Two Porous Polyoxometalate-Resorcin[4]arene-Based Supramolecular Complexes: Selective Adsorption of Organic Dyes and Electrochemical Properties

Zhai Qiu-Yi; Su Juan; Guo Ting-Ting; Yang Jin; Ma Jian-Fang; Chen Jie-Sheng

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Two Porous Polyoxometalate-Resorcin[4]arene-Based Supramolecular Complexes: Selective Adsorption of Organic Dyes and Electrochemical Properties

机译：两种多孔多氧化膦 - 间晶体[4]基于芳烃的超分子复合物：选择性吸附有机染料和电化学性质

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Two new inorganic-organic hybrid complexes, namely, {[Co-4(L)(2)(HCOO)(2)(OH)(2)][SiO4(W3O9)(4)]}center dot 6DMF center dot 5H(2)O (1) and {[Zn-4(L)(2)(HCOO)(2)(OH)(2)][SiO4(W3O9)(4)]}center dot 6DMF center dot 5H(2)O (2), have been solvothermally prepared by using a new methyl imidazole functionalized resorcin[4]arene (L), polyoxometalate (POM), and metal cation. Isostructural 1 and 2 feature porous supramolecular architectures and represent an unusual example of a successful combination of resorcin[4]arenes with polyoxometalates. Remarkably, selective adsorptions for organic dyes were studied by using 1 and 2 as adsorbents. Moreover, their electrocatalytic activities for the oxidation of ascorbic acid and reduction of NaBrO3 were also studied.

机译：两种新的无机 - 有机杂交络合物，即（[CO-4（1）（2）（2）（HCOO）（2）（2）（2））] [SiO4（W3O9）（4）]}中心点6DMF中心点5H （2）O（1）和{[Zn-4（1）（2）（HCOO）（2）（2）（2）（2））] [SiO4（W3O9）（4）]}中心点6dmf中心点5h（2 ）O（2），通过使用新的甲基咪唑官能化的间体[4]芳烃（L），聚氧酸盐（POM）和金属阳离子来溶于溶剂。 Isostrontucture1和2特征多孔超分子架构，并表示具有多氧酸盐的共聚菌素[4]的成功组合的不寻常的例子。值得注意地，通过使用1和2作为吸附剂来研究用于有机染料的选择性吸附。此外，还研究了它们的抗坏血酸氧化和减少NaBro3的电催化活性。

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来源
《Crystal growth & design》 |2018年第10期|共8页
作者
Zhai Qiu-Yi; Su Juan; Guo Ting-Ting; Yang Jin; Ma Jian-Fang; Chen Jie-Sheng;
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Northeast Normal Univ Dept Chem Key Lab Polyoxometalate Sci Changchun 130024 Jilin Peoples R China;

Shanghai Jiao Tong Univ Sch Chem &

Chem Engn Shanghai 200240 Peoples R China;

Northeast Normal Univ Dept Chem Key Lab Polyoxometalate Sci Changchun 130024 Jilin Peoples R China;

Northeast Normal Univ Dept Chem Key Lab Polyoxometalate Sci Changchun 130024 Jilin Peoples R China;

Northeast Normal Univ Dept Chem Key Lab Polyoxometalate Sci Changchun 130024 Jilin Peoples R China;

Shanghai Jiao Tong Univ Sch Chem &

Chem Engn Shanghai 200240 Peoples R China;

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正文语种 eng
中图分类晶体学;
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1. Two Porous Polyoxometalate-Resorcin[4]arene-Based Supramolecular Complexes: Selective Adsorption of Organic Dyes and Electrochemical Properties [J] . Zhai Qiu-Yi, Su Juan, Guo Ting-Ting, Crystal growth & design . 2018,第10期

机译：两种多孔多氧化膦 - 间晶体[4]基于芳烃的超分子复合物：选择性吸附有机染料和电化学性质
2. pH-tuned diverse structures and properties: two Anderson-type polyoxometalate-based metal-organic complexes for selective photocatalysis and adsorption of organic dyes [J] . Wang Xiuli, Sun Junjun, Lin Hongyan, RSC Advances . 2016,第112期

机译：PH调节不同的结构和性质：两种Anderson型多氧化胍基金属 - 有机配合物，用于选择性光催化和吸附有机染料
3. pH-tuned diverse structures and properties: two Anderson-type polyoxometalate-based metal–organic complexes for selective photocatalysis and adsorption of organic dyes [J] . Xiuli Wang, Junjun Sun, Hongyan Lin, RSC Advances . 2016,第112期

机译：PH调节不同的结构和性质：两种Anderson型多氧化胍基金属 - 有机配合物，用于选择性光催化和吸附有机染料
4. Organic versus Hybrid Coacervate Complexes : Co-Assembly and Adsorption Properties [C] . J. Fresnais, J.F. Berret, L. Qi, NSTI BioNano Conference and Trade Show . 2008

机译：有机物与杂交凝聚件复合物：共组装和吸附性能
5. Design and Synthesis of Tunable Porous Organic Polymers for Selective Gas Adsorption [D] . Pandey, Prativa 2013

机译：用于选择性气体吸附的可调节多孔有机聚合物的设计与合成
6. Hierarchically porous silicon–carbon–nitrogen hybrid materials towards highly efficient and selective adsorption of organic dyes [O] . Lala Meng, Xiaofei Zhang, Yusheng Tang, -1

机译：分层多孔的硅-碳-氮杂化材料可高效高效地选择性吸附有机染料
7. Hierarchically porous silicon–carbon–nitrogen hybrid materials towards highly efficient and selective adsorption of organic dyes [O] . Lala Meng, Xiaofei Zhang, Yusheng Tang, 2015

机译：分层多孔硅 - 碳 - 氮杂交材料朝着高效和选择性吸附的有机染料

Two Porous Polyoxometalate-Resorcin[4]arene-Based Supramolecular Complexes: Selective Adsorption of Organic Dyes and Electrochemical Properties

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