大分子微观结构取决于反应速度常数的值，并从主要通过传播速率定义的开始的值，以通过链转移率确定。大分子中单位序列的分散性和随机化程度可以随着该方法的进展而非语文学改变。微观结构的平衡通常需要比获得平衡链长度分布所需的时间明显更长。所提出的新蒙特卡罗算法允许更有效地研究研究的过程。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-24304/'>《Macromolecular theory and simulations》</a> <b style="margin: 0 2px;">|</b><span>2018年第5期</span><b style="margin: 0 2px;">|</b><span>共12页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Szymanski Ryszard&option=202" target="_blank" rel="nofollow">Szymanski Ryszard;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Sosnowski Stanislaw&option=202" target="_blank" rel="nofollow">Sosnowski Stanislaw;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Center of Molecular and Macromolecular StudiesSienkiewicza 112 Lodz 90‐363 Poland;</p> <p>Center of Molecular and Macromolecular StudiesSienkiewicza 112 Lodz 90‐363 Poland;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1185.html" title="高分子化学（高聚物）">高分子化学（高聚物）;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=copolymerization&option=203" rel="nofollow">copolymerization;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=microstructure&option=203" rel="nofollow">microstructure;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Monte Carlo simulation&option=203" rel="nofollow">Monte Carlo simulation;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=ring‐opening polymerization&option=203" rel="nofollow">ring‐opening polymerization;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=segmental exchange&option=203" rel="nofollow">segmental exchange;</a> </p> <div class="translation"> 机译：共聚;微观结构;蒙特卡罗模拟;开环聚合;节段交换; 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