Stability of metallic thin films studied with a free electron model

Biao Wu; Zhenyu Zhang

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Stability of metallic thin films studied with a free electron model

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摘要

The stability of metallic thin films is studied with a free electron model, which is popularly known as the model of "particle in a box." A detailed theoretical framework is presented, along with discussion on typical metals, such as Pb, Al, Ag, Na, and Be. This simple model is found to be able to describe well the oscillation pattern of stability for continuous metallic films. In particular, it yields even-odd oscillations in the stability of Pb(111) film, consistent with both experimental observation and ab initio results. However, the free electron model is too crude to predict at what thickness a film is stable. Film stability is further examined with a model of "particle in a corrugated box," where a lattice potential is added along the vertical direction of a film. The effect of lattice potential is found not substantial.

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《Physical review, B. Condensed matter and materials physics》 |2008年第3期|035410.1-035410.12|共9页
作者
Biao Wu; Zhenyu Zhang;
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作者单位

Institute of Physics, Chinese Academy of Sciences, P.O. Box 603, Beijing 100080, People's Republic of China;

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原文格式 PDF
正文语种英语
中图分类固体物理学;
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thin film structure and morphology; quantum wells; total energy and cohesive energy calculations;

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Stability of metallic thin films studied with a free electron model

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