Fullerene-Attached Polymeric Homogeneous/Heterogeneous Photoactivators for Visible-Light-Induced CuAAC Click Reactions

Taskin Omer S.; Yilmaz Gorkem; Yagci Yusuf

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Fullerene-Attached Polymeric Homogeneous/Heterogeneous Photoactivators for Visible-Light-Induced CuAAC Click Reactions

机译：富勒烯附着的聚合物均相/均相光活化剂，用于可见光诱导的CuAAC Click反应

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In this work, a visible-light -inducedcopper(I)-catalyzed azide alkyne cycloaddition (CuAAC) dick reaction via an electron transfer reaction employing fullerene (C-60) containing linear polystyrene and network polymer as homogeneous and heterogeneous activators, PS-C-60 and Gel-C-60, respectively, is described. Various low molar mass organic and polymeric azide and alkyne compounds are used to conduct the click reaction, and almost quantitative yields are attained. Compared to the bare C-60, the polymers with C-60, units exhibited a much higher promoting effect to catalyze CuAAC reactions.

机译：在这项工作中，通过电子转移反应，使用富勒烯（C-60）包含线性聚苯乙烯和网络聚合物作为均相和非均相活化剂，通过可见光诱导的铜（I）催化的叠氮化物炔烃环加成（CuAAC）迪克反应分别描述了-60和Gel-C-60。各种低摩尔质量的有机和聚合的叠氮化物和炔烃化合物可用于进行点击反应，并获得了几乎定量的产率。与裸露的C-60相比，具有C-60单元的聚合物表现出更高的催化CuAAC反应的促进作用。

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《ACS Macro Letters》 |2016年第1期|共5页
作者
Taskin Omer S.; Yilmaz Gorkem; Yagci Yusuf;
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1. Fullerene-Attached Polymeric Homogeneous/Heterogeneous Photoactivators for Visible-Light-Induced CuAAC Click Reactions [J] . Taskin Omer S., Yilmaz Gorkem, Yagci Yusuf ACS Macro Letters . 2016,第1期

机译：富勒烯附着的聚合物均相/均相光活化剂，用于可见光诱导的CuAAC Click反应
2. Polymer "Clicking" by CuAAC reactions [J] . Meldal M Macromolecular rapid communications: Publishing the newsletters of the European Polymer Federation . 2008,第12a13期

机译：聚合物通过CuAAC反应“点击”
3. The Clicked Pyridyl-Triazole Ligand: From Homogeneous to Robust, Eecyclable Heterogeneous Mono-and Polymetallic Palladium Catalysts for Efficient Suzuki-Miyaura, Sonogashira, and Heck Reactions [J] . Dong Wang, Dominique Denux, Jaime Ruiz Advanced synthesis & catalysis . 2013,第1期

机译：单击的吡啶基-三唑配体：从均相到稳健的，可回收的可杂环非均相单金属和多金属钯催化剂，可有效用于铃木-宫浦，Sonogashira和Heck反应
4. Photoinduced ATRP and CuAAC Click Reactions and Their Combinations for Macromolecular Syntheses [C] . Sean Doran, Eljesa Murtezi, Sajjad Dadashi-Silab American Chemical Society Division of Polymeric Materials Science and Engineering Conference . 2015

机译：Photo诱导ATRP和CUAAC点击反应及其组合用于大分子合成
5. Membrane reactors for the study of homogeneous and heterogeneous reactions using ceramic and ceramic/polymeric membranes. [D] . Zhu, Yifan. 1996

机译：膜反应器，用于研究使用陶瓷和陶瓷/聚合膜的均相和非均相反应。
6. Photo-Mediated Copper(I)-Catalyzed Azide-Alkyne Cycloaddition (CuAAC) Click Reactions for Forming Polymer Networks as Shape Memory Materials [O] . Matthew K. McBride, Tao Gong, Devatha P. Nair, -1

机译：光介导的铜（I）催化的叠氮化物-炔烃环加成（CuAAC）点击反应形成聚合物网络作为形状记忆材料
7. Berichtigung: Facile Synthesis of Sequence-Regulated Synthetic Polymers Using Orthogonal SuFEx and CuAAC Click Reactions [O] . Cangjie Yang, James P. Flynn, Jia Niu 2019

机译：Berichtigung：使用正交Sufex和Cuaac点击反应的序列调节合成聚合物的容易合成

Fullerene-Attached Polymeric Homogeneous/Heterogeneous Photoactivators for Visible-Light-Induced CuAAC Click Reactions

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