A novel heterostranded double-helical coordination polymer with chiral channels emitting blue fluorescence

Zhengfang Tian; Haibao Duan; Fang Xuan

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A novel heterostranded double-helical coordination polymer with chiral channels emitting blue fluorescence

机译：具有手性通道发射蓝色荧光的新型异链双螺旋配位聚合物

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摘要

A novel heterostranded double-helical coordination polymer is self-assembly from two flexible ligands, 4-carboxymethylbenzoic acid (H2L) and 1,1'-(1,4-butanediyl)bis(imidazole) (abbr. as bbi), with Zn~(2+) ion under solvent-thermal condition. The heterostranded double-helix constructs a chiral channel, which is filled by lattice water molecules;; the adjacent heterostranded double-helical channels share Zn~(2+) ions to develop into a homochiral helical two-dimensional sheet, and the right- and left-handed chiral sheets further array in an alternating fashion to generate a racemic crystal via van de Waals forces. This coordination polymer emits blue fluorescence in the solid state.

机译：一种新型的异链双螺旋配位聚合物是由两个柔性配体（4-羧甲基苯甲酸（H2L）和1,1'-（1,4-丁二基）双咪唑）（简称bbi）自组装而成，并带有锌溶剂-热条件下的〜（2+）离子。异链双螺旋构成手性通道，该通道被晶格水分子填充;相邻的异链双螺旋通道共享Zn〜（2+）离子，发展为同手性螺旋二维片，右手和左手性片进一步交替排列以通过van de生成外消旋晶体华力。该配位聚合物以固态发射蓝色荧光。

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《Inorganic Chemistry Communications》 |2009年第5期|共3页
作者
Zhengfang Tian; Haibao Duan; Fang Xuan;
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正文语种 eng
中图分类化学工业;
关键词
4-Carboxymethylbenzoic acid; 1; 1'-(1; 4-Butanediyl)bis(imidazole); Coordination polymer; Heterostranded double-helix; Blue fluorescence;

机译：4-羧甲基苯甲酸;1;1'-（1;4-丁二基）双（咪唑）;配位聚合物;杂多双螺旋;蓝色荧光;

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专利

1. A novel heterostranded double-helical coordination polymer with chiral channels emitting blue fluorescence [J] . Zhengfang Tian, Haibao Duan, Fang Xuan Inorganic Chemistry Communications . 2009,第5期

机译：具有手性通道发射蓝色荧光的新型异链双螺旋配位聚合物
2. Blue fluorescence emission property of a metal-organic coordination polymer with one-dimensional channels [J] . Feng D., Liu S., Zhang W., Zeitschrift fur Anorganische und Allgemeine Chemie . 2010,第6期

机译：具有一维通道的金属有机配位聚合物的蓝色荧光发射特性
3. 2-D zinc coordination polymer with ellipse-like channels and blue fluorescence [J] . Ling Xu, Bing Liu, Guocong Guo, Inorganic Chemistry Communications . 2006,第2期

机译：具有椭圆形通道和蓝色荧光的二维锌配位聚合物
4. Efficient and saturated blue organic polymer light emitting devices with an oxadiazole containing poly (fluorene) polymer emissive layer [C] . Shu-jen Lee, Joseph R. Gallegos, Julien Klein, Society of Photo-Optical Instrumentation Engineers Conference on Organic Light-Emitting Materials and Devices . 2003

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A novel heterostranded double-helical coordination polymer with chiral channels emitting blue fluorescence

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