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Phase Diagram of Hierarchical Structures Formed from A(BC) ₂2 B Multiblock Copolymers

机译：由（BC）形成的分层结构的相图 _{2 2 B多嵌段共聚物}

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Abstract > Due to more than two length scales properties, hierarchical structures, which can combine several properties and respond to multi external conditions, have attracted the continuing attention over the past decades. The corresponding phase diagram of different hierarchical structures is crucially important for the observation of these morphologies. In this paper, the phase diagram of these hierarchical structures in A(BC) <sub>2</sub> B multiblock copolymer is calculated, including hierarchical lamellae, hierarchical cylinder, and hierarchical sphere (also termed as onion‐like sphere), leading to the identification of the correspondingly stable region. Interestingly, as end block f <sub>A</sub> increases, the hierarchical phase transition sequence at low χ <sub>BC</sub> N , which is D→S <sub>3</sub> →C <sub>3</sub> →L <sub>5</sub> →L <sub>3</sub> →C→S→D , is different from that at larger χ <sub>BC</sub> N ( L <sub>B/C</sub> →S <sub>3</sub> →L <sub>5</sub> →L <sub>3</sub> →C→S→D ), where lamella formed by B and C blocks is the dominated phase at small A volume fraction. In addition, the perpendicular lamellae at much higher χ <sub>BC</sub> N are observed, which are consistent with the experimental observation of perpendicular lamellae. Importantly, this phase diagram has great guidance for the experimental observation of different hierarchical nanostructures. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 由于两个以上的长度尺度属性，分层结构可以组合几个属性并响应多个外部条件，在过去几十年中引起了继续关注。不同层次结构的相应相图对于观察这些形态而言是至关重要的。在本文中，在（BC）中这些分层结构的相图 <sub> 2 </ sub> 计算多嵌段共聚物，包括分层薄片，分层圆柱和分级球（也称为洋葱状球体），导致相应稳定区域的识别。有趣的是，作为结束块 f </ i> <sub> a </ sub> 增加，低χ的分层期转换序列 <sub> bc </ sub> n </ i> ，这是 d→s </ i> <sub> 3 </ sub> →c </ i> <sub> 3 </ sub> →l </ i> <sub> 5 </ sub> →l </ i> <sub> 3 </ sub> →c→s→d </ i> ，与较大的χ不同 <sub> bc </ sub> n </ i> （ l </ i> <sub> b / c </ sub> →s </ i> <sub> 3 </ sub> →l </ i> <sub> 5 </ sub> →l </ i> <sub> 3 </ sub> →c→s→d </ i> ），由B和C嵌段形成的薄片是小于体积分数的占主导地相。此外，垂直薄片高得多 <sub> bc </ sub> n </ i> 观察到，与垂直薄片的实验观察一致。重要的是，该相图具有对不同分层纳米结构的实验观察的巨大指导。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-24304/'>《Macromolecular theory and simulations》</a> <b style="margin: 0 2px;">|</b><span>2019年第3期</span><b style="margin: 0 2px;">|</b><span>共8页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Hu Weiguo&option=202" target="_blank" rel="nofollow">Hu Weiguo;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Shao Zhanwei&option=202" target="_blank" rel="nofollow">Shao Zhanwei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Di&option=202" target="_blank" rel="nofollow">Zhang Di;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xu Yuci&option=202" target="_blank" rel="nofollow">Xu Yuci;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Faculty of Materials Science and Chemical EngineeringNingbo UniversityNingbo Zhejiang 315211 China;</p> <p>Faculty of Materials Science and Chemical EngineeringNingbo UniversityNingbo Zhejiang 315211 China;</p> <p>Faculty of Materials Science and Chemical EngineeringNingbo UniversityNingbo Zhejiang 315211 China;</p> <p>Faculty of Materials Science and Chemical EngineeringNingbo UniversityNingbo Zhejiang 315211 China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1185.html" title="高分子化学（高聚物）">高分子化学（高聚物）;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hierarchical structures&option=203" rel="nofollow">hierarchical structures;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=multiblock copolymer&option=203" rel="nofollow">multiblock copolymer;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=phase diagram&option=203" rel="nofollow">phase diagram;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=self‐consistent field theory&option=203" rel="nofollow">self‐consistent field theory;</a> </p> <div class="translation"> 机译：分层结构;多嵌段共聚物;相图;自我持续的场理论; 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href="/academic-conference-cn_meeting-8603_thesis/020222174078.html">刚棒中心含有乙基的线团-刚棒-线团三嵌段共聚物自组装形成三维六方纳米结构</a> <b>[C]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhuoshi Wang&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . Zhuoshi Wang</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=王卓识&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,王卓识</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lirong Tian&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,Lirong Tian</a> <span> <a href="/conference-cn-8603/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 2012年两岸三地高分子液晶态与超分子有序结构学术会议暨第十二届全国高分子液晶态与超分子有序结构学术论文报告 </a> <span> <span> . 2012</span> </span> </div> </li> <li> <div> <b>7. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020316008022.html">多嵌段共聚物嵌套结构的形成</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=胡卫国&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 胡卫国</a> <span> . 2019</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/06120108327207.html">用于对使用基于苯乙烯和基于甲基丙烯酸甲酯的未经结构化的嵌段共聚物的嵌段共聚物膜进行纳米结构化的工艺、以及经纳米结构化的嵌段共聚物膜</a> <b>[P]</b> . <span> 中国专利： CN105829239A </span> <span> . 2016-08-03</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/061204392162.html">由嵌段共聚物形成的囊泡、以及嵌段共聚物</a> <b>[P]</b> . <span> 中国专利： CN107667133B </span> <span> . 2021.05.07</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130501381638.html">RESIN COMPOSITION FOR FORMING PHASE-SEPARATED STRUCTURE, METHOD FOR PRODUCING STRUCTURE INCLUDING PHASE-SEPARATED STRUCTURE, AND BLOCK COPOLYMER</a> <b>[P]</b> . <span> 外国专利：  US2022017741A1 </span> <span> . 2022-01-20</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：用于形成相分离结构的树脂组合物，制备结构的方法，包括相分离的结构和嵌段共聚物 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" 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Phase Diagram of Hierarchical Structures Formed from A(BC) 22 B Multiblock Copolymers

摘要

Phase Diagram of Hierarchical Structures Formed from A(BC) ₂2 B Multiblock Copolymers