An efficient method to prepare aryl acetates by the carbonylation of aryl methyl ethers or phenols

Zhang Dejin; Yang Guoqiang; Xiong Junping; Liu Jia; Hu Xingbang; Zhang Zhibing

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An efficient method to prepare aryl acetates by the carbonylation of aryl methyl ethers or phenols

机译：通过芳基甲基醚或酚的羰基化制备乙酸芳基乙酸的有效方法

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Synthesis of valuable chemicals from lignin based compounds is critical for the application of biomass. Here, we develop a method of preparing aryl acetates by the carbonylation of aryl methyl ethers or phenols under low CO pressure. Good to excellent yields of aryl acetates were obtained using different substrates, and a possible reaction mechanism was proposed by conducting a series of control experiments. This method may provide a potential way for the utilization of lignin.

机译：从木质素基化合物中合成有价值的化学品对于生物质的应用至关重要。在这里，我们开发了一种在低压下通过芳基甲醚或酚的羰基化制备芳基醋酸盐的方法。使用不同的底物可以获得良好到优异的产率，并通过一系列控制实验提出了可能的反应机理。该方法为木质素的利用提供了一条潜在的途径。

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来源
《New Journal of Chemistry》 |2021年第5期|共5页
作者
Zhang Dejin; Yang Guoqiang; Xiong Junping; Liu Jia; Hu Xingbang; Zhang Zhibing;
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作者单位

Nanjing Univ Sch Chem &

Chem Engn Nanjing 210093 Peoples R China;

Nanjing Univ Sch Chem &

Chem Engn Nanjing 210093 Peoples R China;

Nanjing Univ Sch Chem &

Chem Engn Nanjing 210093 Peoples R China;

Nanjing Univ Sch Chem &

Chem Engn Nanjing 210093 Peoples R China;

Nanjing Univ Sch Chem &

Chem Engn Nanjing 210093 Peoples R China;

Nanjing Univ Sch Chem &

Chem Engn Nanjing 210093 Peoples R China;

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正文语种 eng
中图分类化学;
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2. A new route to synthesize aryl acetates from carbonylation of aryl methyl ethers [J] . Qingqing Mei, Youdi Yang, Hangyu Liu, Science Advances . 2018,第5期

机译：由芳基甲基醚羰基化合成乙酸芳基酯的新途径
3. An approach of modifying poly(aryl ether ketone) to phenol-containing poly(aryl ether) and its application in preparing high-performance epoxy thermosets [J] . Lin C.H., Wang Y.R., Feng Y.R., Polymer: The International Journal for the Science and Technology of Polymers . 2013,第6期

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5. Preparation of Poly (aryl ether) Anion Ionomers with N-methyl imidazolium Groups [C] . Qunhui Hu, Wenxiao Wang, Shubo Wang, MST-S 2012;Spring International Conference on Material Sciences and Technology . 2012

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6. Heterogeneous catalysis of dimethyl ether and methanol: Oxidation to formaldehyde on supported metal oxides and carbonylation to methyl acetate on zeolites. [D] . Cheung, Patricia Wing-Kee. 2006

机译：二甲醚和甲醇的多相催化：在负载的金属氧化物上氧化为甲醛，在沸石上羰基化为乙酸甲酯。
7. A new route to synthesize aryl acetates from carbonylation of aryl methyl ethers [O] . Qingqing Mei, Youdi Yang, Hangyu Liu, 2018

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8. A new route to synthesize aryl acetates from carbonylation of aryl methyl ethers [O] . Qingqing Mei, Youdi Yang, Hangyu Liu, 2018

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机译：多面体低聚倍半硅氧烷 - 官能化全氟环丁基芳基醚聚合物：用全氟环丁基（pFCB）芳基醚聚合物共聚物功能化的多面体低聚倍半硅氧烷（pOss）的合成和性质概述

An efficient method to prepare aryl acetates by the carbonylation of aryl methyl ethers or phenols

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