Crystal phase-selective synthesis of intermetallic palladium borides and their phase-regulated (electro)catalytic properties

Li Zhenyu; Zhao Linmin; Chen HuiLiang XiaoAi XuanXie ZhoubingLi XiaotianYang FengLiu HongyangZou Xiaoxin

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Crystal phase-selective synthesis of intermetallic palladium borides and their phase-regulated (electro)catalytic properties

机译：金属间钯的晶体相选择性合成及其相调的（电）催化特性

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摘要

Three crystal phases of Pd–B intermetallics, namely, Pd6B, Pd5B2 and Pd2B, are synthesized, and their phase-dependent catalytic activities toward electrochemical water splitting and Suzuki coupling reactions are studied. In both reactions, their catalytic activities are found to increase in the order Pd, Pd6B, Pd5B2 and Pd2B. This activity trend is strongly associated with the Pd(d)–B(s,p) orbital hybridization-regulated surface adsorption properties.

机译：合成了PD – B间的三个晶体，即PD6B，PD5B2和PD2B，并研究了它们对电化学水分裂和铃木耦合反应的相位依赖性催化活性。在这两种反应中，发现它们的催化活性在PD，PD6B，PD5B2和PD2B方面增加。这种活性趋势与PD（D）–B（S，P）轨道杂交调节的表面吸附特性密切相关。

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来源
《Catalysis science & technology》 |2022年第4期|1038-1042|共5页
作者
Li Zhenyu; Zhao Linmin; Chen HuiLiang XiaoAi XuanXie ZhoubingLi XiaotianYang FengLiu HongyangZou Xiaoxin;
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作者单位

Jilin University;

Southern University of Science and Technology;

Chinese Academy of Sciences;

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原文格式 PDF
正文语种英语
中图分类汉语教学;
关键词
crystalline phase; Catalyst activity; Intermetallic compoundsBoron CompoundsBoridesREACTIONcrystalsadsorptive propertiesSuzuki coupling reactionwater splittingsynthesis;

机译：晶相;催化剂活性;金属间化合物木烷型木菌菌丝ccrystalsadsostalsative propertiesuzuki耦合耦合反应水分分裂合成;

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机译：Hydrothermal synthesis, crystal structures, and luminescent properties of a series of new lanthanide oxalatophosphonates with a layer architecture

Crystal phase-selective synthesis of intermetallic palladium borides and their phase-regulated (electro)catalytic properties

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