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Study on the coloring mechanism of the Ru celadon glaze in the Northern Song Dynasty

机译：北宋Ru Celadon Glaze釉料的着色机制研究

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摘要

The Ru kiln is one of the five most famous kilns in the Chinese Song Dynasty. To clarify the coloring mechanism of the Ru celadon glaze, the celadon samples from the Ru Guan kiln site of Qingliangsi were analyzed by spectrophotometer, X-ray fluorescence spectrum, Raman spectroscopy, scanning electron microscopy and X-ray photoelectron spectrum. The results indicated that the molar ratios of SiO2/Al2O3 and CaO/(CaO + Al2O3) affected the formation of micro-bubbles, anorthite crystals and phase separated structures. A large number of bubbles and anorthite crystals formed special glossiness and opacifying effect in the Ru celadon glaze. And then, dense phase separation droplets in the amorphous region were in short-range order, but their diameters (31-46 nm) were too small to form visible structural colors on glaze surfaces. Only "opal effect" was formed by the light scattering, which added the aesthetic feeling for the Ru celadon. Besides, the phase separation droplets intensified the segregation of iron, and thus deepened the chemical color and made the Ru celadon glaze appear green-blue. Due to the neutral to alkaline soil at the Ru Guan kiln site, the water in the soil and its corrosion on the Ru celadon glaze resulted in the formation of Si-OH bond.
机译：茹克恩是中国宋代五大窑之一。为了澄清Ru Celadon Glaze的着色机制，通过分光光度计，X射线荧光谱，拉曼光谱，扫描电子显微镜和X射线光电子谱分析清凉柱的Ru Guan Kiln位点的Celadon样本。结果表明，SiO 2 / Al 2 O 3和CaO /（CaO + Al2O3）的摩尔比对微泡，钙质晶体和相分离结构的形成影响。大量气泡和钙铜晶体在Ru Celadon Glaze中形成了特殊的光泽和透明度。然后，非晶区域中的致密相分离液滴以短距离顺序，但它们的直径（31-46nm）太小，不能在釉面上形成可见的结构颜色。只有“蛋白石效应”是由光散射形成的，这增加了Ru Celadon的美学感受。此外，相分离液滴加剧了铁的偏析，从而深化了化学色并使Ru Celadon釉面出现了绿色。由于Ru Guan Kiln位点的中性到碱土土壤，土壤中的水及其在Ru Celadon釉上的腐蚀导致了Si-OH键的形成。

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  • 来源
    《CERAMICS INTERNATIONAL》 |2020年第15期|共7页
  • 作者

    Shi Pei; Wang Fen; Zhang Biao; Luo Hongjie; Zhu Jianfeng; Fei Guiqiang;

  • 作者单位

    Shaanxi Univ Sci &

    Technol Shaanxi Key Lab Green Preparat &

    Functionalizat I Sch Mat Sci &

    Engn Xian 710021 Peoples R China;

    Shaanxi Univ Sci &

    Technol Shaanxi Key Lab Green Preparat &

    Functionalizat I Sch Mat Sci &

    Engn Xian 710021 Peoples R China;

    Shaanxi Univ Sci &

    Technol Shaanxi Key Lab Green Preparat &

    Functionalizat I Sch Mat Sci &

    Engn Xian 710021 Peoples R China;

    Shanghai Univ Res Inst Cultural Rel Shanghai 200444 Peoples R China;

    Shaanxi Univ Sci &

    Technol Shaanxi Key Lab Green Preparat &

    Functionalizat I Sch Mat Sci &

    Engn Xian 710021 Peoples R China;

    Shaanxi Univ Sci &

    Technol Coll Chem &

    Chem Engn Xian 710021 Peoples R China;

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  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类 陶瓷工业;硅酸盐工业;
  • 关键词

    Ru Guan kiln; Qingliangsi; Celadon glaze; Northern Song Dynasty; Coloring mechanism;

    机译：茹关窑;清凉山;青瓷釉;北宋;着色机制;

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