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Regeneration of spent catalysts in oxy-combustion atmosphere

机译:氧燃烧气氛中废催化剂的再生

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摘要

The feasibility of adopting an oxy-combustion stage to regenerate a spent catalyst proposed for methane thermo-catalytic decomposition has been investigated in a laboratory scale bubbling fluidized bed reactor operated at 800 C and different inlet oxygen concentrations. The efficiency of carbon oxy-combustion regeneration strategy has been evaluated on the basis of the efficiency of carbon removed from the catalyst and the performance of regenerated catalyst. The effect of multiple cycles of decomposition and regeneration steps has been also quantified. Experimental activity confirmed the possibility of producing a CO2 stream that can be finalized to a sequestration unit but also indicated the requirement of a good temperature control of catalytic particles.
机译:在实验室规模的鼓泡流化床反应器中,在800℃和不同的入口氧气浓度下进行了研究,研究了采用氧燃烧阶段来再生提议用于甲烷热催化分解的废催化剂的可行性。基于从催化剂除去的碳的效率和再生的催化剂的性能,已经评估了碳氧燃烧再生策略的效率。还已经量化了分解和再生步骤的多个循环的影响。实验活动证实了产生可以最终封存到螯合单元的CO 2物流的可能性,但也表明需要对催化剂颗粒进行良好的温度控制。

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