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Effects of dust particle internal structure on light scattering

机译:尘粒内部结构对光散射的影响

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There is a large variety of internal structures inside atmospheric dust particles, making them inherently inhomogeneous. Such structures may have a large effect on ground-level and atmospheric radiation. So far, dust particle internal structures and their effect on the light scattering properties have proved to be hard to quantify, in part due to challenges in obtaining information about these structures. Recently, internal structures of individual dust particles were revealed through focused ion beam milling and analyzed. Here, we perform a sensitivity study to evaluate the optical impacts of some of the typical internal structures revealed. To obtain suitable model particles, the first step is to generate inhomogeneous particles with varying internal structures by using an algorithm that is based on three-dimensional Voronoi tessellation. The parameters for the particle generation are obtained from studies of real-world Asian dust particles. The second step is to generate homogeneous versions of the generated particles by using an effective-medium approximation, for comparison. Third, light scattering by both versions of these particles is simulated with discrete dipole approximation code. This allows us to see how different internal structures affect light scattering, and how important it is to account for these structures explicitly. Further, this allows us to estimate the potential inaccuracies caused by using only homogeneous model particles for atmospheric studies and remote-sensing measurements. The results show that the effects vary greatly between different kinds of internal structures and single-scattering quantity considered, but for most structure types the effects are overall notable. Most significantly, hematite inclusions in particles impact light scattering heavily. Furthermore, internal pores and hematite-rich coating both affect some form of light scattering noticeably. Based on this work, it seems that it is exceedingly important that the effects of dust particle internal structures on light scattering are accounted for in a wide variety of applications.
机译:大气尘埃颗粒内部有各种各样的内部结构,使其固有地不均匀。这样的结构可能对地面和大气辐射产生很大影响。到目前为止,已证明很难量化灰尘颗粒的内部结构及其对光散射特性的影响,部分原因是在获取有关这些结构的信息方面存在挑战。最近,通过聚焦离子束研磨揭示并分析了单个尘埃颗粒的内部结构。在这里,我们进行了敏感性研究,以评估所揭示的一些典型内部结构的光学影响。为了获得合适的模型粒子,第一步是使用基于三维Voronoi细分的算法来生成具有变化内部结构的不均匀粒子。颗粒生成的参数是通过对现实世界中亚洲尘埃颗粒的研究获得的。第二步是通过使用有效介质近似来生成生成粒子的均匀形式,以进行比较。第三,使用离散偶极近似代码模拟了这两种粒子的两个版本的光散射。这使我们能够看到不同的内部结构如何影响光散射,以及明确说明这些结构的重要性。此外,这使我们能够估计由于仅将均质模型粒子用于大气研究和遥感测量而引起的潜在误差。结果表明,不同种类的内部结构和所考虑的单散射量之间的影响差异很大,但对于大多数结构类型而言,效果总体上是显着的。最重要的是,颗粒中的赤铁矿夹杂物会严重影响光散射。此外,内部孔隙和富含赤铁矿的涂层都会明显影响某种形式的光散射。基于这项工作,在各种应用中考虑灰尘颗粒内部结构对光散射的影响似乎极为重要。

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