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Near-field properties of a gold nanoparticle array on different substrates excited by a femtosecond laser

机译:飞秒激光在不同基底上形成金纳米粒子阵列的近场特性

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In this paper we present experimental and theoretical results on the properties of the electromagnetic field in the near-field zone of gold nanoparticles excited by an 800 nm ultrashort laser pulse. The near-field properties are studied for the case of a single isolated particle and 2D nanoparticle array case. Particles are deposited on different substrates: metal (Au), semiconductor (Si) and dielectric (SiO_2). The calculations based on the finite difference time domain (FDTD) simulation technique predict that the field in the vicinity of the particles is enhanced as the magnitude of the field intensity depends on the substrate material and the interparticle distance for 2D array. For closely arrayed nanoparticles on the gold substrate, the maximal field intensity is more than two times lower than that of a single particle. With the increase of the distance between 200 nm diameter gold particles, the value of the field intensity increases up to a distance of about 800 nm. The theoretical prediction of the field enhancement on the substrate is confirmed experimentally. The irradiation of the nanoparticles deposited on the three different substrates with a single laser pulse of a Ti:sapphire laser results in a nanohole formation. Discussion on the observed properties is presented.
机译:在本文中,我们介绍了由800 nm超短激光脉冲激发的金纳米颗粒的近场区中电磁场特性的实验和理论结果。研究了单个分离粒子和二维纳米粒子阵列情况的近场特性。粒子沉积在不同的基板上:金属(Au),半导体(Si)和电介质(SiO_2)。基于有限时域(FDTD)模拟技术的计算预测,随着场强的大小取决于2D阵列的基板材料和粒子间距离,粒子附近的场会增强。对于在金基底上紧密排列的纳米粒子,最大场强比单个粒子的场强低两倍以上。随着直径200 nm的金颗粒之间距离的增加,场强的值增加到大约800 nm的距离。实验证实了在衬底上的场增强的理论预测。用Ti:蓝宝石激光器的单个激光脉冲辐照沉积在三个不同基板上的纳米颗粒会形成纳米孔。提出了关于观察到的性质的讨论。

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