Catalytic hydrogenation of CO2 with unsymmetric N-heterocyclic carbene-nitrogen-phosphine ruthenium complexes

Ji Li; Cui Tianhua; Nie XufengZheng YanlingZheng XueliFu HaiyanYuan MaolinChen HuaXu JiaqiLi Ruixiang

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Catalytic hydrogenation of CO2 with unsymmetric N-heterocyclic carbene-nitrogen-phosphine ruthenium complexes

机译：与不对称催化加氢的二氧化碳氮杂carbene-nitrogen-phosphine钌配合物

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Unsymmetric Ru-CNP and Ru-CN(H)P complexes are synthesized and applied in the hydrogenation of CO2 to formate for the first time. The Ru-CNP complex shows excellent stability and high activity. The TON is around 170 000 after 48 h at 200 degrees C, which is a relatively high record value among all the Ru complexes.

机译：不对称Ru-CNP和Ru-CN (H) P复合物合成和应用的加氢二氧化碳为第一次甲酸。复杂的显示了卓越的稳定性和高活动。200摄氏度,这是一个相对较高的记录值在所有俄文复合物。

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来源
《Catalysis science & technology》 |2021年第21期|6965-6969|共5页
作者
Ji Li; Cui Tianhua; Nie XufengZheng YanlingZheng XueliFu HaiyanYuan MaolinChen HuaXu JiaqiLi Ruixiang;
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作者单位

Sichuan Univ, Coll Chem, Minist Educ, Key Lab Green Chem & Technol, Chengdu 610064, Sichuan, Peoples R China;

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正文语种英语
中图分类汉语教学;
关键词
Catalysis; formate; Carbon DioxideRutheniumHydrogenationTon;

机译：催化;甲酸;碳;

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Catalytic hydrogenation of CO2 with unsymmetric N-heterocyclic carbene-nitrogen-phosphine ruthenium complexes

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