Enhanced NH <sub xmlns='http://www.wiley.com/namespaces/wiley'>3</sub>3 capture by imidazolium‐based protic ionic liquids with different anions and cation substituents

Shang Dawei; Bai Lu; Zeng Shaojuan; Dong Haifeng; Gao Hongshuai; Zhang Xiangping; Zhang Suojiang

摘要

Abstract <section xml:id="jctb5467-sec-0001" numbered="no"> <title type="main">BACKGROUND > Ionic liquids have become potential absorbents to treat exhausted gases containing NH <sub>3</sub> , which threatens the living environment of human beings. </section> <section xml:id="jctb5467-sec-0002" numbered="no"> <title type="main">RESULTS > In this study, 10 kinds of protic and conventional ILs were synthesized and characterized and their densities, viscosities and thermal decomposition temperatures measured. The NH <sub>3</sub> solubility in ILs from the vapor liquid equilibrium (VLE) experiments revealed that the chain length of cations had little influence on the NH <sub>3</sub> solubility of the protic ILs because of the high NH <sub>3</sub> capacities in protic ILs resulting from protic hydrogen atom compared with conventional ILs. The 2‐H atom on the cation influenced the NH <sub>3</sub> solubility in both protic and conventional ILs with different trends as the pressure was increased. Considering the effect of anions with the same cation [Bim] + , the order of NH <sub>3</sub> solubility in protic ILs was [Bim][NTf <sub>2</sub> ] [Bim][SCN] [Bim][NO <sub>3</sub> ]. Dynamic absorption of NH <sub>3</sub> in [Eim][NTf <sub>2</sub> ] preliminarily revealed that the absorption was fast under ambient pressure and through 5 cycles of absorption and desorption, the NH <sub>3</sub> absorption ability remained stable. </section> <section x </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract XMLNS =“http://www.wiley.com/namespaces/wiley”type =“main”xml：lang =“en”> <title type =“main”>抽象</ title> <section XML：ID =“JCTB5467-SEC-0001”编号=“否”> <标题类型=“main”>背景</标题> >离子液体已成为治疗含有NH <sub> 3 </ sub>的耗尽气体的潜在吸收剂，威胁着人类的生活环境。 </ p> </ section> <section XML：ID =“JCTB5467-SEC-0002”编号=“否”> <标题类型=“main”>结果</ title> >在本研究中，10种合成特征和常规ILS，其特征及其密度，测量的密度，粘度和热分解温度。来自蒸汽液体平衡（VLE）实验的ILS中的NH <sub> 3 /亚>溶解度显示，阳离子的链长对NH <Sub> 3 </ sub>溶解度的影响很小与常规IL相比，由质子氢原子得到的质子ILS中的高NH <亚> 3 </亚>容量。在阳离子上的2-H原子影响了NH <Sub> 3 </ sub>在具有不同趋势的质子和常规IL中的NH <sub>溶解度随着压力而增加。考虑到阴离子与相同阳离子的效果[BIM] + </ sup>，NH <sub> 3 </ sub>在质子ILs中的溶解度的顺序为[BIM] [NTF <sub> 2 </ sub >]＆ [BIM] [SCN]＆GT; [BIM] [没有<sub> 3 </ sub>]。 NH <Sub> 3 </ sub>在[EIM] [NTF <sub> 2 </ sub>]中的动态吸收初步揭示了在环境压力下的吸收和通过5个吸收和解吸，NH <sub > 3 </ sub>吸收能力保持稳定。 </ p> </ section> <section x </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-33908/'>《Journal of Chemical Technology & Biotechnology》</a> <b style="margin: 0 2px;">|</b><span>2018年第5期</span><b style="margin: 0 2px;">|</b><span>共9页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Shang Dawei&option=202" target="_blank" rel="nofollow">Shang Dawei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Bai Lu&option=202" target="_blank" rel="nofollow">Bai Lu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zeng Shaojuan&option=202" target="_blank" rel="nofollow">Zeng Shaojuan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Dong Haifeng&option=202" target="_blank" rel="nofollow">Dong Haifeng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Gao Hongshuai&option=202" target="_blank" rel="nofollow">Gao Hongshuai;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Xiangping&option=202" target="_blank" rel="nofollow">Zhang Xiangping;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Suojiang&option=202" target="_blank" rel="nofollow">Zhang Suojiang;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Key Laboratory of Green Process and Engineering State Key Laboratory of Multiphase Complex System Beijing Key Laboratory of Ionic Liquids Clean Process Institute of Process EngineeringChinese Academy of SciencesBeijing China;</p> <p>Key Laboratory of Green Process and Engineering State Key Laboratory of Multiphase Complex System Beijing Key Laboratory of Ionic Liquids Clean Process Institute of Process EngineeringChinese Academy of SciencesBeijing China;</p> <p>Key Laboratory of Green Process and Engineering State Key Laboratory of Multiphase Complex System Beijing Key Laboratory of Ionic Liquids Clean Process Institute of Process EngineeringChinese Academy of SciencesBeijing China;</p> <p>Key Laboratory of Green Process and Engineering State Key Laboratory of Multiphase Complex System Beijing Key Laboratory of Ionic Liquids Clean Process Institute of Process EngineeringChinese Academy of SciencesBeijing China;</p> <p>Key Laboratory of Green Process and Engineering State Key Laboratory of Multiphase Complex System Beijing Key Laboratory of Ionic Liquids Clean Process Institute of Process EngineeringChinese Academy of SciencesBeijing China;</p> <p>Key Laboratory of Green Process and Engineering State Key Laboratory of Multiphase Complex System Beijing Key Laboratory of Ionic Liquids Clean Process Institute of Process EngineeringChinese Academy of SciencesBeijing China;</p> <p>Key Laboratory of Green Process and Engineering State Key Laboratory of Multiphase Complex System Beijing Key Laboratory of Ionic Liquids Clean Process Institute of Process EngineeringChinese Academy of SciencesBeijing China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/180.html" title="生物工程学（生物技术）">生物工程学（生物技术）;</a><a href="https://www.zhangqiaokeyan.com/clc/20827.html" title="生物化学过程">生物化学过程;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=NH 3 solubility&option=203" rel="nofollow">NH 3 solubility;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=protic and conventional ILs&option=203" rel="nofollow">protic and conventional ILs;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=vapor liquid equilibrium&option=203" rel="nofollow">vapor liquid equilibrium;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=dynamic absorption&option=203" rel="nofollow">dynamic absorption;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=influence of ILs structures&option=203" rel="nofollow">influence of ILs structures;</a> </p> <div class="translation"> 机译：NH 3溶解度;质子和常规ILS;蒸汽液体平衡;动态吸收;ILS结构的影响; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704025422832.html">Enhanced NH <sub xmlns="http://www.wiley.com/namespaces/wiley">3</sub>3 capture by imidazolium‐based protic ionic liquids with different anions and cation substituents</a> <b>[J]</b> . <span> 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By Iwao Ojima (Editor)Wiley-VCH: New York (http://www.wiley.com/). 2000. Pages: XIV 864 Pages Hardcover. Price: 169.- Euro / 330.54 DM / 294.- SFR. 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class="enjiyixqcontent" href="/patent-detail/06130434124083.html">Solution system based on molten ionic liquid e.g. imidazolium salt for dissolving carbohydrate e.g. starch, cellulose or derivative and regeneration e.g. for fiber production also contains water and/or other protic solvent</a> <b>[P]</b> . <span> 外国专利：  DE102005062608A1 </span> <span> . 2007-07-05</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：基于熔融离子液体的溶液系统用于溶解碳水化合物的咪唑盐，例如淀粉，纤维素或衍生物和再生例如纤维生产中还含有水和/或其他质子溶剂 </span> </p> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130409273039.html">Protic ammonium cation ionic liquids (3-hydroxypropyl)dimethyl-ammonium and anion the herbicide and the method for their preparation</a> <b>[P]</b> . <span> 外国专利：  PL226687B1 </span> <span> . 2017-08-31</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：质子铵阳离子离子液体（3-羟丙基）二甲基铵和阴离子除草剂及其制备方法 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704025422832','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div class="journalsub-pop-up" style="display: none"> <div class="journal-sub"> <h2>期刊订阅</h2> <img src="https://cdn.zhangqiaokeyan.com/img/loginclose.png" alt="关闭" onclick="$('.journalsub-pop-up').hide()"> <p class="pardon">抱歉，该期刊暂不可订阅，敬请期待！</p> <p class="current">目前支持订阅全部北京大学中文核心（2020）期刊目录。</p> <div 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Enhanced NH 33 capture by imidazolium‐based protic ionic liquids with different anions and cation substituents

摘要

Enhanced NH ₃3 capture by imidazolium‐based protic ionic liquids with different anions and cation substituents