Fabrication of Holey Graphene: Catalytic Oxidation by Metalloporphyrin-Based Covalent Organic Framework Immobilized on Highly Ordered Pyrolytic Graphite

Wanji Seo; David L. White; Alexander Star

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Fabrication of Holey Graphene: Catalytic Oxidation by Metalloporphyrin-Based Covalent Organic Framework Immobilized on Highly Ordered Pyrolytic Graphite

机译：HOLENY石墨烯的制造：通过固定在高度有序的热解石墨上的金属卟啉的共价有机骨架催化氧化

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摘要

We report a facile chemical method for fabricating holey graphene by catalytic oxidation of highly ordered pyrolytic graphite (HOPG) using an Fe~(III) porphyrin complex-based covalent organic framework (COF) as a bifunctional surface catalyst-template. We demonstrate regular hole formation after oxidation with H_2O_2 and NaOCl, COF removal, and HOPG exfoliation.

机译：我们通过使用Fe〜（III）卟啉复合物的共价有机骨架（COF）作为双官能表面催化剂模板，通过催化氧化高度有序的热解石墨（HOPG）来报告一种用于制造多孔石墨烯的化学方法。我们展示氧化后常规孔形成，氧化H_2O_2和NAOCL，COF去除和HOPG去角质。

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《Chemistry: A European journal》 |2017年第24期|共6页
作者
Wanji Seo; David L. White; Alexander Star;
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作者单位

Department of Chemistry University of Pittsburgh Pittsburgh PA 15260 (USA);

Department of Chemistry University of Pittsburgh Pittsburgh PA 15260 (USA);

Department of Chemistry University of Pittsburgh Pittsburgh PA 15260 (USA);

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原文格式 PDF
正文语种 eng
中图分类应用化学;
关键词
catalytic oxidation; covalent organic frameworks; graphene; nanopatterning; surface catalysts;

机译：催化氧化;共价有机框架;石墨烯;纳米透明剂;表面催化剂;

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1. Fabrication of Holey Graphene: Catalytic Oxidation by Metalloporphyrin-Based Covalent Organic Framework Immobilized on Highly Ordered Pyrolytic Graphite [J] . Wanji Seo, David L. White, Alexander Star Chemistry: A European journal . 2017,第24期

机译：HOLENY石墨烯的制造：通过固定在高度有序的热解石墨上的金属卟啉的共价有机骨架催化氧化
2. Facile fabrication of magnetically recyclable metal-organic framework nanocomposites for highly efficient and selective catalytic oxidation of benzylic C-H bonds [J] . Yifa Chen, Xianqiang Huang, Xiao Feng, Chemical Communications . 2014,第61期

机译：轻松制造可磁循环利用的金属-有机骨架纳米复合材料，以高效且选择性地催化氧化苄基C-H键
3. Engineering 3D Ru/Graphene Aerogel Using Metal–Organic Frameworks: Capture and Highly Efficient Catalytic CO Oxidation at Room Temperature [J] . Jiafu Qu, Dongyun Chen, Najun Li, Small . 2018,第16期

机译：使用金属有机框架的工程3D Ru /石墨烯气凝胶：室温捕获和高效催化作用CO氧化
4. Conductivity of Graphene-Like Thin Films Prepared from Chemically Exfoliated Carbon Nanotubes (CNTs), Highly Oriented Pyrolytic Graphite (HOPG), Natural Flake Graphite, and Carbon Powder [C] . Matthew M. Marchese, Rosario A. Gerhardt Materials Research Society Symposium DD on De Novo Carbon Nanomaterials . 2013

机译：石墨烯样薄膜的电导率由化学剥离碳纳米管（CNT），高度取向的热解石墨（HOPG），天然薄片石墨和碳粉制备
5. Covalent Organic Frameworks for the Catalytic Reduction of Carbon Dioxide [D] . Diercks, Christian S. 2018

机译：催化还原二氧化碳的共价有机骨架
6. Fabrication of holey graphene: Catalytic oxidation by metalloporphyrin–based covalent organic framework immobilized on highly ordered pyrolytic graphite [O] . Wanji Seo, David L. White, Alexander Star -1

机译：多孔石墨烯的制备：固定在高度有序热解石墨上的基于金属卟啉的共价有机骨架的催化氧化
7. Fabrication of Holey Graphene: Catalytic Oxidation by Metalloporphyrin-Based Covalent Organic Framework Immobilized on Highly Ordered Pyrolytic Graphite [O] . Wanji Seo, David L. White, Alexander Star 2017

机译：HOLENY石墨烯的制造：催化氧化通过固定在高度有序热解石墨上的金属卟啉基共价有机骨架

Fabrication of Holey Graphene: Catalytic Oxidation by Metalloporphyrin-Based Covalent Organic Framework Immobilized on Highly Ordered Pyrolytic Graphite

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