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Path-length-resolved dynamic light scattering: modeling the transition from single to diffusive scattering

机译:解析路径长度的动态光散射:模拟从单一散射到扩散散射的过渡

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摘要

Dynamic light-scattering spectroscopy is used to study Brownian motion within highly scattering samples. The fluctuations of the light field that is backscattered by a suspension of polystyrene microspheres are measured as power spectra by use of low-coherence interferometry to obtain path-length resolution. The data are modeled as the sum of contributions to the detected light weighted by a Poisson probability for the number of events that each component has experienced. By analyzing the broadening of the power spectra as a function of the path length for various sizes of particles, we determine the contribution of multiple scattering to the detected signal as a function of scattering anisotropy.
机译:动态光散射光谱法用于研究高散射样品中的布朗运动。通过使用低相干干涉测量法测量由聚苯乙烯微球悬浮液反向散射的光场的波动,作为功率谱,以获得光程分辨率。数据被建模为对每个组件经历的事件数的由泊松概率加权的检测光贡献的总和。通过分析功率谱的拓宽与各种尺寸粒子的路径长度的关系,我们确定了多次散射对检测信号的贡献,即散射各向异性的函数。

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