Electrochemical recovery of copper complexed by DTPA and C <sub xmlns='http://www.wiley.com/namespaces/wiley'>12</sub>12 ‐DTPA from aqueous solution using a membrane cell

Eivazihollagh Alireza; B?ckstr?m Joakim; Norgren Magnus; Edlund H?kan

摘要

Abstract <section xml:id="jctb5510-sec-0001" numbered="no"> <title type="main">BACKGROUND > The electrochemical recovery of copper from diethylenetriaminepentaacetic acid (DTPA) and C <sub>12</sub> –DTPA (a surface‐active derivative of DTPA) complex solutions was investigated in a membrane flow cell. Electrolysis time, solution flow rate, applied current density, and solution pH were evaluated. </section> <section xml:id="jctb5510-sec-0002" numbered="no"> <title type="main">RESULTS > The chelating surfactant C <sub>12</sub> ‐DTPA can promote the kinetics of copper electrodeposition more than DTPA depending on the experimental conditions. At a current density of 30 A m –2 , a solution flow rate of 0.6 L min –1 , and pH 10 after 180 min treatment, the copper recovery and current efficiency were 50% and 43.3%, respectively, in the Cu(II)‐DTPA system and about 65% and 53.6%, respectively, in the Cu(II)‐C <sub>12</sub> ‐DTPA system. The differences in the amount of recovery could be explained in terms of differences in the diffusion of copper complexes with DTPA and C <sub>12</sub> ‐DTPA to the cathode, as well as their solution behavior and pH‐dependent conditional stability constants (log <sub>10</sub> <fi>K</fi> ' <sub>CuDTPA</sub> 3‐ ). </section> <section xml:id="jctb5510-sec-0003" numbered="no"> <title type="main">CONCLUSION > Electrochemical methods could be effectively combined with foam flotation for the chelating surfactant C </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract XMLNS =“http://www.wiley.com/namespaces/wiley”type =“main”xml：lang =“en”> <title type =“main”>抽象</ title> <section XML：ID =“JCTB5510-SEC-0001”编号=“否”> <标题类型=“main”>背景</标题> >铜的电化学回收来自二亚乙基三胺丙酮酸（DTPA）和C <SUB> 12 </ sub >在膜流动细胞中研究了-DTPA（DTPA的表面活性衍生物）复合溶液。评估电解时间，溶液流速，施加电流密度和溶液pH。 </ p> </ section> <section XML：ID =“JCTB5510-SEC-0002”编号=“否”> <标题类型=“main”>结果</ title> >螯合表面活性剂C <sub>根据实验条件，12 </ sub> -DTPA可以促进铜电沉积的动力学超过DTPA。在电流密度为30 A m -2 / sop>，溶液流速为0.6 l min -1 -1 / sop>，并在180分钟处理后pH 10，铜回收和电流效率分别在Cu（II）-DTPA系统中分别为50％和43.3％，分别在Cu（II）-C -C <Sub> 12 </ sub> -DTPA系统中分别为约65％和53.6％。可以在铜复合物扩散与DTPA和C <sub> 12 -12-DTPA的差异方面解释恢复量的差异，以及它们的溶液行为和pH依赖性条件稳定性常量（log <sub> 10 </ sub> <fi> k </ fi>'<sub> cudtpa </ sub> 3 - </ sup>）。 </ p> </段> <部分XML：ID =“JCTB5510-SEC-0003”编号=“否”> <标题类型=“MAIN”>结论</标题> <P>电化学方法可以有效地结合使用螯合表面活性剂C的泡沫浮选C. </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-33908/'>《Journal of Chemical Technology & Biotechnology》</a> <b style="margin: 0 2px;">|</b><span>2018年第5期</span><b style="margin: 0 2px;">|</b><span>共11页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Eivazihollagh Alireza&option=202" target="_blank" rel="nofollow">Eivazihollagh Alireza;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=B?ckstr?m Joakim&option=202" target="_blank" rel="nofollow">B?ckstr?m Joakim;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Norgren Magnus&option=202" target="_blank" rel="nofollow">Norgren Magnus;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Edlund H?kan&option=202" target="_blank" rel="nofollow">Edlund H?kan;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>FSCN Surface and Colloid EngineeringMid Sweden UniversitySundsvall Sweden;</p> <p>Department of Natural SciencesMid Sweden UniversitySundsvall Sweden;</p> <p>FSCN Surface and Colloid EngineeringMid Sweden UniversitySundsvall Sweden;</p> <p>FSCN Surface and Colloid EngineeringMid Sweden UniversitySundsvall Sweden;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/180.html" title="生物工程学（生物技术）">生物工程学（生物技术）;</a><a href="https://www.zhangqiaokeyan.com/clc/20827.html" title="生物化学过程">生物化学过程;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Electrochemistry&option=203" rel="nofollow">Electrochemistry;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Heavy Metals&option=203" rel="nofollow">Heavy Metals;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Recycling&option=203" rel="nofollow">Recycling;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Waste‐Water&option=203" rel="nofollow">Waste‐Water;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Hydrometallurgy&option=203" rel="nofollow">Hydrometallurgy;</a> </p> <div class="translation"> 机译：电化学;重金属;回收;废水;潮湿冶金; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> 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translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：使用电化学池从水溶液中回收金，银和铜的电化学回收和萃取工艺 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130437808040.html">gold, silver and copper electrochemical recovery and extraction process from aqueous solutions using an electrochemical cell</a> <b>[P]</b> . <span> 外国专利：  BR0303985A </span> <span> . 2006-04-25</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：使用电化学池从水溶液中回收金，银和铜的电化学回收和萃取工艺 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130446840864.html">Process for preparing a supported Catalyst, Palladium, Gold and copper, Where The Catalyst is prepared by impregnating a porous Carrier with an aqueous solution of a water-soluble Salt of palladium and Copper.Setting the palladium and copper, and then The Catalyst impregnated with a water-soluble Salt of Gold (Divisional Application 1210 - 98).</a> <b>[P]</b> . <span> 外国专利：  CL2001002468A1 </span> <span> . 2002-10-02</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：制备负载型催化剂，钯，金和铜的方法，其中催化剂是通过将多孔载体用钯和铜的水溶性盐的水溶液浸渍而制备的，将钯和铜定型，然后将催化剂浸渍水溶性金盐（分案申请号1210-98）。 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704025422848','4',7,2,1,'',this,24)" class="delivery" 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Electrochemical recovery of copper complexed by DTPA and C 1212 ‐DTPA from aqueous solution using a membrane cell

摘要

Electrochemical recovery of copper complexed by DTPA and C ₁₂12 ‐DTPA from aqueous solution using a membrane cell