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Influence of particle size on the ice nucleating ability of mineral dusts

机译:粒径对矿物粉尘冰核能力的影响

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摘要

The recently developed Zurich Ice Nucleation Chamber (ZINC) was used to explore ice nucleation of size-selected mineral dust particles at temperatures between -20°C and -55°C. Four different mineral dust species have been tested: montmorillonite, kaolinite, illite and Arizona test dust (ATD). The selected particle diameters are 100 nm, 200 nm, 400 nm and 800 nm. Relative humidities with respect to ice (RH,) required to activate 1 % of the dust particles as ice nuclei (IN) are reported as a function of temperature. An explicit size dependence of the ice formation efficiency has been observed for all dust types. 800nm particles required the lowest RH_i to activate. Deposition nucleation below water saturation was found only below -30°C or -35°C dependent on particle size. Minimum RH_i for 1% activation were 105% for illite, kaolinite and montmorillonite at -40°C, respectively 110% for ATD at -45°C. In addition, a possible parameterisation for the measured activation spectra is proposed, which could be used in modeling studies.
机译:最近开发的苏黎世冰核室(ZINC)用于在-20°C至-55°C的温度下探索选定尺寸的矿物粉尘颗粒的冰核。已测试了四种不同的矿物粉尘:蒙脱土,高岭石,伊利石和亚利桑那粉尘(ATD)。选择的粒径是100nm,200nm,400nm和800nm。据报道,将1%的尘埃颗粒激活为冰核(IN)所需的相对于冰的相对湿度(RH)是温度的函数。对于所有粉尘类型,已经观察到冰形成效率的明显尺寸依赖性。 800nm的颗粒需要最低的RH_i才能激活。仅在低于-30°C或-35°C以下才发现水饱和以下的沉积成核,具体取决于粒径。 1%活化的最低RH_i在-40°C下为伊利石,高岭石和蒙脱石的105%,在-45°C下为ATD的分别为110%。另外,提出了用于测量的活化谱的可能参数化,其可以用于建模研究中。

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