Regulation of hydrophobicity and water adsorption of MIL-101(Cr) through post-synthetic modification

Li Yi; Wang Hao-Tian; Zhao Yan-Long; Lv Jie; Zhang Xin; Chen Qiang; Li Jian-Rong

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Regulation of hydrophobicity and water adsorption of MIL-101(Cr) through post-synthetic modification

机译：通过合成后修饰调节MIL-101（CR）的疏水性和水吸附

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Hydrophobic property of metal-organic frameworks (MOFs) is not only important for their stability improvement but also has a profound effect on the performance of many applications. The essence of coordination bonds led to most of the MOFs are hydrophilic and hydrophobic MOFs are generally achieved by hydrophobic modification of pore surface. Here, we report the systematic regulation of water adsorption and hydrophobic property of a classical MOF MIL-101(Cr) through post-synthetic modification. The contact angle (CA) of modified MIL-101 could vary from 17.9 degrees to 146.5 degrees by changing the alkyl chain length of primary amines. The water adsorption capacity and step pressure can also be tuned correspondingly.

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来源
《Inorganic Chemistry Communications》 |2021年第1期|共4页
作者
Li Yi; Wang Hao-Tian; Zhao Yan-Long; Lv Jie; Zhang Xin; Chen Qiang; Li Jian-Rong;
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作者单位

Beijing Univ Technol Fac Environm &

Life Beijing Key Lab Green Catalysis &

Separat Beijing 100124 Peoples R China;

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原文格式 PDF
正文语种 eng
中图分类无机化学;基本无机化学工业;
关键词
Hydrophobic; Water adsorption; Metal-organic framework; MIL-101(Cr); Post-synthetic modification;

机译：疏水性;水吸附;金属 - 有机框架;MIL-101（CR）;合成后修饰;

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专利

1. RuCl3 anchored onto post-synthetic modification MIL-101(Cr)-NH2 as heterogeneous catalyst for hydrogenation of CO2 to formic acid [J] . Shengping Wang, Shihui Hou, Chao Wu, 中国化学快报（英文版） . 2019,第002期
2. Heterogeneity of Adsorption Sites and Adsorption Kinetics of n-Hexane on Metal-Organic Framework MIL-101(Cr) [J] . Xuejiao Sun, Jinpeng Miao, Jing Xiao, 中国化学工程学报（英文版） . 2014,第009期
3. Enhancement of CO2 adsorption on nanoporous chromium terephthalate (MIL-101) by amine modification [J] . Mansoor Anbia, Vahid Hoseini 天然气化学（英文版） . 2012,第003期
4. Adsorption equilibrium and the effect of honeycomb heat exchanging device on charge/discharge characteristic of methane on MIL-101(Cr) and activated carbon [J] . Guobin Zhao, Qingrong Zheng, Xuan Zhang, 中国化学工程学报（英文版） . 2020,第007期
5. Ru(III) complex anchored onto amino-functionalized MIL-101(Cr) framework via post-synthetic modification: an efficient heterogeneous catalyst for ring opening of epoxides [J] . Jafari Aneseh Khalatbari, Kardanpour Reihaneh, Tangestaninejad Shahram, Journal of the Iranian Chemical Society . 2018,第5期

机译：Ru（III）通过合成后修饰锚定到氨基官能化的MIL-101（CR）框架上：环氧化环开口的有效的异质催化剂
6. Post-synthetic modification of MIL-101(Cr) with pyridine for high-performance liquid chromatographic separation of tocopherols [J] . Yang Fang, Yang Cheng-Xiong, Yan Xiu-Ping Talanta: The International Journal of Pure and Applied Analytical Chemistry . 2015,第Null期

机译：吡啶对MIL-101（Cr）的后合成修饰，用于高效液相色谱分离生育酚
7. Synthesis and post-synthetic modification of MIL-101(Cr)-NH_2 via a tandem diazotisation process [J] . Dongmei Jiang, Luke L. Keenan, Andrew D. Burrows, Chemical Communications . 2012,第99期

机译：通过串联重氮化工艺合成MIL-101（Cr）-NH_2及其后合成修饰
8. STUDY OF WASTE HEAT DRIVEN ADSORPTION COOLING SYSTEM EMPLOYING DOPED MIL-101(Cr) AND WATER AS ADSORBENT ADSORBATE PAIR [C] . Anutosh Chakraborty, Syed Muztuza Ali, How Wei Benjamin Teo ASME international mechanical engineering congress and exposition . 2016

机译：掺MIL-101（Cr）和水作为吸附剂对的废热驱动吸附冷却系统的研究
9. Sum frequency generation vibrational spectroscopy studies on model peptide adsorption at the hydrophobic solid-water and hydrophilic solid-water interfaces. [D] . York, Roger Louis. 2007

机译：总和频率产生振动光谱研究模型肽在疏水性固体-水和亲水性固体-水界面上的吸附。
10. Adsorption of Uranyl ions on Amine-functionalization of MIL-101(Cr) Nanoparticles by a Facile Coordination-based Post-synthetic strategy and X-ray Absorption Spectroscopy Studies [O] . Jian-Yong Zhang, Na Zhang, Linjuan Zhang, -1

机译：基于一种简单的配位后合成策略和X射线吸收光谱研究MIL-101（Cr）纳米粒子的胺功能化上铀离子的吸附。
11. Adsorption of Uranyl ions on Amine-functionalization of MIL-101(Cr) Nanoparticles by a Facile Coordination-based Post-synthetic strategy and X-ray Absorption Spectroscopy Studies [O] . Jian-Yong Zhang, Na Zhang, Linjuan Zhang, 2015

机译：通过基于体配位的合成后策略和X射线吸收光谱研究对MIL-101（Cr）纳米粒子胺官能化的铀酰离子的吸附
12. Sum Frequency Generation Vibrational Spectroscopy Studies on Model Peptide Adsorption at the Hydrophobic Solid-Water and Hydrophilic Solid-Water Interfaces [R] . York, R. L. 2007

机译：和谐频率生成振动光谱研究模型肽在疏水固 - 水和亲水固 - 水界面上的吸附

Regulation of hydrophobicity and water adsorption of MIL-101(Cr) through post-synthetic modification

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