Isopropanol as a hydrogen source for single atom cobalt-catalyzed Wacker-type oxidation

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Isopropanol as a hydrogen source for single atom cobalt-catalyzed Wacker-type oxidation

机译：异丙醇作为单原子氢源cobalt-catalyzed Wacker-type氧化

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The first example of a heterogeneous cobalt catalytic system for Wacker-type oxidation catalyzed by a single atom dispersed Co-N/C catalyst using alcohol as the hydrogen source under an oxygen atmosphere is presented. By combining a well-designed, controlled experiment and various methods of characterization, we determined that single atom cobalt was the active center rather than nanoparticle or oxide counterparts.

机译：第一个例子的异构钴Wacker-type氧化催化体系由一个原子催化分散Co-N / C使用酒精作为催化剂氢源在氧气气氛。结合一个设计良好的控制实验各种方法的描述,我们确定单原子钴是活跃的中心而不是纳米颗粒或氧化物同行。

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《Catalysis science & technology》 |2020年第9期|2769-2773|共5页
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正文语种英语
中图分类汉语教学;
关键词
Hydrogen; OXYGEN ATMOSPHERE; OxidationNanoparticlesAtomsACTIVE CENTRESingle;

机译：氢、氧气氛;OxidationNanoparticlesAtomsACTIVE;

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1. Recyclable Palladium Catalyst in PEG/CH_3CN Biphasic System for Electro-oxidative Wacker-type Reaction [J] . Koichi MITSUDO, Satoshi FUKUNAGA, Tomoya FUJITAHiroki MANDAISeiji SUGAHideo TANAKA 電気化学および工業物理化学 . 2013,第5期

机译：可回收钯催化剂/ CH_3CN挂钩两相的系统Electro-oxidative Wacker-type反应
2. Cobalt-catalyzed C(sp(2))-H/C(sp(3))-H coupling via directed C-H activation and 1,5-hydrogen atom transfer [J] . Sun Qiao, Yoshikai Naohiko Organic Chemistry Frontiers . 2018,第4期

机译：Cobalt-catalyzed C (sp (2)) - h / C - h耦合(sp (3))通过直接碳氢键活化,5-hydrogen原子转移
3. Cobalt-catalyzed hydrogen desorption from the LiNH2–LiBH4 system [O] . Henderson, William, Linklater, Rachael A., Cameron, Nicola E., 2008

机译：Cobalt-catalyzed hydrogen desorption from the LiNH2–LiBH4 system

Isopropanol as a hydrogen source for single atom cobalt-catalyzed Wacker-type oxidation

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