Oxide/Electrolyte interface: Electron transfer phenomena

Fernandez-Ibanfz P.; Malato S.

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Oxide/Electrolyte interface: Electron transfer phenomena

机译：氧化物/电解质界面：电子转移现象

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Electron transfer on a titamum dioxide I electrolyte solution interface has been studied. As observed by other researchers on similar interfaces (TiO_2- and ZnO- electrolyte solution), slow consumption of OH~- ions was found.A theoretical model has been developed for calculating the change in Fermi energy levels of both electrolyte solution and semi-conductor, showing that ion consumption from the solution is favoured by a decreased difference in their Fermi energies. A kinetic constant (v) is found to characterise the consumption process, its value increasing with electrolyte and semiconductor mass concentrations. Furthermore, this process may be used to estimate the point of zero charge of a titanium dioxide colloidal dispersion.

机译：已经研究了在二氧化钛I电解质溶液界面上的电子转移。正如其他研究人员在类似界面（TiO_2-和ZnO-电解质溶液）上观察到的那样，发现OH〜-离子消耗缓慢。已建立了一个理论模型来计算电解质溶液和半导体的费米能级的变化，表明溶液中的离子消耗因其费米能量的减小而受到促进。发现动力学常数（v）表征了消耗过程，其值随电解质和半导体质量浓度的增加而增加。此外，该过程可用于估计二氧化钛胶体分散体的零电荷点。

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《Boletin de la Sociedad Espanola de Ceramica y Vidrio》 |2000年第4期|共7页
作者
Fernandez-Ibanfz P.; Malato S.;
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中图分类硅酸盐工业;
关键词
titanium dioxide; fermi level; point of zero charge; electrophoretic mobility.;

机译：二氧化钛;费米能级;零电荷点;电泳迁移率;

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1. Oxide/Electrolyte interface: Electron transfer phenomena [J] . Fernandez-Ibanfz P., Malato S. Boletin de la Sociedad Espanola de Ceramica y Vidrio . 2000,第4期

机译：氧化物/电解质界面：电子转移现象
2. Theory for Influence of the Metal Electrolyte Interface on Heterogeneous Electron Transfer Rate Constant: Fractional Electron Transferred Transition State Approach [J] . Kant Rama, Kaur Jasmin, Mishra Gaurav Kumar The journal of physical chemistry, C. Nanomaterials and interfaces . 2020,第4期

机译：金属电解质界面对非均相电子传递速率恒定的影响理论：分数电子转移过渡状态方法
3. Electron Transfer at the Metal Oxide/Electrolyte Interface: A Simple Methodology for Quantitative Kinetics Evaluation [J] . Azcarate Iban, Costentin Cyrille, Methivier Christophe, The journal of physical chemistry, C. Nanomaterials and interfaces . 2018,第24期

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4. Interface Chemistry and Charge Transfer Resistances at the Interface of the Nasicon Solid Electrolyte and Oxide Cathode System [C] . Anisur Rahman, Bilge Yildiz Meeting of the Electrochemical Society;International Meeting on Chemical Sensors . 2020

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5. Ionic and electronic transport across interfaces in thin electrolyte film, anode supported solid oxide fuel cells. [D] . Lim, Hyung-Tae. 2009

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7. Electroneutrality Coupling of Electron Transfer at an Electrode Surface and Ion Transfer across the Interface between Thin-layer of 1-Octyl-3-methylimidazolium Bis(perfluoroalkylsulfonyl)imide Covering the Electrode Surface and an Outer Electrolyte Solution [O] . Kazuyuki TANAKA, Naoya NISHI, Takashi KAKIUCHI 2004

机译：电极表面的电阻耦合电极表面和离子转移穿过覆盖电极表面和外电解质溶液的1-辛基-3-甲基咪唑鎓双（全氟烷基磺酰基）酰亚胺的薄层之间的界面

Oxide/Electrolyte interface: Electron transfer phenomena

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